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Physical Review A

Optical-double-resonance spectra and intensity-intensity correlations under intense fields with finite bandwidths: Some analytical results

S. V. Lawande, Ravinder Rupchand Puri, Richard D’Souza

Published Apr 1, 1986• 12 citations
Publisher

Abstract

A formalism is presented to treat the effects of finite-bandwidth excitations on the fluorescent spectra and second-order intensity-correlation functions in optical double resonance. It is assumed that the bandwidth arises from the phase and/or amplitude fluctuations in the fields driving a three-level atom. Under the conditions that one or both these fields are intense, secular approximation and the theory of multiplicative stochastic processes are invoked to derive a Markovian master equation for the atomic-density operator averaged over both phase and amplitude ensembles. The quantum regression theorem is used to derive analytical expressions for the fluorescent spectra and the second-order intensity-correlation functions.

DOI
10.1103/physreva.33.2504

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Journal of Physics B Atomic and Molecular Physics•Aug 28, 1986•8 citations
A formalism is presented to treat the effects of finite-bandwidth excitations on the fluorescent spectra and second-order intensity-correlation functions in optical double resonance. It is assumed that the bandwidth arises from the phase and/or amplitude fluctuations in the fields driving a three-level atom. Under the conditions that one or both these fields are intense, secular approximation and the theory of multiplicative stochastic processes are invoked to derive a Markovian master equation for the atomic-density operator averaged over both phase and amplitude ensembles. The quantum regression theorem is used to derive analytical expressions for the fluorescent spectra and the second-order intensity-correlation functions.
We generalize our earlier formalism to treat the effects of both the finite-bandwidth excitations and finite arbitrary detunings, on the fluorescent spectra and second-order intensity correlation functions in optical double resonance. It is assumed that the bandwidth arises from the phase and/or amplitude fluctuations in the fields driving a three-level atom in cascade configuration. Under the conditions that one or both of these fields are intense, secular approximation and the theory of multiplicative stochastic processes are invoked to derive a Markovian master equation for the atomic-density operator averaged over both phase and amplitude. The quantum regression theorem is used to derive analytical expressions for the fluorescent spectra and the second-order intensity correlation functions which explicitly display the effects due to detunings and fluctuations.
We study fluorescence from a three-level atom in a cascade configuration driven by two coherent fields and damped by a broadband squeezed vacuum. Under the conditions that one or both of these fields are intense, a secular approximation is invoked to derive an analytical solution of the relevant master equation. When the two fields are in exact resonance with their respective transitions, expressions for the fluorescent spectra show a narrowing of the central peak for some specific values of the parameters of the squeezed vacuum and the phases between the driving fields and the squeezed vacuum. We also present analytical expressions for second-order intensity correlations. The inhibition of fluorescence in a squeezed vacuum is reflected in the quantum-jump-like behavior shown by these correlations.
A system of N identical superimposed two-level atoms (the Dicke model) interacting with one another and driven by a fluctuating laser field of finite phase and amplitude bandwidths is considered. An exact master equation for the phase-averaged reduced atomic density operator is derived using the theory of multiplicative stochastic processes. It is shown that in the absence of amplitude fluctuations, this equation admits an exact steady-state solution. The exact solution is further used to obtain and analyse the behaviour of the phase-averaged atomic observables and atomic correlation functions in the steady state. The principal results of our analysis is that the phase fluctuations tend to smooth the discontinuities in the observables and the correlation functions found in the non-fluctuating case. Further, including the amplitude fluctuations as well we derive in the high-field limit a Markovian master equation for the density operator averaged over the ensembles of both phase and amplitude fluctuations. The quantum regression theorem is used to derive and discuss exact analytical expressions for the fluorescent spectrum and the second-order intensity correlation function for a system of two interacting atoms.
A systematic method is presented for averaging the integral equations of motion for the atomic density matrix operator and its quantum correlation functions over the fluctuations of Markovian exciting fields with arbitrary bandwidth. The theory takes into account the statistics of the field to all orders. The method is applied to the investigation of resonance fluorescence in the presence of three different Markovian fields: (i) a phase-diffusion field, (ii) a chaotic field, and (iii) a Gaussian-amplitude field. It is shown that in the case of a resonant, intense phase-diffusion field a center line dip develops in the spectrum of resonance fluorescence when the Rabi frequency is approximately equal to the bandwidth of the field. In the case of amplitude fluctuations the sidebands of the on-resonance spectrum tend to reproduce the probability distribution for the amplitude of the exciting field.
A method of calculation of multiple-time correlation functions of the resonance fluorescence light from a two-level atom driven by a realistic laser field with phase and amplitude fluctuations is developed. Both kinds of fluctuations are assumed to be Gaussian. The phase fluctuations are treated in the phase-diffusion model. The averaging over the amplitude fluctuations can be performed in a closed way when the relative mean-square amplitude fluctuation is small compared with the ratio of the amplitude correlation decay rate to the characteristic atomic relaxation rate. There is no restriction to Markovian amplitude fluctuations. Arbitrary values for the mean Rabi frequency are allowed. Results are presented for the intensity, the intensity correlation function, and the spectrum of the fluorescent light. It is shown that even in the case when the relative strength of the amplitude fluctuations is small, significant effects can occur due to the finite correlation length of the fluctuations. The results for fast amplitude correlation decay correspond to the situation without amplitude fluctuations. When the correlation time of the amplitude fluctuations becomes comparable with the atomic relaxation times, the Rabi oscillations of the intensity and the intensity correlation function are nearly washed out, and non-Lorentzian line shapes for the side peaks in the spectrum are observed. It is found that the ratio of the heights of the central peak to the side peak increases with increasing correlation time.
The authors apply the recently developed theory of multiplicative stochastic correlation functions with Markovian random jumps to the problem of resonance fluorescence from a two-level atom in a strong laser field. The finite bandwidth of a single-mode laser or the appearance of distinct lines in a multimode laser is considered to be brought about by a random mode-switching process. The two-time dipole correlation functions, which determine the spectral distribution of the fluorescence and the temporal correlations between the emitted photons are averaged exactly over the stochastics of the driving field. The authors' explicit expressions only involve single-time averages, which can be easily evaluated for a given probability distribution. These results generalise and modify earlier results. The authors obtain closed expressions, rather than implicit differential equations, which can handle the continuous case as well, and take into account the initial correlations, which always arise when the laser coherence time is finite. They illustrate the dependence on the stochastics of the laser model by comparing the multimode description with the phase-diffusion process and the Lorentz wave, which all give rise to the same laser profile, but to a different fluorescence spectrum.