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Journal of the Optical Society of America B

Spectra of single-atom lasers

James Clemens, Perry R. Rice, Leno M. Pedrotti

Published Nov 1, 2004• 15 citations
Publisher

Abstract

We calculate the output spectrum of a single-atom laser in a microcavity across a wide range of operating conditions. We considered both three-level and four-level atomic level structures. We used a numerical routine to calculate spectra that is more efficient than others used previously. We found that the linewidth of a single-atom laser generally scales as the inverse of the photon number and that there is no pump value at which an abrupt change occurs that might locate a lasing threshold. For a three-level gain atom we found vacuum–Rabi splitting similar to that found by Loffler et al. [Phys. Rev. A 55, 3923 (1997)] and used quantum trajectory theory to obtain a new interpretation of the results. For a four-level gain atom the vacuum–Rabi structure can appear at a small nonzero pump level and is maintained for large pumps, even when the intracavity photon number is larger than unity and the laser is on. We use the quantum trajectory approach to explain these results.

DOI
10.1364/josab.21.002025

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Annual Meeting Optical Society of America•Jan 1, 1989•0 citations
We calculate the output spectrum of a single-atom laser in a microcavity across a wide range of operating conditions. We considered both three-level and four-level atomic level structures. We used a numerical routine to calculate spectra that is more efficient than others used previously. We found that the linewidth of a single-atom laser generally scales as the inverse of the photon number and that there is no pump value at which an abrupt change occurs that might locate a lasing threshold. For a three-level gain atom we found vacuum–Rabi splitting similar to that found by Loffler et al. [Phys. Rev. A 55, 3923 (1997)] and used quantum trajectory theory to obtain a new interpretation of the results. For a four-level gain atom the vacuum–Rabi structure can appear at a small nonzero pump level and is maintained for large pumps, even when the intracavity photon number is larger than unity and the laser is on. We use the quantum trajectory approach to explain these results.
We consider a laser composed of a single atom in a microcavity, with a coherent or incoherent pump. We consider both three- and four-level gain schemes, and examine the output spectrum of such lasers. We find that the linewidth generally scales as the inverse of the photon number. For large atom-field coupling, a vacuum-Rabi doublet structure is obtained. In the three-level case, this vacuum-Rabi splitting is apparent only for small intracavity photon numbers, and vanishes for large pumps. In the four-level scheme, the vacuum-Rabi structure appears at a nonzero pump level, and is maintained for large pumps, even when the intracavity photon number is larger than unity. This behavior is explained utilizing the quantum trajectory approach.
We consider a laser model consisting of a single four-level or three-level atom, an optical cavity, and an incoherent pump. Results for photon statistics for varying pump levels are obtained using a quantum trajectory algorithm. In particular, we calculate the mean photon number, Fano factor (which is the variance over the mean). We examine that the behavior of the single-atom device as \ensuremath{\beta}, the fraction of spontaneous emission into the lasing mode, is varied. Typical values considered for \ensuremath{\beta} are $0.01<\ensuremath{\beta}<1.0.$ We find that for large enough \ensuremath{\beta}, lasing action, with properties similar to those predicted by semiclassical theories that factorize atom-field correlations and use a small-noise approximation, can occur. Squeezing can occur as \ensuremath{\beta} is increased. There is no evidence of a sharp phase transition from weakly excited thermal light to coherent light at a particular pump power. This is consistent with work on many-atom lasers with \ensuremath{\beta} values in the range considered here. As \ensuremath{\beta} is increased, the output goes from quasithermal light to coherent and finally to squeezed light, progressing into a fully quantum-mechanical regime. We also consider the effects of cavity damping and spontaneous emission rates on these results.
Our recent paper reports the experimental realization of a one-atom laser in a regime of strong coupling [J. McKeever, A. Boca, A. D. Boozer, J. R. Buck, and H. J. Kimble, Nature (London) 425, 268 (2003)]. Here we provide the supporting theoretical analysis relevant to the operating regime of our experiment. By way of a simplified four-state model, we investigate the passage from the domain of conventional laser theory into the regime of strong coupling for a single intracavity atom pumped by coherent external fields. The four-state model is also employed to exhibit the vacuum-Rabi splitting and to calculate the optical spectrum. We next extend this model to incorporate the relevant Zeeman hyperfine states as well as a simple description of the pumping processes in the presence of polarization gradients and atomic motion. This extended model is employed to make quantitative comparisons with our earlier measurements for the intracavity photon number versus pump strength and for the photon statistics as expressed by the intensity correlation function ${g}^{(2)}(\ensuremath{\tau})$.
We use standard quantum laser theory to examine the linewidth of lasers with a four-level atomic gain medium as a function of the spontaneous emission rate into the lasing mode and the decay rates from the upper and lower lasing levels. We find that the laser linewidth ceases to exhibit the customary decrease with increased photon number when a critical photon number, proportional to the ratio of the decay rate from the lower lasing level to the rate of spontaneous emission into the lasing mode, is reached. This critical photon number would decrease as the size of the optical cavity is decreased. In addition we show that, in general, the laser linewidth depends critically on the ratio of the overall decay rates from the upper and lower lasing levels.
The standard theory of resonance fluorescence is a weak-coupling theory.1 If n ¯ is the mean photon number for the driving field, g is the atom field coupling constant, and γ is the Einstein A coefficient, formally the standard theory of resonance fluorescence assumes the limit n ¯ → ∞ , g/ γ → 0, with the ratio of Rabi frequency to atomic linewidth 2 n ¯ n g / γ finite. The limit g/γ → 0 allows the variation of the Rabi frequency 2 n g across the photon number distribution of the driving field to be neglected. By placing the atom inside an optical cavity the ratio g/γ can be changed. In this paper we calculate spectra for intracavity resonance fluorescence in the strong-coupling limit g/γ ≫ 1, g/κ ≫ 1, where κ is the cavity linewidth. We consider a single two-level atom interacting on resonance with a single cavity mode driven by a resonant coherent field. The cavity subtends a small solid angle at the atom, so that the spontaneous emission into free-space modes is not negligible. We calculate the spectrum of the light transmitted by the cavity (the transmitted spectrum) and the spectrum of the light radiated by the atom into free space (the fluorescent spectrum). The transmitted and fluorescent spectra show fundamental differences from the (weak-coupling) spectrum of free-space resonance fluorescence.