We study the general problem of matter-laser interaction within the framework of nonrelativistic quantum electrodynamics, with particular emphasis on strong laser field effects. Consequently, we formulate a well-defined approximation leading in a straightforward manner toward the conventional semiclassical mode of description. Namely, we arrive naturally to two coupled equations of motion: (i) the Schr\"odinger equation which governs the quantum dynamics of an atomic system driven by classically described radiation field (composed of an incoming laser pulse plus radiation emitted from the atom), and (ii) the classical Maxwell wave equation which describes the emission of radiation from the mentioned atomic source. Employing the formalism of adiabatic Floquet theory, we derive a simple criterion of validity of the just described semiclassical approach. It shows that the semiclassical treatment is justified in most situations. On the other hand, it turns out that the semiclassical approximation breaks down completely in certain special but realistic cases, regardless of the fact that the incoming laser pulse contains a huge number of photons. Under such special circumstances, we anticipate new effects arising due to the quantized nature of the radiation field, to be observable, for example, in harmonic generation spectra. Our considerations are illustrated more explicitly using a simple model of a two-level atom strongly driven by a laser. The quantum dynamics of this model problem is resolved within the framework of quantum electrodynamics while adopting well-defined and physically justifiable approximations. As an outcome, analytic formulas are found serving as a quantitative criterion of (non)applicability of the semiclassical approach and demonstrating the breakdown of semiclassical theory under well-defined conditions. An illustrative numerical calculation is provided.
The interaction of nonrelativistic matter with the quantized electromagnetic field is investigated in the classical limit of large photon numbers. Quantization of both matter, say an atom, and the field results in a time-independent Schr\"odinger equation (TISE). However, for very strong fields (quantum mechanically, large photon numbers) this is impractical to solve. The standard approach then is simply to replace the quantized field by a classical field to give a time-dependent Schr\"odinger equation (TDSE) for the atom alone. Here we show how this TDSE can be derived from the TISE for atom plus field, illustrating at each stage the approximations that are necessary to treat the field classically. An important difficulty at the semiclassical stage is a breakdown of the approximation at classical turning points. We show how the use of coherent field states can circumvent this problem. In the limit that the field can be treated classically, time emerges from the Maxwell equations and a TDSE for the atom alone results.
The interaction of an atomic system with an unquantized electromagnetic field is studied by means of the Heisenberg-operator equations of motion. The electromagnetic fields created by the atom are taken into account by assuming that the charge and probability current densities are the actual charge and current source terms in Maxwell's equation. When Ehrenfest's theorem is written to order (1/c
)2, the equations of motion are found to have a constant of motion that can be interpreted as stating that the sum of the atomic energy, energy of interaction, and energy stored in the electromagnetic field is constant. This constant of integration can be expressed as an expectation of a new semiclassical Hamiltonian that now includes the effects of the atomic self-fields to order 1/
c2. This Hamiltonian is related to the classical Darwin Lagrangian. Since the new approximate Hamiltonian is the sum of an atomic and a field Hamiltonian, it provides a formulation of semiclassical radiation theory that is formally close to the usual formulation of quantum electrodynamics. A Schr\"odinger equation can be derived by applying the variational principle to the expectation of the new Hamiltonian. The result is a nonlinear integro-differential equation, in \ensuremath{\Psi}, which is somewhat similar to Hartree's self-consistent equation for a multielectron atom.When the Heisenberg equations are written to include the next-higher-order terms, 1/
c3, it is found that the total energy of the atom and the electromagnetic field in the vicinity of the atom decreases at a rate that is given by the Larmor power formula (2
e2/3
c3)(d〈v〉/dt
)2, where 〈v〉 is the quantum-mechanical expectation of the electron's velocity operator. This approximate formulation of semiclassical radiation theory is applied to semiclassical calculations of atomic radiative shifts. It is then shown that, if some retardation effects are included to all orders of 1/c in the vector potential, the semiclassical analysis provides a formula for radiative energy-level shifts that are time dependent and that contain coefficients similar to the starting point of the Bethe calculation of the Lamb shift. The incorporation of mass renormalization in semiclassical theory is then discussed.
A symplectically covariant quantum-mechanical uncertainty relation more accurate than previously known ones is derived for multidimensional systems. It is shown that the quantum-mechanical description of a linear Hamiltonian system in terms of squeezed states is completely equivalent to its description in terms of a phase-space distribution function. A new approach to the semiclassical limit is proposed, based on the use of squeezed states. By analyzing explicit formulas for squeezed states, a semiclassical asymptotic form of the solution to the Cauchy problem for a multidimensional Schrödinger equation is found in the limit of ħ → 0. The behavior of the semiclassical solution in the neighborhood of a caustic is analyzed in the one-dimensional case, and the phase shift across the caustic is determined. General properties and examples of squeezed states are discussed that point to the fundamental importance of squeezed states for developing a nonrelativistic quantum-mechanical description of a system of charged particles in an electromagnetic field in the dipole approximation.
In a concise, but accessible for the first acquaintance form the procedure for the quantization of linear oscillator is set out. By analogy with this procedure the procedure of quantization (second quantization) of classical Maxwell’s electrodynamics is set up. The physical sense of the wave functions arguments of transverse electromagnetic field and its Fourier transformation is set up. One pay attention as for quantum coherent (almost a classic) states of the electromagnetic field and for photonics Fock states. Attention is drawn to the fact of absence the power of the universal content of such concepts as field amplitude, phase and number of particles (photons), which are used by experimenter’s to describe the states of a quantized field. The semi quantitative description the interaction processes of a quantum electromagnetic field with substance is set up. Specified situations are shown in which the discrepancy between the predictions of classical and quantum electrodynamics is noticeable at the macroscopic level.