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Physical Review Letters

Young-Type Experiment Using a Single-Electron Source and an Independent Atomic-Size Two-Center Interferometer

J.-Y. Chesnel, Anas Hajaji, R O Barrachina, F. Frémont

Published Mar 8, 2007• 30 citations
Publisher

Abstract

Evidence is given for Young-type interferences caused by a single electron acting on a given double-center scatterer analogous to an atomic-size double-slit system. The electron is provided by autoionization of a doubly excited He atom following the capture of the electrons of H2 by a He2+ incoming ion. The autoionizing projectile is a single-electron source, independent of the interferometer provided by the two H+ centers of the fully ionized H2 molecule. This experiment resembles the famous thought experiment imagined by Feynman in 1963, in which the quantum nature of the electron is illustrated from a Young-like double-slit experiment. Well-defined oscillations are visible in the angular distribution of the scattered electrons, showing that each electron interferes with itself.

DOI
10.1103/physrevlett.98.100403

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Evidence is given for Young-type interferences caused by a single electron acting on a given double-center scatterer analogous to an atomic-size double-slit system. The electron is provided by autoionization of a doubly excited He atom following the capture of the electrons of H2 by a He2+ incoming ion. The autoionizing projectile is a single-electron source, independent of the interferometer provided by the two H+ centers of the fully ionized H2 molecule. This experiment resembles the famous thought experiment imagined by Feynman in 1963, in which the quantum nature of the electron is illustrated from a Young-like double-slit experiment. Well-defined oscillations are visible in the angular distribution of the scattered electrons, showing that each electron interferes with itself.
Interferences caused by a single electron impacting on an independent double-center scatterer, which plays the role of an atomic-size double-slit system, are experimentally evidenced for the first time. The electron originates from the autoionization of doubly excited 2 l n l ' (n ⩾ 2) configurations of He following a double charge exchange process by He 2+ ions impinging on H 2 molecules. Well-defined oscillations are visible in the angular distribution of the electrons emitted towards the receding H + protons. The presence of these oscillations demonstrates that a single electron interferes with itself. This is analogous to the famous "thought" experiment imagined and discussed by Feynman in 1963, in which the quantum nature of the electron was illustrated by making it traverse an atomic-size double-slit arrangement.
For the last 50 years, there has been considerable interest in the possibility of observing the equivalence of a Young's double-slit wave interference at the quantum level for diatomic molecules. For electron-impact ionization of diatomic molecules, indirect evidence for this type of interference has been found by changing the energy (wavelength) of the ejected electron while keeping the incident projectile scattering angle fixed. The present work represents an experimental and theoretical collaboration to better understand the physics of this type of interference. In addition to examining the effect of changing the ejected electron energy for a fixed scattered projectile angle, we have also examined the effect of keeping the ejected electron energy fixed while varying the projectile scattering angle. Model calculations are performed for three different types of possible two-center interference effects, and it is found that the most important one is diffraction of the projectile off two scattering centers.
Des interférences dues à la diffusion d’un électron unique sur deux protons, qui jouent le rôle de deux trous de Young, ont été mises en évidence expérimentalement pour la première fois. L’électron provient de l’auto-ionisation de l’hélium excité après capture de deux électrons de la molécule H2 par un projectile He2+. Ces interférences se manifestent par l’apparition d’oscillations d’intensité dans la distribution angulaire des électrons diffusés. La présence de ces oscillations prouve qu’un électron peut interférer avec lui-même. L’expérience présente est analogue a une expérience de pensée imaginée par Feynman en 1963.
We report the first observation of Young-type interference effects in a two-electron transfer process. These effects change strongly as the projectile velocity changes in fast (1.2 and 2.0 MeV) He(2+) + H(2) collisions as manifested in strong variations of the double-electron capture rates with the H(2) orientation. This is consistent with fully quantum mechanical calculations, which ignore sequential electron transfer, and a simple projectile de Broglie wave picture assuming that two-electron transfer probabilities are higher in collisions where the projectile passes close to either one of the H(2) nuclei.
A single-atom "double-slit" experiment is realized by photoionizing rubidium atoms using two independent low power lasers. The photoelectron wave of well-defined energy recedes to the continuum either from the 5P or 6P states in the same atom, resulting in two-path interference imaged in the far field using a photoelectron detector. Even though the lasers are independent and not phase locked, the transitions within the atom impart the phase relationship necessary for interference. The experiment is designed so that either 5P or 6P states are excited by one laser, before ionization by the second beam. The measurement cannot determine which excitation path is taken, resulting in interference in wave-vector space analogous to Young's double-slit studies. As the lasers are tunable in both frequency and intensity, the individual excitation-ionization pathways can be varied, allowing dynamic control of the interference term. Since the electron wave recedes in the Coulomb potential of the residual ion, a quantum model is used to capture the dynamics. Excellent agreement is found between theory and experiment.