The excitation of a low-energy ground state helium beam to its metastable states by electron impact is analysed. It is shown that the narrowest velocity distribution for the resulting metastable helium beam is obtained by directing the helium and electron beams parallel or antiparallel. A source of metastable helium atoms was constructed according to this analysis which produced a beam of 3*10 14 metastable atoms/s sr with a velocity resolution of 3% FWHM for a room-temperature beam (E=66 meV). A possible source of errors in time-of-flight experiments with metastable atoms is pointed out.
Describes the construction and characterisation of a pulsed, superthermal molecular beam source incorporating a rotor accelerator and a synchronously pulsed electron bombarder. The addition of the pulsed bombarder greatly improves the kinetic energy resolution of the superthermal metastable atomic and molecular beams, particularly for light particles at low velocities and eliminates problems of 'wrap-around' at low velocities. The optimum conditions of resolution at a desired signal level are discussed: a typical velocity distribution for Ar( 3 P 2 ) at a most probable beam velocity of 1500 m s -1 would have a standard deviation sigma approximately=0.07.
The supersonic short-pulse helium atomic beam and its metastables were studied. A pulsed high-density helium atomic beam was ejected from a nozzle, collimated by a skimmer and then flowed through a penning-type discharge device. After discharging, the metastable density of the pulsed helium atomic beam was up to 1.24 × 10 11 cm −3 . Excellent symmetry of atomic beam profile was obtained. The deviation of angle of the atomic beam with respect to the axis was less than 0.14°. The mean diffusion angle of the pulsed beam was 4°, and a mean velocity of atomic beam was up to 1350 ms −1 . Laser induced fluorescence of metastable atoms has been studied.
A time-of-flight technique has been used to measure the radiative lifetime of the
21S0 state of helium. After passing from a cooled source, helium atoms are excited by a pulsed anti-parallel electron beam. The atomic beam then contains not only ground-state helium atoms but also metastable atoms in both the
23S1 and the
21S0 states. The metastable atoms are detected at two positions, 1.9 and 6.7 m from the electron gun, by Auger ejection of an electron from a copper target, the first of which is a 60% transmitting mesh. Ground-state helium atoms cannot cause an electron to be ejected and hence are not detected. The time-of-flight distribution for the metastable
21S0 state is separated from that of the
23S1 state by illuminating the beam with an rf-discharge helium lamp. The
21S0 state is quenched by resonant absorption of a 20 581 - \AA{}A photon, raising the atom to the
21P1 state, which then decays preferentially to the
1S0 ground state; the
23S1 state remains unaffected because it is the ground state for the triplet system. The time-of-flight distribution for the
21S0 atoms is therefore obtained from the difference between the full beam and the quenched beam. A comparison of the number of
21S0 metastables within a given velocity interval at the two detectors determines the number which decay in flight and yields a value for the two-photon radiative lifetime. The value of the singlet lifetime for both
He3 and
He4 is 19.7 \ifmmode\pm\else\textpm\fi{} 1.0 msec, agreeing with the theoretical value of 19.5 msec, but disagreeing with the value 38 \ifmmode\pm\else\textpm\fi{} 8 msec measured by Pearl using a movable detector. The 1.0-msec error is an estimate of the remaining systematic errors in the experiment.
In this work I report on the development of a Magneto Optic Trap (MOT) for metastable helium atoms (He*). The metastable helium atoms are produced in a discharge nozzle source and collimated, slowed and compressed to provide a slow bright beam for loading the trap. The trap confines approximately 107 atoms, has a diameter of about 3 mm and with temperature approximately 1 mK. The trap is used for intra-trap and electron-atom scattering experiments. The results from these two experiments are reported. The electron scattering experiment is unique and employs a He* MOT for the first time, in combination with a new diagnostic technique (Phase Modulation Spectroscopy) to measure the trap loss. The results of these experiments have yielded the first total electron-metastable atom collision cross section measurements at intermediate (10-100 eV) electron energies.