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Physical Review A

Quasiclassical theory of laser-induced atomic-beam dispersion

E. Arimondo, Arturo Bambini, Stig Stenholm

Published Aug 1, 1981• 81 citations
Publisher

Abstract

We present a theoretical model for the interaction of a beam of two-level atoms with a resonant laser beam. It is shown that the radiation force, while averaging to zero at resonance, produces a transverse spread of the atomic velocities. If radiative damping is ignored, this spread increases linearly with time and finally saturates towards a steady value. Although the spread has a quantum-mechanical origin, we show that it is possible, in the limit $\ensuremath{\hbar}k\ensuremath{\rightarrow}0$, to describe the phenomenon in terms of differential equations of motion for the atomic translational variables, as in the classical case. In this model it is also possible to describe the effects of radiative damping, as well as other additional effects, which may occur in a real experiment. Finally a comparison of our results with experimental data, recently obtained on an Na atomic beam, has been made. Although an order-of-magnitude fit of the experimental data could be obtained, the weights of the different causes, reducing the spread, were found to be ambiguous and have been left partly open.

DOI
10.1103/physreva.24.898

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Richard J. Cook

A general theory of the motion of a two-level atom in a resonant or near-resonant electromagnetic wave of arbitrary amplitude and phase, including effects of radiative relaxation due to interaction with the quantized vacuum field, is developed from first principles. Particular emphasis is placed on the effects of quantum-mechanical fluctuations of the radiation force and on the associated diffusion of atomic momentum due to spontaneous and induced absorption and emission processes. Analytic results and numerical examples are presented for (1) the lower bound on the temperature achievable by radiation cooling in a standing wave tuned below resonance, (2) the heating rate in a strong resonant standing wave, (3) the maximum confinement time for an atom in a Gaussian radiation trap, (4) the deflection and spreading of an atomic beam transversely illuminated by a strong resonant running wave, and (5) the transverse cooling of an atomic beam by a strong running wave tuned below resonance.

Physical Review A•Sep 1, 1980•131 citations
We present a theoretical model for the interaction of a beam of two-level atoms with a resonant laser beam. It is shown that the radiation force, while averaging to zero at resonance, produces a transverse spread of the atomic velocities. If radiative damping is ignored, this spread increases linearly with time and finally saturates towards a steady value. Although the spread has a quantum-mechanical origin, we show that it is possible, in the limit \ensuremathℏk\ensuremath→0\ensuremath{\hbar}k\ensuremath{\rightarrow}0\ensuremathℏk\ensuremath→0, to describe the phenomenon in terms of differential equations of motion for the atomic translational variables, as in the classical case. In this model it is also possible to describe the effects of radiative damping, as well as other additional effects, which may occur in a real experiment. Finally a comparison of our results with experimental data, recently obtained on an Na atomic beam, has been made. Although an order-of-magnitude fit of the experimental data could be obtained, the weights of the different causes, reducing the spread, were found to be ambiguous and have been left partly open.
The effect of field fluctuations on the motion of a two-level atom in resonant laser radiation is investigated theoretically. The internal motion of the atom is treated quantum mechanically (optical Bloch equations); the translational motion, which is coupled to the internal motion, is treated classically (Ehrenfest's theorem); and the fluctuating radiation is treated as a classical electromagnetic wave with stochastic phase (phase-diffusion model). An expression for the radiation force and equations of motion for the ensemble-averaged Bloch vector are derived and used to calculate (i) the radiation force in a plane running wave, (ii) the steady-state radiation force in a general standing wave, and (iii) the dissipative force in a plane standing wave in the limit of strong phase fluctuations. In case (iii) it is found that the atomic velocity is damped when the radiation is tuned above resonance, which is opposite to the case of a weak coherent standing wave, in which damping occurs for radiation tuned below resonance. It is shown that fluctuations have a substantial effect on the radiation force only when the spectral width of the radiation approaches or exceeds the spontaneous emission rate.
Abstract This present paper is an attempt to describe the operation of a laser by a method patterned closely after the classical theory of dispersion. There, the electromagnetic field is treated as a classical system interacting with a collection of classical harmonic oscillators which are at rest. In the present case the radiation field is still treated classically, but, in accordance with the correspondence principle, the oscillators are now virtual oscillators associated with the up-and-down transitions in effective two-state atoms which are described quantum mechanically. The atoms carrying these virtual oscillators are not at rest but move with different velocities. We show how the Lorentz averaging can be performed for such systems, and derive a closed set of equations linking the average electric field E, with the average polarization density P„ and the average population inversion density Mp associated with atoms moving with the velocity v. Next, we investigate the conditions for the existence of a steady state if pumping is present, and if the electric field is represented by a standing wave, or a travelling wave of a single frequency (single-mode case). It turns out that, notwithstanding the nonlinear nature of the equations, the steady-state conditions give a simple complex dispersion relation; moreover, the real and imaginary part of this dispersion relation are equivalent to the usual heuristic expressions which specify the operating frequency in terms of the index of refraction and cavity length, and which balance the gain against the losses. The single-mode case is analysed in detail without any smallness assumptions for the resultant intensity. The small-intensity case gives the usual results exhibiting the tuning dip. For high intensities the relative depth of the dip tends to zero. At the end of the paper we discuss proposed extensions and additional applications.
The theory of the resonance radiation force is studied as it applies to the slowing of a two-level atom using a swept frequency laser. The theory is developed in detail for this case. A single partial differential equation called the Fokker-Planck equation is found to describe the atomic motion for many cases. This equation is solved numerically for a one dimensional geometry. Results from this numerical solution are found to be within 10% of experimental results. Analysis of this problem in one dimension leads to the prediction that for fixed amounts of frequency sweeping, a faster scan rate will yield smaller full width at half maximum (FWHM) spread in the velocity distribution for the atomic beam. This program also predicts that the atoms can be slowed arbitrarily close to 0 m/sec using this technique. The program used for this analysis is included. Keywords: Resonance radiation force; Slowing an atomic beam; Laser cooling of atoms; Fokker Planck equation; Thesis.
We study the deflection of an atomic system with a resonant multilevel energy structure in classical and quantized wave light fields. We obtain that the shape of the momentum distribution is very sensitive to the energy level structure, whereas its moments are not. Comparison with a two-level case is made. PACS: 32.80, 33.80, 42.50 During the last two decades a remarkable development in mechanically manipulating atomary particles with resonant laser light has taken place (for a review, see for example [1, 2] and references therein). In addition to trapping and cooling of particles, the deflection of particles by a laser beam offers interesting possibilities, for example, to construct atomic interferometers or beam splitters [2-4]. This problem has been studied extensively both theoretically [2, 5, 8] and experimentally [9-12]. The fact that the momentum distribution caused by the scattering is connected to the quantum statistical properties of the scattered light has been known for some time [13]. Recently, one has also realized that the quantum statistics of the light causing the scattering can be important [14]. At low photon numbers, for example, the initial field state strongly influences the resulting momentum distribution. A related effect is that a standing wave and two counterpropagating traveling plane waves of equal emplitudes cause a different diffraction pattern when fields are treated quantum mechanically [15]. Most previous work on the deflection of particles by light fields used two-level atoms. In this paper we study how resonant multilevel systems scatter when they traverse a plane wave. In practical applications, molecules or highly excited atoms have similar energy structures as the models we use in this work. In most cases, we assume that the Raman-Nath regime is valid, i.e., the kinetic energy of the particle can be neglected. However, the field coupling is assumed to be sufficiently strong to make multiple scattering events possible. Our results show that the final momentum distribution of a multi-level system can strongly deviate from that of a two-level atom. It is of interest that the momentum distributions for resonant ladder systems are in general superpositions of few or several distributions similar to that of a two-level system. We also study the expectation values related to the momentum distribution and show that the spread in momentum is remarkably independent of the system considered. The absorption and reabsorption of photons during the scattering process causes the photon distribution to be smoothed out, and for long times a steady state is reached. The cases we studied did not show a creation of sub-Poissonian light. Our model and assumptions are described and discussed in Sect. 1. Some of the general properties of the momentum distribution are discussed in Sect. 2. In Sect. 3 we derive the generating function of the moments of momentum change in Raman-Nath regime. The main part of the paper is contained in Sects. 4 and 5, in which the momentum distribution itself is discussed for several model systems. In Sect. 4 a semiclassical field is assumed and in Sect. 5 a quantum field is used. The effects of the scattering on the field photon statistics are studied in Sect. 6. The final discussion of the results is given in Sect. 7.
The quantum kinetic equation describing slow atomic motion in laser light is derived by an operational method which provides mathematical expressions with a transparent physical structure. The authors prove in a general way that the coefficients appearing in this equation, which is of a Fokker-Planck type, are simply related to the mean value and to the correlation functions of the Heisenberg radiative force of the semiclassical approach, where the atomic position is treated classically. They derive in particular a new theoretical expression for the damping force responsible for radiative cooling and they interpret it in terms of linear response theory. The authors also obtain a new crossed r-p derivative term, which does not appear in semiclassical treatments, but which they find to be very small in most situations. Finally, all the theoretical expressions derived are valid for any J g to J e transitions and are not restricted to two-level atoms.
A general theory of the motion of a two-level atom in a resonant or near-resonant electromagnetic wave of arbitrary amplitude and phase, including effects of radiative relaxation due to interaction with the quantized vacuum field, is developed from first principles. Particular emphasis is placed on the effects of quantum-mechanical fluctuations of the radiation force and on the associated diffusion of atomic momentum due to spontaneous and induced absorption and emission processes. Analytic results and numerical examples are presented for (1) the lower bound on the temperature achievable by radiation cooling in a standing wave tuned below resonance, (2) the heating rate in a strong resonant standing wave, (3) the maximum confinement time for an atom in a Gaussian radiation trap, (4) the deflection and spreading of an atomic beam transversely illuminated by a strong resonant running wave, and (5) the transverse cooling of an atomic beam by a strong running wave tuned below resonance.