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Low Temperature Physics

Fine structure of critical opalescence spectra

M. Ya. Sushko

Published Sep 1, 2007• 1 citation
Publisher

Abstract

The effect of the 1.5-scattering mechanism on the time and temperature behavior of the electric field autocorrelation function for the light wave scattered from fluids has been studied for the case where the order-parameter fluctuations obey the diffusion-like kinetics with spatially-dependent kinetic coefficient. The leading contributions to the relevant static correlation functions of the order-parameter fluctuations were obtained by using the Ginzburg-Landau model with a cubic term, and then evaluated with the use of the Gaussian uncoupling for many-point correlation functions and the Ornstein-Zernicke form for the pair correlation function. It is shown that the presence of the 1.5-scattering effects in the overall scattering pattern may be detected in the form of a small but noticeable deviation from exponential decay of the total electric field autocorrelation function registered experimentally near the critical point. Obtained with the standard methods of analysis, the effective half-width of the corresponding spectrum can reveal a stronger temperature dependence and a multiplicative renormalization as compared to the half-width of the spectrum of the pair correlator.

DOI
10.1063/1.2784150

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