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Journal of Modern Optics

Projection lithography by means of parametric photon pairs

Naoki Fukutake

Published Feb 21, 2006• 4 citations
Publisher

Abstract

It is well known that entangled-photon pairs generated by spontaneous parametric down-conversion exhibit a property that is analogous to that of ordinary incoherent lights. We formulate an image-forming optical theory of quantum lithography that comprehends the both conceptions of partial coherence and partial entanglement by extending a classical image-forming optical theory. Our optical system consists of an image-forming system, an illumination system with a second-order nonlinear medium, and two-photon absorbing materials. We evaluate the resolution of the quantum lithography system by using the optical transfer function and show a special case to be a super-resolving system.

DOI
10.1080/09500340500443128

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arXiv:0909.4382•Physical Review A•Oct 19, 2009•47 citations
It is well known that entangled-photon pairs generated by spontaneous parametric down-conversion exhibit a property that is analogous to that of ordinary incoherent lights. We formulate an image-forming optical theory of quantum lithography that comprehends the both conceptions of partial coherence and partial entanglement by extending a classical image-forming optical theory. Our optical system consists of an image-forming system, an illumination system with a second-order nonlinear medium, and two-photon absorbing materials. We evaluate the resolution of the quantum lithography system by using the optical transfer function and show a special case to be a super-resolving system.
We formulate an image-forming optical theory of quantum lithography in which Entangled-photon pairs generated by spontaneous parametric down-conversion play an important role. Our optical system consists of an image-forming system, an illumination system with a second-order nonlinear medium, and two-photon absorbing materials. We evaluate the resolution of the quantum lithography system by using the optical transfer function and show a super-resolving condition which is, however, difficult to achieve.
Relating to magnified image formation systems, we consider two processes in this work: quantum and classical incoherent imaging. There are similarities and differences between them. A similarity is that the optical transfer functions (OTFs) of both systems are obtained by calculating a correlation function. Concerning the differences, only two were found. The first difference is that, unlike classical incoherent imaging, quantum imaging with photon pairs generated by spontaneous parametric down-conversion is sensitive to the phase in the function which describes the object. The second difference is that the OTF of the quantum imaging system is a cross-correlation function of the OTFs of the signal and idler arms, while the OTF of the classical incoherent imaging system is an autocorrelation of the only pupil function existing in this case. We explore experimentally the second difference. We report the observation of a highly resolved image produced by a quantum light source in a setup where an incoherent light source is unable to spatially resolve the image of the object. The spatial resolution of the image is studied in a situation where the size of the object is magnified at the image.
At the end of last century, the name of “quantum lithography” has been emerged. This exciting approach was proposed for making a resolution two times higher than that of the conventional optics without changing a wavelength and a numerical aperture. For those who want optical lithography to last long, this has been thought to be a great technology. However, an applicability of the proposed method to the current exposure system i.e., reduced projection exposure system has not yet been examined clearly. We have investigated the proposed quantum lithography to apply into the current exposure system using reticle. For simplicity, coherent illumination i.e. sigma is zero condition is used for calculation. Our quantum lithography compatible to mask exposure system explains probability of one and two photon absorption on the image plane i.e. on wafer. We have shown that the half-wavelength quantum lithography using conventional mask exposure system is impossible because diffraction at the mask makes biphoton into two photon. We have found that there is still super-resolution quantum lithography using mask exposure, however, there is little possibility of quantum lithography practically today because biphoton light source is as dark as stars. To realize quantum lithography practically, further development of not only biphoton light source but also two-photon absorption resist is indispensable.
Entangled-photon pairs (biphotons) generated by spontaneous optical parametric down-conversion exhibit a number of properties that are analogous to those of ordinary photons generated by incoherent sources. The spatial pump-field distribution and the two-particle wave function in the biphoton case play the respective roles of the source intensity distribution and the second-order coherence function in the incoherent case. The van Cittert--Zernike theorem, which is applicable for incoherent optical sources emitting independent photons, has a counterpart for biphotons. Likewise, the partial-coherence theory of image formation has an analogous counterpart for biphoton beams transporting spatial information. However, an underlying duality, rather than analogy, accompanies the mathematical similarity between incoherent and biphoton emissions if the comparison is made between the photon count rate in the incoherent case and the biphoton count rate in the entangled-photon case. The smaller the size of an incoherent source, the more separable is the coherence function and the more coherent is the field, and therefore the higher the visibility of ordinary interference fringes. In contrast, the narrower the size of a biphoton pump source, the more separable is the wave function and the less entangled is the field, and therefore the lower the visibility of biphoton interference fringes. This duality is similar to the complementarity between single and two-photon interference exhibited for biphotons.
Since the early days of quantum mechanics, physicists have been puzzled by the counterintuitive consequences of entanglement. Quantum imaging is one of the most intriguing effects exhibiting the typical nonlocal behavior of entangled states and has in fact stimulated an intense debate regarding fundamental issues of quantum theory. Recently, particular attention has been given to the possibility of simulating quantum imaging classically, that is, without entanglement. The study of quantum imaging has also lead to useful practical applications such as high precision nonlocal timing-positioning and quantum lithography, in which measurements may achieve resolution even beyond the classical limits. In this paper, we first introduce the concept of quantum imaging and emphasize its peculiar quantum nature through a set of inequalities derived from the historical argument of Einstein, Podolsky and Rosen (EPR). The EPR inequalities are the quantitative formulation of the very different physics governing entangled and separable systems. We show that two-photon imaging may achieve its fundamental limit only through nonlocal measurements realized on entangled photon pairs. Furthermore, we show that quantum imaging may be exploited to overcome the Rayleigh diffraction limit; this is the basic idea behind quantum lithography. Finally, we discuss the possibility of extending the coherent two-photon imaging typical of entangled photon pairs to incoherent coincidence imaging, by employing chaotic light. From an applicative viewpoint, chaotic radiation may represent the ideal candidate for mimicking quantum ghost imaging, provided adequate detection schemes are developed.
The second-order Talbot effect is analyzed for a periodic object illuminated by entangled photon pairs in both the quantum imaging and quantum lithography configurations. The Klyshko picture is applied to describe the quantum imaging scheme, in which self-images of the object that may or may not be magnified can be observed nonlocally in the photon coincidences but not in the singles count rate. In the quantum lithography setup, we find that the second-order Talbot length is half that of the classical first-order case, thus the resolution may be improved by a factor of 2.