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Reviews of Modern Physics

The semiclassical theory of laser cooling

Stig Stenholm

Published Jul 1, 1986• 617 citations
Publisher

Abstract

This paper reviews the basic theory of the mechanical action of light in resonant interaction with atoms. At present the main application is laser cooling, but the approach is applicable to a broader range of phenomena. It is based on an adiabatic elimination philosophy, which turns out to give the lowest-order quantum corrections to the behavior found when the photon momentum goes to zero. Hence it is called a semiclassical theory. In this manner a subjective but consistent approach can be presented; other treatments are incorporated or mentioned at the appropriate places. Both the classical and the quantum-mechanical approach are discussed. Those readers who wish to obtain only a heuristic overview of the phenomena can concentrate on Sec. III, which treats both the photon momentum effects and their connection with photon counting statistics. The detailed theoretical treatment utilizes Wigner functions and Fokker-Planck techniques. The ensuing theory is applied both to the cooling of free particles and trapped ones. The paper ends with an extensive bibliography, where the author lists most papers of interest for research into the mechanical manifestations of light. For completeness, many papers are included that are not explicitly mentioned in the text.

DOI
10.1103/revmodphys.58.699

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This paper reviews the basic theory of the mechanical action of light in resonant interaction with atoms. At present the main application is laser cooling, but the approach is applicable to a broader range of phenomena. It is based on an adiabatic elimination philosophy, which turns out to give the lowest-order quantum corrections to the behavior found when the photon momentum goes to zero. Hence it is called a semiclassical theory. In this manner a subjective but consistent approach can be presented; other treatments are incorporated or mentioned at the appropriate places. Both the classical and the quantum-mechanical approach are discussed. Those readers who wish to obtain only a heuristic overview of the phenomena can concentrate on Sec. III, which treats both the photon momentum effects and their connection with photon counting statistics. The detailed theoretical treatment utilizes Wigner functions and Fokker-Planck techniques. The ensuing theory is applied both to the cooling of free particles and trapped ones. The paper ends with an extensive bibliography, where the author lists most papers of interest for research into the mechanical manifestations of light. For completeness, many papers are included that are not explicitly mentioned in the text.
The quantum kinetic equation describing slow atomic motion in laser light is derived by an operational method which provides mathematical expressions with a transparent physical structure. The authors prove in a general way that the coefficients appearing in this equation, which is of a Fokker-Planck type, are simply related to the mean value and to the correlation functions of the Heisenberg radiative force of the semiclassical approach, where the atomic position is treated classically. They derive in particular a new theoretical expression for the damping force responsible for radiative cooling and they interpret it in terms of linear response theory. The authors also obtain a new crossed r-p derivative term, which does not appear in semiclassical treatments, but which they find to be very small in most situations. Finally, all the theoretical expressions derived are valid for any J g to J e transitions and are not restricted to two-level atoms.
Preface. List of symbols. 1. Introduction. 2. Basic properties and types of lasers. 3. Laser resonators. 4. The intensity of laser light. Rate equations. 5. The basic equations of the semiclassical laser theory. 6. Applications of semiclassical theory. 7. Ultrashort pulses. 8. Instability hierachies of laser light. Chaos, and routes to chaos. 9. Optical bistability. 10. Quantum theory of the laser I. A first approach via quantum mechanical Langevin equations. Coherence, noise and photon-statistics. 11. Quantum theory of the laser II. A second approach via the density matrix equation and quantum classical correspondence. 12 A theoretical treatment of the two-photon laser. 13. The laser - trailblazer of synergetics. References. Subject index.
Abstract The straightforward application of energy and linear momentum conservation to the absorption/emission of photons by atoms allows us to establish the essential features of laser cooling of two level atoms at low laser intensities. The lowest attainable average kinetic energy of the atoms depends on the ratio between the natural linewidth and the recoil energy and tends to E R as tends to zero (in one dimension). This treatment, like the quantum mechanical ones, is valid for any value of the ratio and contains the semiclassical theory of laser cooling as the limiting case in which .
We consider the mechanical forces exerted on atoms by light as a tool to make the atom more concrete as a particle. It can be pushed, trapped and observed in its own scattered light. Recent theoretical and experimental progress in the field of cooling and trapping of atoms demonstrates their palpable reality. The theory of the mechanical manifestations of light is reviewed, and its application to laser cooling is discussed. Traps for atoms are considered. The feasibility of pure light traps is discussed, and the use of other types of traps in laser applications is reviewed. We present briefly the main experiments proving the possibility of laser cooling and trapping. A brief discussion of applications and future experimental possibilities is given.
We present a theoretical analysis of a new one-dimensional laser-cooling scheme that was recently demonstrated on a beam of metastable 4He atoms. Both internal and translational degrees of freedom are treated quantum mechanically. Unlike semiclassical approaches, such a treatment can be applied to situations in which the atomic coherence length is of the same order of or larger than the laser wavelength, which is the case for atoms cooled below the one-photon recoil energy. We introduce families of states that are closed with respect to absorption and stimulated emission, and we establish the generalized optical Bloch equations that are satisfied by the corresponding matrix elements. The existence of velocity-selective trapping states that are linear combinations of states with different internal and translational quantum numbers is demonstrated, and the mechanism of accumulation of atoms in these trapping states by fluorescence cycles is analyzed. From a numerical solution of the generalized optical Bloch equations, we study in detail how the final atomic-momentum distribution depends on the various physical parameters: interaction time, width of the initial distribution, laser detuning, laser power, and imbalance between the two counterpropagating waves. We show that the final temperature decreases when the interaction time increases, so that there is no fundamental limit to the lowest temperature that can be achieved by such a method. Finally, possible extensions of this method to two-dimensional cooling are presented.
When an atom or a molecule interacts with a light beam, the light emitted or absorbed carries valuable information about the atomic or molecular structure. This phenomenon underlies the whole field of spectroscopy. But the interaction of a photon with an atom can be used to manipulate the atom as well as to probe its structure. For example, in an approach called optical pumping, invented by Alfred Kastler, one can use the resonant exchange of angular momentum between atoms and polarized photons to align or orient the spins of atoms or to put them in nonequilibrium situations. In his original 1950 paper Kastler also proposed using optical pumping to cool and to heat the internal degrees of freedom, calling the phenomena the “effet luminofrigorique” and the “effet luminocalorique.” Another famous example of the use of photon-atom interaction to control atoms is laser cooling. This technique relies on resonant exchange of linear momentum between photons and atoms to control their external degrees of freedom and thus to reduce their kinetic energy. Laser cooling was suggested independently by Theodor Hänsch and Arthur Schawlow for neutral atoms and by David Wineland and Hans Dehmelt for trapped ions. In an article written three years ago for PHYSICS TODAY (June 1987, page 34), Wineland and Wayne Itano presented the principle of laser cooling and the potential applications of cold atoms to fields of physics such as ultrahigh resolution spectroscopy, atomic clocks, collisions, surface physics and collective quantum effects. At that time laser cooling had brought temperatures down to a few hundred microkelvin, but unexpected improvements during the last three years have dramatically lowered those temperatures to only a few microkelvin. We now feel we understand the new physical mechanisms responsible for these very low temperatures.