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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Efficient nonlinear wave-mixing processes via slow and fast light

Yuri V. Rostovtsev

Published Feb 10, 2011• 0 citations
Publisher

Abstract

The talk consists of two parts. In the first, we have demonstrated enhancement of nonlinear signals and suggested a new approach that extends Raman spectroscopy to media which has a high level of scattering. The stimulated Raman scattering has an advantage of relaxing phase-matching condition which is difficult or even impossible to meet under condition of strong scattering. The second topic is related to enhanced optico-mechanical coupling that occurs when the group velocity of light is ultra-slow. We show theoretically that, due to dragging of the light by the mechanical motion of the medium, it is possible to control phase-matching condition.

DOI
10.1117/12.880800

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The talk consists of two parts. In the first, we have demonstrated enhancement of nonlinear signals and suggested a new approach that extends Raman spectroscopy to media which has a high level of scattering. The stimulated Raman scattering has an advantage of relaxing phase-matching condition which is difficult or even impossible to meet under condition of strong scattering. The second topic is related to enhanced optico-mechanical coupling that occurs when the group velocity of light is ultra-slow. We show theoretically that, due to dragging of the light by the mechanical motion of the medium, it is possible to control phase-matching condition.
The predominantplace occupiedby optical fibers inmodernphotonic systems has steadily stimulated research to realize slow and fast light devices directly in this close-to-perfect transmission line. This potentially offers the key advantage of a seamless and flexible integration in most optical transmission systems. The main obstacle for such a realization is related to the highly disordered amorphous nature of the silica constituting the optical fibers, prohibiting the use of narrowband atomic transitions. The most efficient approach to create a narrowband gain or loss in optical fibers remains the exploitation of an optical interaction requiring a strict phase matching condition to be satisfied. This can be realized using the nonlinear optical response of the material that offers the possibility to transfer the energy from one optical wave to another lightwave. For instance, a resonant coupling over a narrow frequency range is observed in parametric interactions, which are conditioned to the generation of a third idler wave for the fulfillment of a phase matching condition. The optical wave that benefits from the energy transfer will actually experience a linear gain and therefore be subject to light slowing, while the depleted wave undergoes a linear loss and will experience a fast light effect.
In today's information age demand for ultra-fast information transfer with ultra-high bandwidths has reached extraordinary levels. Hence, the transmission in the future internet-backbone will be increasingly constrained in the network nodes. At the same time, the power consumption of the network systems will increase to unsustainable levels.\nNowadays, optical signal processing and switching can be implemented relatively easily. However, the realization of optical bu ers and short-term memories is still an unsolved challenge. The slow- and fast-light e ect has been investigated as one solution for the optical bu ering over the last few years. It means the slowing down and acceleration of the group velocity of light pulses in a medium. To realize this, many di erent methods and material systems have been developed but due to its signi cant advantages the nonlinear e ect of stimulated Brillouin scattering (SBS) is particularly promising. However, it also su ers from disadvantages which limit the slow- and fast-light performance.
Slow and fast light (SFL) in nonlinear media has attracted considerable interest for several years and has been observed in plenty of configurations. It generally requires a sharp spectral resonance which in turn results in a strong change of the group velocity at the resonance, thus leading to optical delaying or advancement. SFL has also been observed in optical fibres by taking advantage of the parametric gain, stimulated Brillouin or Raman scattering, leading to the development of all-optical tunable fiber-based delay lines at telecommunication wavelengths. But the implications of SFL go well beyond pulse delaying or advancement. As the group and phase velocities have to be distinguished one from another in a slow-light medium, this can have other important implications, in particular on the pulse walk-off or on the frequency chirp. We recently demonstrated in a Raman medium with normal dispersion that pulse walk-off between the pump and the signal can be cancelled out despite the large frequency detuning, leading to an increasing interaction length and enhancement Raman conversion efficiency.
Summary form only given. Recently, considerable attention has been drawn to extremely slow light obtained in the conditions of electromagnetically induced transparency. The reason is that slow light may lead to exceptionally large nonlinearities and, in particular, to efficient nonlinear processes at energies of a few photons per atomic cross section. Extremely low group velocities of light have been observed in resonant systems such as a Bose-Einstein condensate of ultracold sodium atoms or hot rubidium vapors. Meanwhile, there is a large number of nonlinear optical techniques based on nonresonant interaction. Therefore, it is desirable to study the possibility of slow light in far-off-resonance media. In the present work, we demonstrate experimentally that far-off-resonance stimulated Raman scattering in solid hydrogen driven by a strong coupling field allows us to slow down the intensity-peak velocity of the Stokes and antiStokes fields.
We study the propagation dynamics of weak Raman sideband fields in a far-off-resonance Raman medium driven by a strong coupling field. We show that the interaction of the system with the strong field, under the conditions of high density, narrow Raman-transition width, and small two-photon detuning, results ina slow group velocity and a substantial enhancement of the injected anti-Stokes sideband field as well as an efficient generation of a Stokes sideband field. We find that the effective group velocity is the same for the two weak fields and is proportional to the field frequency difference instead of the frequency of the corresponding field. We also discuss the condition for exponential growth of the two sideband fields in the medium. We perform numerical calculations for solid hydrogen, a realistic system where the requirements for high density and small Raman width can be met. We demonstrate that the group velocity can be slowed down by several orders, and that the slow light plays a key role for the stimulated Raman scattering process in solid hydrogen.PACS Nos.: 42.50Gy, 42.50Hz, 42.65Ky, 42.79Nv