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Physical review. B, Condensed matter

1n expansion for quantum Heisenberg antiferromagnets

G. C. Psaltakis

Published Feb 1, 1989• 3 citations
Publisher

Abstract

The quantum Heisenberg antiferromagnet is expressed in terms of physical electron operators, with a constraint to one electron per site, as it emerges in the large-$U$ limit of the Hubbard model. It is then possible to carry out a systematic $\frac{1}{n}$ expansion built on a translation-invariant singlet ground state. Such an expansion yields a Fermi-liquid picture for the elementary excitations which should be appropriate for low-dimensional antiferromagnets. Explicit calculations in one dimension show that the excitation spectrum consists of a gapless continuum in qualitative agreement with exact Bethe ansatz results.

DOI
10.1103/physrevb.39.2834

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The quantum Heisenberg antiferromagnet is expressed in terms of physical electron operators, with a constraint to one electron per site, as it emerges in the large-UUU limit of the Hubbard model. It is then possible to carry out a systematic 1n\frac{1}{n}n1​ expansion built on a translation-invariant singlet ground state. Such an expansion yields a Fermi-liquid picture for the elementary excitations which should be appropriate for low-dimensional antiferromagnets. Explicit calculations in one dimension show that the excitation spectrum consists of a gapless continuum in qualitative agreement with exact Bethe ansatz results.
The spin fluctuations parallel to the external magnetic field in the ground state of the one-dimensional (1D) s=12s=\frac{1}{2}s=21​ Heisenberg antiferromagnet are dominated by a two-parameter set of collective excitations. In a cyclic chain of N sites and magnetization 0<Mz<N/2,0<{M}_{z}<N/2,0<Mz​<N/2, the ground state, which contains 2Mz{2M}_{z}2Mz​ spinons, is reconfigured as the physical vacuum for a different species of quasiparticles, identifiable in the framework of the coordinate Bethe ansatz by characteristic configurations of Bethe quantum numbers. The dynamically dominant excitations are found to be scattering states of two such quasiparticles. For $\stackrel{\ensuremath{\rightarrow}}{N}\ensuremath{\infty},$ these collective excitations form a continuum in $(q,\ensuremath{\omega})$ space with an incommensurate soft mode. Their matrix elements in the dynamic spin structure factor ${S}_{\mathrm{zz}}(q,\ensuremath{\omega})$ are calculated directly from the Bethe wave functions for finite N. The resulting line- shape predictions for $\stackrel{\ensuremath{\rightarrow}}{N}\ensuremath{\infty}$ complement the exact results previously derived via algebraic analysis for the exact two-spinon part of ${S}_{\mathrm{zz}}(q,\ensuremath{\omega})$ in the zero-field limit. They are relevant for neutron-scattering experiments on quasi-1D antiferromagnetic compounds in a strong magnetic field.
A Wigner-Jordan (WJ) transformation is used to study the one-dimensional (1D) and two-dimensional (2D) quantum antiferromagnetic Heisenberg model. The advantage of using the Wigner-Jordan transformation is that it preserves all spin-commutation relations as well as the spin on-site exclusion principle. In the 1D case a nearest-neighbor covalent-bonding state of the WJ fermions is found to have a ground-state energy (-0.4351J per site) comparable with that from the Bethe-ansatz solution (-0.4431J per site), and a linear energy spectrum at low energies with velocity 1.6366J, in close agreement with the velocity obtained by Haldane for the quantum antiferromagnetic Heisenberg model with 1/d2{\mathit{d}}^{2}d2 interaction (1.5708J). The method used for studying the 1D model is then applied to the 2D Heisenberg model in a square lattice. The resulting state at finite temperature is the in-phase flux state, i.e., a flux state of the Wigner-Jordan spinless fermions with an in-phase fermion orbital current circulating around each elementary plaquette.The single-particle excitation spectrum, i.e., the energy dispersion of reversing orientation of a spin in the system, of the in-phase flux state is overall similar to that of spin waves, with significant difference near the edge point k=(\ensuremath{\pi},0), at which the excitation energy of the WJ fermion is zero, whereas that of the spin-wave excitation is 2J. The specific heat of the in-phase flux state predicts a correct temperature dependence over the entire temperature range, namely a T2{\mathit{T}}^{2}T2 dependence at low temperature, a peak near T/J=0.6, and a 1/T2{\mathit{T}}^{2}T2 decreasing at high temperature. It also gives excellent agreement with the specific heat calculated from numerical methods. In contrast, the spin-wave theory only correctly predicts a T2{\mathit{T}}^{2}T2 dependence at low temperature. The Raman spectrum of the in-phase flux state is calculated and shows significant improvement over that from spin-wave theories compared with the experimental spectrum of La2{\mathrm{La}}_{2}La2​CuO4{\mathrm{CuO}}_{4}CuO4​. The exchange parameter, J, obtained from the comparison is 1060 ${\mathrm{cm}}^{\mathrm{\ensuremath{-}}1}$, in agreement with that obtained from analyzing the neutron-scattering data.
The two-dimensional Hubbard model is extended by placing 2S orbitals at each lattice site and studied in a systematic 1/S expansion. The 1/S results for the magnetic susceptibility and the spectra of spin-wave excitations at half-filling are consistent with the large S calculations for the Heisenberg antiferromagnet. The 1/S corrections to the fermionic spectrum lift the degeneracy along the edge of the magnetic Brillouin zone yielding minima at (\ifmmode\pm\else\textpm\fi{}\ensuremath{\pi}/2,\ifmmode\pm\else\textpm\fi{}\ensuremath{\pi}/2). Relation to previous papers on the subject is discussed.
We consider quantum spin systems with dimerization, which at strong coupling have singlet ground states. To account for strong correlations, the S=1S\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}1S=1 elementary excitations are described as a dilute Bose gas with infinite on-site repulsion. This approach is applied to the two-layer Heisenberg antiferromagnet at T=0T\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}0T=0 with general couplings. Our analytic results for the triplet gap, the excitation spectrum, and the location of the quantum critical point are in excellent agreement with numerical results obtained by dimer series expansions.
We have developed a general scheme for carrying out systematic perturbation expansions for groundstate properties of quantum lattice models. As an application, we study the onset of spontaneous N\'eel order in S=12S=\frac{1}{2}S=21​ Heisenberg antiferromagnets by expanding around dimerized Hamiltonians. In one dimension (1D) we recover accurately the known exact results. On the square lattice we find novel critical points separating N\'eel ordered and disordered phases; the estimated critical exponents are consistent with those of the 3D classical Heisenberg model.
The authors investigate the properties of the two-dimensional quantum S=1/2 Heisenberg antiferromagnetic model on a square lattice by means of a block approach. The lattice is divided into four spin square blocks and the Hamiltonian is expressed in terms of low-energy block states. In the framework of the mean-field theory based on the 'auxiliary-boson' formalism; they show that the spin excitation spectrum contains one singlet mode with the temperature-dependent gap and three degenerate triplet modes. The asymptotic low-temperature spin-spin correlations are proportional to R -3/2 exp(-R(1/ xi 1 +1/ xi 2 )), where xi 1 =exp(A/T), xi 2 =constant and A approximately=0.5J. The uniform susceptibility tends to zero in agreement with numerical results; the energy per site is close to -0.57J. Beyond the meanfield theory the authors find gapless collective excitations analogous to the gapless mode in the neutral Fermi gas with attraction.