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Journal of Physics A Mathematical and Theoretical

Non-adiabatic and adiabatic transitions at level crossing with decay: two- and three-level systems

M. B. Kenmoe, S. E. Mkam Tchouobiap, C. Kenfack-Sadem, A. B. Tchapda, Lukong Cornelius Fai

Published Feb 10, 2015• 12 citations
Publisher

Abstract

We investigate the Landau–Zener (LZ) like dynamics of decaying two- and three-level systems with decay rates Γ 1 and Γ 2 for levels with minimum and maximum spin projection. Non-adiabatic and adiabatic transition probabilities are calculated from diabatic and adiabatic bases for two- and three-level systems. We extend the familiar two-level model of atoms with decay from the excited state out of the system into the hierarchy of three-level models which can be solved analytically or computationally in a non-perturbative manner. Exact analytical solutions are obtained within the framework of an extended form of the proposed procedure which enables to take into account all possible initial moments rather than large negative time t 0 = − ∞ as in standard LZ problems. We elucidate the applications of our results from a unified theoretical basis that numerically analyzes the dynamics of a system as probed by experiments.

DOI
10.1088/1751-8113/48/9/095303

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We investigate the Landau–Zener (LZ) like dynamics of decaying two- and three-level systems with decay rates Γ 1 and Γ 2 for levels with minimum and maximum spin projection. Non-adiabatic and adiabatic transition probabilities are calculated from diabatic and adiabatic bases for two- and three-level systems. We extend the familiar two-level model of atoms with decay from the excited state out of the system into the hierarchy of three-level models which can be solved analytically or computationally in a non-perturbative manner. Exact analytical solutions are obtained within the framework of an extended form of the proposed procedure which enables to take into account all possible initial moments rather than large negative time t 0 = − ∞ as in standard LZ problems. We elucidate the applications of our results from a unified theoretical basis that numerically analyzes the dynamics of a system as probed by experiments.
We study the Landau–Zener problem for a decaying two-level system described by a non-Hermitian Hamiltonian, depending analytically on time. Use of a super-adiabatic basis allows us to calculate the survival probability P in the slow-sweep limit, without specifying the Hamiltonian explicitly. It is found that P consists of a 'dynamical' and a 'geometrical' factor. The former is determined by the complex adiabatic eigenvalues E ± ( t ), only, whereas the latter solely requires the knowledge of α ± ( t ), the ratio of the components of each of the adiabatic eigenstates. Both factors can be split into a universal one, depending only on the complex level crossing points, and a nonuniversal one, involving the full time dependence of E ± ( t ) and α ± ( t ). This general result is applied to the Akulin–Schleich model where the initial upper level is damped with damping constant γ. For analytic power-law sweeps we find that Stückelberg oscillations of P exist for γ smaller than a critical value γ c and disappear for γ > γ c . A physical interpretation of this behaviour will be presented by use of a damped harmonic oscillator.
Two aspects of the classic two-level Landau-Zener (LZ) problem are considered. First, we address the LZ problem when one or both levels decay, i.e., ${\ensuremath{\varepsilon}}_{j}(t)\ensuremath{\rightarrow}{\ensuremath{\varepsilon}}_{j}(t)\ensuremath{-}i{\ensuremath{\Gamma}}_{j}/2$. We find that if the system evolves from an initial time $\ensuremath{-}T$ to a final time +T+T+T such that $|{\ensuremath{\varepsilon}}_{1}(\ifmmode\pm\else\textpm\fi{}T)\ensuremath{-}{\ensuremath{\varepsilon}}_{2}(\ifmmode\pm\else\textpm\fi{}T)|$ is not too large, the LZ survival probability of a state $|j\ensuremath{\rangle}$ can increase with increasing decay rate of the other state $|i\ensuremath{\ne}j\ensuremath{\rangle}$. This surprising result occurs because the decay results in crossing of the two eigenvalues of the instantaneous non-Hermitian Hamiltonian. On the other hand, if $|{\ensuremath{\varepsilon}}_{1}(\ifmmode\pm\else\textpm\fi{}T)\ensuremath{-}{\ensuremath{\varepsilon}}_{2}(\ifmmode\pm\else\textpm\fi{}T)|\ensuremath{\rightarrow}\ensuremath{\infty}$ as $T\ensuremath{\rightarrow}\ensuremath{\infty}$, the probability is independent of the decay rate. These results are based on analytic solutions of the time-dependent Schr\"odinger equations for two cases: (a) the energy levels depend linearly on time, and (b) the energy levels are bounded and of the form ${\ensuremath{\varepsilon}}_{1,2}(t)=\ifmmode\pm\else\textpm\fi{}\ensuremath{\varepsilon}tanh(t/\mathcal{T})$. Second, we study LZ transitions affected by dephasing by formulating the Landau-Zener problem with noise in terms of a Schr\"odinger-Langevin stochastic coupled set of differential equations. The LZ survival probability then becomes a random variable whose probability distribution is shown to behave very differently for long and short dephasing times. We also discuss the combined effects of decay and dephasing on the LZ probability.
Abstract Three analytic solutions to the Schrödinger equation for the time-dependent Landau–Zener (LZ) Hamiltonian are presented. They correspond to specific finite-time driving paths in a bounded parameter space of a two-level system. Two of these paths go through the avoided crossing of levels, either with a constant speed or with variable speed that decreases in the region of reduced energy gap, the third path bypasses the crossing such that the energy gap remains constant. The solutions yield exact time dependencies of the excitation probability for the system evolving from the ground state of the initial Hamiltonian. The LZ formula emerges as an approximation valid within a certain interval of driving times for the constant-speed driving through the avoided crossing. For long driving times, all solutions converge to the prediction of the adiabatic perturbation theory. The excitation probability vanishes at some discrete time instants.
Using a comparison equation method rooted in the Landau-Zener model, we report results for the probability of transition and survival in two-state models for a crossing of levels having some width, to account for dissipation. The theory allows arbitrary forms for the state energies, their rate of decay, and coupling, subject only to the limitation inherent in the Landau-Zener class (coupling with infinite ``pulse area''). We show how the strong decay result of adiabatic elimination can be recovered, but with important restrictions as to its usability. We also confirm the validity of the well-known Dykhne formula for crossings of real energy levels, and use the new theory to extend the Dykhne result to a class of dissipative crossings we call pseudoreal. Finally, we examine the overall probability for transition at two successive crossings, as occurs in atomic collisions. Here, interference of the crossing states leads to oscillations in the transition probability with collision time. For slow collisions we find that even a modest level of dissipation heavily damps these oscillations, but at the same time enhances the average probability of transition.
We compute Landau-Zener probabilities for three-level systems with a linear sweep of the uncoupled energy levels of the $3\ifmmode\times\else\texttimes\fi{}3$ Hamiltonian matrix H(t)H(t)H(t). Two symmetry classes of Hamiltonians are studied: For $H(t)\ensuremath{\in}$ su(2) (expressible as a linear combination of the three spin-1 matrices), an analytic solution to the dynamical problem is obtained in terms of the parabolic cylinder DDD functions. For $H(t)\ensuremath{\in}$ su(3) (expressible as a linear combination of the eight Gell-Mann matrices), numerical solutions are calculated. In the adiabatic regime, full population transfer is obtained asymptotically at large times, but at intermediate times, all three levels are populated, and St\"uckelberg oscillations can manifest from the occurrence of two avoided crossings. For the open system, (wherein interaction with a reservoir occurs), we numerically solve a Markovian quantum master equation for the density matrix with Lindblad operators that models interaction with isotropic white Gaussian noise. We find that St\"uckelberg oscillations are suppressed and that the decoherence cannot be modeled in terms of a simple exponential.
We study the Landau-Zener (LZ) dynamics in a setup of two Rydberg atoms with time-dependent detuning, both linear and periodic, using both the exact numerical calculations as well as the method of adiabatic impulse approximation (AIA). By varying the Rydberg-Rydberg interaction strengths, the system can emulate different three-level LZ models, for instance, bow-tie and triangular LZ models. The LZ dynamics exhibits nontrivial dependence on the initial state, the quench rate, and the interaction strengths. For large interaction strengths, the dynamics is well captured by AIA. In the end, we analyze the periodically driven case, and AIA reveals a rich phase structure involved in the dynamics. The latter may find applications in quantum state preparation, quantum phase gates, and atom interferometry.