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Physical Review A

Atomic diffusion in an optical quasicrystal with five-fold symmetry

Luca Guidoni, B. Dépret, A. di Stefano, Philippe Verkerk

Published Dec 1, 1999• 54 citations
Publisher

Abstract

We present experimental and numerical studies of the atomic motion in an optical lattice displaying a fivefold rotational symmetry. The atomic transport has been investigated by measuring the time evolution of the size of the atomic cloud. The experimental results are compared to those of a semiclassical Monte Carlo simulation of the atomic motion in a three-dimensional optical quasicrystal. A good agreement has been obtained on the anisotropy of the diffusive expansion of the cloud.

DOI
10.1103/physreva.60.r4233

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•Jun 23, 2025•0 citations
We present experimental and numerical studies of the atomic motion in an optical lattice displaying a fivefold rotational symmetry. The atomic transport has been investigated by measuring the time evolution of the size of the atomic cloud. The experimental results are compared to those of a semiclassical Monte Carlo simulation of the atomic motion in a three-dimensional optical quasicrystal. A good agreement has been obtained on the anisotropy of the diffusive expansion of the cloud.
Quasicrystals are nonperiodic structures having no translational symmetry but nonetheless possessing long-range order. The material properties of quasicrystals, particularly their low-temperature behavior, defy easy description. We present a compact optical setup for creating quasicrystal optical potentials with five-fold symmetry using interference of nearly co-propagating beams for use in ultracold atom quantum simulation experiments. We verify the optical design through numerical simulations and demonstrate a prototype system. We also discuss generating phason excitations and quantized transport in the quasicrystal through phase modulation of the beams.
We study the kinetic temperature and the localization of cesium atoms in a three dimensional quasiperiodic optical potential created by the interference of five or six laser beams. Bragg scattering experiments show evidence of a quasiperiodic order for the atomic density. Temperature measurements are consistent with the topological invariance of the optical potential under phase variations of the laser beams. Numerical semiclassical Monte Carlo simulations show results in reasonable agreement with the experimental observations.
We carry out quantum and semiclassical numerical simulations of the dynamics, particularly diffusion, of atoms in an optical lattice. We consider specifically the situation of a $J=1/2\ensuremath{\leftrightarrow}J=3/2$ atomic transition, whose experimental counterpart can be realized in Mg+{\mathrm{Mg}}^{+}Mg+ experiments. The semiclassical results, which cover a larger range of parameters than would be practical for fully quantum calculations, confirm and extend the work of Marksteiner et al. [Phys. Rev. A 53, 3409 (1996)], characterize the transition from normal to anomalous diffusion and the atomic trajectories which give rise to it, and provide a physical explanation for the difference between these two regimes. The full quantum calculations reveal uniquely quantum features of individual atomic trajectories, and in addition, predict significantly lower diffusion, by a factor of 1.2 to 2, than their semiclassical counterparts.
We study dissipative transport of spontaneously emitting atoms in a one-dimensional (1D) standing-wave laser field in the regimes where the underlying deterministic Hamiltonian dynamics is regular and chaotic. A Monte Carlo stochastic wave-function method is applied to simulate semiclassically the atomic dynamics with coupled internal and translational degrees of freedom. It is shown in numerical experiments and confirmed analytically that chaotic atomic transport can take the form either of ballistic motion or a random walking with specific statistical properties. The character of spatial and momentum diffusion in the ballistic atomic transport is shown to change abruptly in the atom-laser detuning regime where the Hamiltonian dynamics is irregular in the sense of dynamical chaos. We find a clear correlation between the behavior of the momentum diffusion coefficient and Hamiltonian chaos probability which is a manifestation of chaoticity of the fundamental atom-light interaction in the diffusivelike dissipative atomic transport. We propose to measure a linear extent of atomic clouds in a 1D optical lattice and predict that, beginning with those values of the mean cloud's momentum for which the probability of Hamiltonian chaos is close to 1, the linear extent of the corresponding clouds should increase sharply. A sensitive dependence of statistical characteristics of dissipative transport on the values of the detuning allows us to manipulate the atomic transport by changing the laser frequency.
We investigate the properties of Bose–Einstein condensates (BECs) in a two-dimensional quasi-periodic optical lattice (OL) with eightfold rotational symmetry by numerically solving the Gross–Pitaevskii equation. In a stationary external harmonic trapping potential, we first analyze the evolution of matter-wave interference pattern from periodic to quasi-periodic as the OL is changed continuously from four-fold periodic to eight-fold quasi-periodic. We also investigate the transport properties during this evolution for different interatomic interaction and lattice depth, and find that the BEC crosses over from ballistic diffusion to localization. Finally, we focus on the case of eightfold symmetric lattice and consider a global rotation imposed by the external trapping potential. The BEC shows vortex pattern with eightfold symmetry for slow rotation, becomes unstable for intermediate rotation, and exhibits annular solitons with approximate axial symmetry for fast rotation. These results can be readily demonstrated in experiments using the same configuration as in Phys. Rev. Lett. 122 110404 (2019).
This thesis concerns the physics of ultracold bosons in quasicrystalline lattices, studied by means of quantum simulation using ultracold 39K atoms loaded to an eight-fold rotationally symmetric optical quasicrystal. Quasicrystalline and quasiperiodic systems, thanks to their long-range order and lack of periodicity, exhibit a wealth of interesting properties such as a dense and self-similar momentum space, and a localization transition to Anderson insulator or Bose glass states (in non-interacting or interacting cases respectively) reminiscent of that in disordered systems, whilst lacking the rare regions that typically exist in such systems. Here we will cover experiments into this system’s behaviour in both equilibrium and non-equilibrium settings. First, we focus on mapping out its phase diagram in both weakly and strongly interacting regimes. We observe consistency with numerical predictions for the superfluid-Bose glass phase transition using coherence measurements, as well as finding a region of roughly zero compressibility around where the numerics predicts the existence of a Mott insulator ground state. We also study which regimes of the phase diagram can be ramped through adiabatically, finding that entropy is created upon traversing the Bose glass phase irrespective of ramp duration, which we attribute to its localized nature. Next we look into the dynamics of the system after a quench of the lattice depth in the weakly interacting regime. Upon quenching from the superfluid regime to the Bose glass regime, we observe a quantum walk to higher order diffraction peaks in momentum space whose maximum order is unbounded by kinetic energy thanks to the dense, self-similar nature of the quasicrystal’s momentum space. Quenching in the opposite direction we observe instead a walk between sites in real space for short times by looking at the position (as opposed to momentum) space autocorrelation function of the cloud, finding an expansion rate in agreement with an intuitive estimate based on the Lieb-Robinson bounds of a periodic system. We also look into the timescales of these dynamics in the context of what we might expect from the underlying Hamiltonian, before finally investigating the loss of coherence exhibited by the system after a slower quench of the lattice depth from an initially superfluid cloud. We observe that coherence is lost sooner after the quench for deeper final lattices, with the loss becoming almost instantaneous for quenches that cross the localization transition across the whole cloud. After this we explore the system’s transport dynamics by means of a quench to an excited state at the same time as an additional confining potential is switched off. We observe that unlike in the case of a periodic square lattice, where ballistic expansion that scales with the tunnelling strength occurs in the non-interacting case before becoming slower upon the introduction of interactions thanks to diffusion, in the quasicrystal the transport rate no longer scales with tunnelling strength. Instead we observe a drop relative to the tunnelling rate by 2 − 3 orders of magnitude as the lattice depth is increased from 1Er to 5Er with little dependence on the interaction strength. We also note that the finite rate measured for the deeper lattices is potentially an overestimate since the finite loss rate of atoms makes mass transport indistinguishable from density-dependent losses at that point. Finally, we discuss use of a quantum gas magnification scheme with which to magnify the real space density distribution of our atoms such that it can be measured with single-site resolution. Some preliminary results are presented regarding how the density distribution changes with lattice depth in the weakly interacting regime, in which we observe that as lattice depth increases a higher proportion of atoms occupy deeper sites close to the centre of the quasicrystal’s configuration space, as we might expect.