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Physical Review A

Heisenberg’s equations of motion for dissipative tunneling

Mohsen Razavy

Published Jun 1, 1990• 12 citations
Publisher

Abstract

The quantum-mechanical problem of tunneling of a particle coupled to a heat bath that consists of a large number of harmonic oscillators is studied in this paper. Here the equation of motion for the particle which is a nonlinear integro-differential equation is found by eliminating the degrees of freedom of the oscillators. The nonlinear operator equation may be solved by noting that the position operator at the time t can be expanded as a power series in terms of the initial position and momentum with time-dependent c-number coefficients. These coefficients also satisfy nonlinear integro-differential equations. For the problem of dissipative tunneling of a particle in a double-well potential, the first few terms of expansion have been calculated numerically. The expansion parameter in this formulation is a small dimensionless parameter which is inversely proportional to the product of the width and the square root of the height of the barrier.

DOI
10.1103/physreva.41.6668

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The quantum-mechanical problem of tunneling of a particle coupled to a heat bath that consists of a large number of harmonic oscillators is studied in this paper. Here the equation of motion for the particle which is a nonlinear integro-differential equation is found by eliminating the degrees of freedom of the oscillators. The nonlinear operator equation may be solved by noting that the position operator at the time t can be expanded as a power series in terms of the initial position and momentum with time-dependent c-number coefficients. These coefficients also satisfy nonlinear integro-differential equations. For the problem of dissipative tunneling of a particle in a double-well potential, the first few terms of expansion have been calculated numerically. The expansion parameter in this formulation is a small dimensionless parameter which is inversely proportional to the product of the width and the square root of the height of the barrier.
A wave equation formulation of the problem of quantum tunneling in a dissipative medium is developed by considering a many-body system in which the central particle is subject to an arbitrary force law, and at the same time is coupled to a bath of noninteracting harmonic oscillators. For the motion of the central particle it is possible to obtain an effective Lagrangian and Hamiltonian by eliminating the degrees of freedom of the oscillators. However both of these operators are nonlocal, and it is difficult to derive a wave equation for this motion. As an alternative method one can write a many-body Schrödinger equation for the whole system, and then eliminate the wave functions of all of the oscillators. This result is a many-channel Schrödinger equation for the motion of the central particle. By truncating this set of coupled equations, one can solve the problem for different force laws. In particular, in this work, the cases of dissipative tunneling, hopping, and quantum coherence are studied in detail. It is also shown how this approach can be generalized to multidimensional dissipative systems.
The motion of a particle subject to an external force and coupled to a large number of harmonic oscillators is reducible to a nonlinear integro-differential equation for the position operator. This is achieved by eliminating the degrees of freedom corresponding to the motion of the oscillators. Upon this elimination the commutator of the position and the mechanical momentum of the particle becomes time dependent and a c number for a quadratic potential, but in general a q number for other fields of force. For a harmonically bound particle interacting with the heat bath the time evolution of the position and momentum operators are given in terms of the solutions of an integro-differential equation. Certain forms of the coupling of the motion of the particle to the heat bath allow for further reduction of these equations to quartic differential equations with constant coefficients. For these cases the time dependence of the position-momentum commutator, the energy of the particle as well as the heat bath are studied.
A method of integration of the Heisenberg equation of motion is proposed in which the time evolution of the basis set {Tm,{\mathit{T}}_{\mathit{m},}Tm,​n(t)} of the Weyl-ordered operators introduced by Bender and Dunne [Phys. Rev. D 40, 3504 (1989)] is obtained from the Taylor expansion and is expressible in terms of the initial {Tm,{\mathit{T}}_{\mathit{m},}Tm,​n(0)}'s. In the absence of damping forces, the constant values of the energy and the position-momentum commutation relation are used to check the accuracy of the integration. This method is applied to obtain the mean position and velocity of the particle as a function of time as well as the dwell time of the particle inside the barrier. In the example that is considered here, the potential is assumed to be the sum of a harmonic and a cubic term, and the calculation is done with and without dissipative coupling.
The canonical treatment of the quantum dynamics of systems with dissipation affected degrees of freedom proceeds within the sum over histories picture of quantum theory. This paper proposes to supplement that approach with a Schrodinger equation approach to the same physics. Starting from a Lagrangian that is of the same form as those obtained by path integration, one can arrive at a quantized Hamiltonian analogue using the standard rules applied to non-dissipative systems. The resulting Hamiltonian is non-diagonal in position representation, so that the corresponding Schrodinger equation is a nonlinear integro-differential equation reminiscent of the Hartree equation. In the case of the normal tunnel junction, with a quasiparticle heat bath, this equation has an exact solution.
Finite temperatures are incorporated into the calculation of the tunneling rate in the presence of linear dissipation. A theory of finite-temperature tunneling is introduced which is based on the density matrix which provides an approximate description of the metastable state. Semiclassical functional integral methods are used to calculate the density matrix and the Wentzel-Kramers-Brillouin approximation is used to derive the tunnel current from the density matrix. Dissipation appropriate to superconducting quantum-interference devices is introduced into the calculation by the use of the existing model of a heat bath consisting of a prescribed distribution of harmonic oscillators linearly coupled to the tunneling variable. The finite-temperature tunnel escape rate obtained is of the form \ensuremath{\Gamma}=A exp(-S/\ensuremath{\Elzxh}). S is determined from the solution of a nonlinear integro-differential equation. An existing numerical technique was modified to achieve this. The quantity A is approximately evaluated.
From a quantized many-body system a wave equation for the motion of a particle linearly coupled to a heat bath is derived. The effective Hamiltonian describing the motion of the single particle is explicitly time dependent, and for a quadratic potential, has a simple dependence on the initial position and momentum of the particle. For the case of dissipative harmonic motion, a time-dependent wave equation is derived and the ground-state wave function is determined. It is also shown that if the equations of motion for the many-body system is Galilean invariant, the reduced form of equation of motion for the single particle is not. However a generalized form of transformation for the position and momentum operators, to a coordinate system moving with constant velocity, is obtained, which reduces to the Galilean transformation when the coupling to the dissipative system is turned off.