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physica status solidi (b)

Kinetics of the Dephasing and the Condensation of Excitons

O.M. Schmitt, P. Gärtner, L. B�nyai, D. B. Tran Thoai, H. Haug

Published Sep 1, 2000• 3 citations
Publisher

Abstract

The dephasing and condensation kinetics of bosonic excitons after coherent pulse excitation is studied in the vicinity of a Bose-Einstein condensation (BEC). For a system of excitons interacting with acoustic phonons various excitation conditions are investigated. Significant qualitative changes of the polarization dephasing in the vicinity of the BEC are discussed. Furthermore the kinetics of excitons, interacting via a two particle interaction, is studied. Both the bosonic mean-field terms and the scattering terms are calculated on a microscopic level. As in the phonon-model the dephasing rate of the exciton–exciton scattering diminishes considerably in the vicinity of the BEC. All results are suited as experimentally observable signatures of an excitonic BEC.

DOI
10.1002/1521-3951(200009)221:1<221::aid-pssb221>3.0.co;2-h

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The dephasing and condensation kinetics of bosonic excitons after coherent pulse excitation is studied in the vicinity of a Bose-Einstein condensation (BEC). For a system of excitons interacting with acoustic phonons various excitation conditions are investigated. Significant qualitative changes of the polarization dephasing in the vicinity of the BEC are discussed. Furthermore the kinetics of excitons, interacting via a two particle interaction, is studied. Both the bosonic mean-field terms and the scattering terms are calculated on a microscopic level. As in the phonon-model the dephasing rate of the exciton–exciton scattering diminishes considerably in the vicinity of the BEC. All results are suited as experimentally observable signatures of an excitonic BEC.
Photo-excited excitons, i.e. closely bound electron-hole pairs, are in the low-density regime approximately bosons. For sufficiently low temperatures and sufficiently high densities of the exciton gas, a nonequilibrium phase transition in the form of a Bose-Einstein condensation (BEC) can be expected. Various levels of the description of the kinetics of relaxation and condensation due to the coupling of the excitons to a cold reservoir of acoustic phonons are discussed. For noninteracting excitons a rate equation approach with the exciton Boltzmann equation can be used. For interacting excitons the nonmarkovian quantum kinetics is required for the description of the BEC in order to incorporate the changes of the energy spectrum during the condensation self-consistently. Finally colored Langevin fluctuations can be used to calculate the phase diffusion of the condensate.
The time-dependent correlation function of the order parameter of Bose-Einstein condensation is calculated for a dilute interacting exciton gas cooled by a cold phonon bath. This calculation is achieved by combining two theoretical concepts: (i) a non-Markovian quantum kinetics, which is necessary in order to include the changing single-particle spectrum during the condensation self-consistently, and (ii) the stochastic non-Markovian Langevin fluctuations which are connected with the dissipative scattering integrals. A linearization around the mean quantum kinetics is used in order to determine the order parameter's fluctuations around its mean value. Similarly as in the laser theory the linewidth or the coherence time of the coherent order parameter amplitude is determined. The results show a clear reduction of the linewidth of the coherent exciton amplitude as the system cools down in time through the threshold of the Bose-Einstein condensation. The observation of this line narrowing by nonlinear optical spectroscopy would give a direct indication of the temporal build-up of an exciton condensate in a semiconductor.
Bose-Einstein condensation (BEC) is a thermodynamic phase transition of an interacting Bose gas. Its key signatures are remarkable quantum effects like superfluidity and a phonon-like Bogoliubov excitation spectrum, which have been verified for atomic BECs. In the solid state, BEC of exciton-polaritons has been reported. Polaritons are strongly coupled light-matter quasiparticles in semiconductor microcavities and composite bosons. However, they are subject to dephasing and decay and need external pumping to reach a steady state. Accordingly the polariton BEC is a nonequilibrium process of a degenerate polariton gas in self-equilibrium, but out of equilibrium with the baths it is coupled to and therefore deviates from the thermodynamic phase transition seen in atomic BECs. Here we show that key signatures of BEC can even be observed without fulfilling the self-equilibrium condition in a highly photonic quantum degenerate nonequilibrium system.
We describe the kinetics of bosonic excitons in a potential trap by rate equations in the basis of the single-particle eigenfunctions. We consider the interaction of the excitons with a thermal bath of acoustic phonons. Starting with an initial spatially homogeneous exciton distribution in the continuum, we show both a subcritical and a supercritical scenario for a spherically symmetric model potential. In particular, we observe for the case of Cu2O{\mathrm{Cu}}_{2}\mathrm{O}Cu2​O the buildup of a Bose-Einstein condensate within a microsecond time scale. However, the condensation time depends strongly on the depth and width of the trapping potential and the initial exciton distribution.