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Modern Physics Letters B

THE MECHANICAL ACTION OF LASER LIGHT ON RYDBERG ATOMS

G. Alber, Walter T. Strunz, O. Zobay

Published Oct 20, 1994• 2 citations
Publisher

Abstract

The momentum exchange between a standing wave laser field and an atomic center-of-mass is dominated by the internal dynamics of an atomic electron in the exciting laser field. Rydberg atoms are one of the simplest physical systems where the dependence of this radiative force on the electronic dynamics can be investigated in detail. The characteristics of the momentum transfer between an atomic center-of-mass and a standing wave laser field strongly depend on whether the “particle” or the “wave” aspect of the electronic dynamics prevail. In this review recent theoretical advances in the description of the mechanical action of laser light on Rydberg atoms are discussed. These advances have become possible by the application of semiclassical path integral techniques with respect to the electronic dynamics which clearly exhibit the “particle” and “wave” aspects of this momentum transfer.

DOI
10.1142/s0217984994001436

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The momentum exchange between a standing wave laser field and an atomic center-of-mass is dominated by the internal dynamics of an atomic electron in the exciting laser field. Rydberg atoms are one of the simplest physical systems where the dependence of this radiative force on the electronic dynamics can be investigated in detail. The characteristics of the momentum transfer between an atomic center-of-mass and a standing wave laser field strongly depend on whether the “particle” or the “wave” aspect of the electronic dynamics prevail. In this review recent theoretical advances in the description of the mechanical action of laser light on Rydberg atoms are discussed. These advances have become possible by the application of semiclassical path integral techniques with respect to the electronic dynamics which clearly exhibit the “particle” and “wave” aspects of this momentum transfer.
It is shown that semiclassical path representations provide a well-suited framework for the description of the diffraction of Rydberg atoms by laser light. They allow one to relate the momentum exchange between the atomic center-of-mass motion and the laser field directly to elementary laser-assisted collisions between the excited Rydberg electron and the ionic core. Thus besides a convenient calculational tool they provide also direct physical insight into the underlying internal dynamics of the Rydberg atoms.
The influence of laser-induced two-electron excitation processes on the deflection of atoms by a standing-wave laser field is investigated. In particular, isolated-core excitation processes are studied in which, after preparing one valence electron as an electronic Rydberg wave packet, the core electron is driven resonantly by the standing wave. The dynamics of the two electrons are entangled through laser-induced electron correlation effects. A theoretical approach is developed that clearly exhibits the intricate interplay between these correlation effects and the atomic center-of-mass motion that originates from the stimulated light force. Various examples are analyzed that show the manifestations of this interplay in the diffraction pattern of a deflected atom.
In quantum optical problems involving the interaction of atoms with laser fields, the atoms are usually considered being stationary during the interaction. Since every photon has a momentum, the atomic momentum (motion) can be changed in the process of absorption and emission of photons. This may force a stationary atom to move or to change momentum of an already moving atom. Therefore, the dynamical behaviour of atoms can be varied by the interaction with a radiation field. For a weak driving field, the influence of this field on the atomic motion can be neglected. However, the intensities of laser fields are generally very strong, and then the motion of the atoms can be considerably changed by the laser field. Here, we discuss this aspect, especially the effect of a driving field on the motion of atoms and the atomic momentum distribution. In particular, we will consider diffraction of atoms by a standing-wave laser field due to an exchange of momentum with the photons of the wave, and radiation force on atoms driven by a running-or standing-wave laser field.
The formation of atom-optical gratings induced by multiphoton excitation of Rydberg states is discussed for fast atoms. With the help of semiclassical path-integral methods the correlation between the dynamics of a laser-excited Rydberg electron and the momentum transferred to the atomic center of mass in a spatially modulated laser field is exhibited quantitatively. These types of laser excitation processes might offer new perspectives for the realization of atomic multiple beam splitters and for atom-lithographic applications.
In the preceding chapters, we discussed the manipulation and observation of atomic variables associated with the internal degrees of freedom. A complete separation between internal and external degrees of freedom, like position and momentum, is not always possible, however. It therefore appears appropriate to include a discussion of the mechanical effects of light, which have received increasing attention in recent years. The transfer of momentum between photons and atoms, first observed more than sixty years ago, had to wait for the wide availability of lasers to become a useful experimental tool. In particular the cooling of atoms and atomic ions to very low temperatures has found numerous applications. Light-induced forces That light exerts mechanical forces on massive particles like atoms may appear surprising. To motivate the existence of such an effect two different approaches are possible. The first approach considers the light as a collection of photons that carry, apart from energy and angular momentum, linear momentum as well. Photons interacting with atoms can therefore change the momentum of the atoms. The second approach considers light as a wave, i.e., an inhomogeneous electromagnetic field interacting with the atomic dipole moment. Both approaches provide a possible description for the numerous phenomena that can occur in this context, but in many situations, one of them turns out to be more intuitive or more useful for calculations than the other.
Deflection of an atom due to momentum transfer from a strong resonant standing electromagnetic wave is investigated theoretically in the limit of short atom-field interaction time. The translational and internal motions of the atom are treated quantum mechanically, while the field is treated classically. It is shown that momentum transfer from a standing wave to an atom proceeds at the induced or Rabi rate, rather than the spontaneous rate characteristic of radiation pressure. In a typical case, atomic deflections of order 1\ifmmode^\circ\else\textdegree\fi{} are achieved with 106{10}^{6}106 W/cm2{\mathrm{cm}}^{2}cm2 field intensity in a time less than the natural lifetime of the excited atom.