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Physical Review A

Atom microscopy via two-photon spontaneous emission spectroscopy

Sajid Qamar, Jörg Evers, Muhammad Suhail Zubairy

Published Apr 15, 2009• 34 citations
Publisher

Abstract

We study subwavelength position measurement via spontaneous emission spectroscopy with two photons. Our model systems are a single $\ensuremath{\Lambda}$-type three-level atom, in which a dual interaction generates two independent photons, and an $M$-type five-level atom, which emits two photons in a double-Raman process. The difference is that the $M$-type system emits correlated pairs of photons, while the photon pairs from the $\ensuremath{\Lambda}$ system are uncorrelated. In order to evaluate the performance of the position measurement, we introduce an analysis scheme motivated by a possible experimental measurement procedure. We find characteristic differences in the spontaneous emission spectra of the two systems arising from the photon correlation in the $M$-type system. But interestingly, the effect of this photon pair correlation on the conditional position probability distribution does not lead to an increase in the position information of the single atom. Nevertheless, both schemes allow for an efficient measurement of the particle position with unambiguous position determination over a wide range of parameters.

DOI
10.1103/physreva.79.043814

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We study subwavelength position measurement via spontaneous emission spectroscopy with two photons. Our model systems are a single \ensuremathΛ\ensuremath{\Lambda}\ensuremathΛ-type three-level atom, in which a dual interaction generates two independent photons, and an MMM-type five-level atom, which emits two photons in a double-Raman process. The difference is that the MMM-type system emits correlated pairs of photons, while the photon pairs from the \ensuremathΛ\ensuremath{\Lambda}\ensuremathΛ system are uncorrelated. In order to evaluate the performance of the position measurement, we introduce an analysis scheme motivated by a possible experimental measurement procedure. We find characteristic differences in the spontaneous emission spectra of the two systems arising from the photon correlation in the MMM-type system. But interestingly, the effect of this photon pair correlation on the conditional position probability distribution does not lead to an increase in the position information of the single atom. Nevertheless, both schemes allow for an efficient measurement of the particle position with unambiguous position determination over a wide range of parameters.
A scheme for two-dimensional (2D) subwavelength atom localization is proposed, in which the atom is in a four-level tripod configuration and driven by two orthogonal standing-wave lasers. Because of the spatial dependence of atom-field interaction, the spontaneously emitted photon carries information about the position of the atom in standing-wave fields. We exploit this fact to 2D atom localization conditioned on the measurement of spontaneously emitted photon at a particular frequency, and obtain a high precision and resolution in the position probability distribution. Moreover, an improvement by a factor of 2 in the detecting probability of an atom can be achieved by initially preparing the atom in the coherent population trapping state. Qualitatively, the high-precision, high-resolution atom localization can be attributed to the quantum interference effect between competitive multiple spontaneous decay channels.
Entanglement of the atom and field leads towards the measurement of the state of the atom or field depending on the kind of measurement made. Taking advantage of this fact, we propose spectroscopic methods for the single atom localization within the subwavelength domain of the optical standing wave field. \n \nWhen a two-level atom interacts with some intense radiation field the spectrum of the scattered light signal exhibits a three-peak Mollow spectrum. We propose a scheme of atom localization based on the resonance fluorescence from a two-level atom interacting with a standing wave field. The Rabi frequency is considered to be position dependent and therefore, the spontaneously emitted photon carries the information about the center-of-mass motion of the atom. This leads to the localization of the single atom by measuring the frequency of the spontaneously emitted photon even during the passage of the atom through the standing wave field. We predict a spatial resolution in position information of up to λ/60 where λ is the optical wavelength. \n \nDetuning of the coherent field with the atomic transition plays an important role in the characterization of the peaks present in the Autler- Townes spectrum of a three-level atom. Strong line narrowing is observed in one of the peaks of the Autler- Townes doublet depending on the choice of the detuning. We investigate how this detuning effects the position information of the atom inside the standing wave field in upper-level and lower-level coupling schemes of Autler- Townes microscopy. We show an enhancement in precision position measurement by factor of at least 4 in upper-level coupling scheme due to the quantum interference phenomenon. This enhancement is not observed in lower-level coupling scheme where the quantum interference is not taking place. \n \nWe also consider a system where a three-level atom is interacting with a monochromatic radiation field in such a way that the decay takes place from upper level to the intermediate level with a rate T and from intermediate level to lower level at a rate γ. This type of system exhibits a non stationary scattered light signal. We report the results of the spontaneous emission spectrum for non stationary scattered light signal by using the definition of time-dependent physical spectrum. This is a rare example of problems where time-dependent physical spectrum can be calculated exactly. We study the characteristics of the spontaneous spectrum for a resonant and off-resonant case and show that this physical spectrum recovers the results of earlier work quite successfully. We also show that the decay rate r disturbs the atomic coherence and finally eliminates the dark line from the center of the spontaneous spectrum. Here we only consider upper-level coupling case for the time-dependent spontaneous spectrum because in lower-level coupling case the system automatically evolved a pumping mechanism due to the coupling of ground level to the upper level via radiation field. Thus a steady-state limit exists in lower-level coupling scheme. \n \nWe investigate the phenomenon of atom localization by using the non stationary Autler-Townes microscopy. The decay rate T reduces the precision in position measurement which is consistent with the results of the non stationary spontaneous emission spectrum. This is due to the fact that for the upper-level coupling case, the standing wave field is coupled to atomic transition and it induces a coherence in the upper-level atomic transition but the spontaneous decay from the upper level to the intermediate level disturbs this coherence. When the effect of the spontaneous decay dominates the coherence effect the quantum interference phenomenon vanishes and thus the precision in localization reduces.
A scheme is proposed for two-dimensional atom localization in the subwavelength domain via controlled spontaneous emission. We consider a five-level M-type atomic system interacting with two orthogonal standing-wave laser fields and the vacuum of the radiation field. The interaction of the atom with space-dependent standing-wave fields can provide information about the position of the atom passing through, thus leading to atom localization. It is found that the localization is significantly improved due to the interference effect between the spontaneous decay channels and the dynamically induced quantum interference generated by the two standing-wave fields. By properly varying the system parameters, we can achieve high-precision and high-resolution atom localization.
We study the collective spontaneous emission of three identical two-level atoms initially prepared in the excited states by measuring Glauber's third-order photon correlation function. Assuming two atoms at subwavelength distance from each other such that they are subject to the dipole-dipole interaction while the third one is located several wavelengths away, we observe super- and subradiant decay alike, depending on the direction of observation. Unlike the case where no remote atom is introduced or no conditional measurements are performed, the spontaneous emission behavior of the conditioned three-atom system is strongly modified, i.e., differing from the single-atom and the canonical two-atom configuration. The conditional measurements associated with the three-photon correlation function in combination with the dipole-dipole interaction between the adjacent atoms lead to quantum interference among the different decay channels allowing one to engineer the spontaneous emission in space and time.
We propose a scheme for two-dimensional (2D) atom localization based on the controlled spontaneous emission, in which the atom interacts with two orthogonal standing-wave fields. Due to the spatially dependent atom-field interaction, the position probability distribution of the atom can be directly determined by measuring the resulting spontaneously emission spectrum. The phase sensitive property of the atomic system leads to quenching of the spontaneous emission in some regions of the standing-waves, which significantly reduces the uncertainty in the position measurement of the atom. We find that the frequency measurement of the emitted light localizes the atom in half-wavelength domain. Especially the probability of finding the atom at a particular position can reach 100% when a photon with certain frequency is detected. By increasing the Rabi frequencies of the driving fields, such 2D sub-half-wavelength atom localization can acquire high spatial resolution.
A scheme for realizing two-dimensional (2D) atom localization is proposed based on controllable spontaneous emission in a coherently driven cycle-configuration atomic system. As the spatial-position-dependent atom-field interaction, the frequency of the spontaneously emitted photon carries the information about the position of the atom. Therefore, by detecting the emitted photon one could obtain the position information available, and then we demonstrate high-precision and high-resolution 2D atom localization induced by the quantum interference between the multiple spontaneous decay channels. Moreover, we can achieve 100% probability of finding the atom at an expected position by choosing appropriate system parameters under certain conditions.