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Physical Review A

Measurements of quantum noise in optical phase conjugation via four-wave mixing in an atomic vapor

Mary Yvonne Lanzerotti, Robert W. Schirmer, Alexander L. Gaeta, G. S. Agarwal

Published Dec 1, 1999• 3 citations
Publisher

Abstract

We present the results of a comprehensive investigation of the quantum-noise properties of a continuous-wave phase-conjugate mirror (PCM) formed using backward-four-wave mixing in potassium vapor. We characterize the quantum-noise properties of the PCM as functions of the vapor density, pump detuning from resonance, and relative frequency detuning of the signal beam from the probe beam. We compare the noise measurements of the PCM with the predicted noise of an ideal quantum-noise-limited PCM and determine the value of the minimum signal that can be used to perform phase conjugation with unity signal-to-noise ratio. For the range of vapor densities studied, we find that the PCM operates nearest the quantum-noise limit and that the value of the minimum signal is lowest under conditions in which the reflectivity is maximized. These results demonstrate that it is possible to perform phase conjugation with signals as weak as 14 fW with near-unity reflectivity. Our measurements are in qualitative agreement with the predictions of a quantum theory of phase conjugation via nearly degenerate four-wave mixing in a two-level system.

DOI
10.1103/physreva.60.4980

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We present the results of a comprehensive investigation of the quantum-noise properties of a continuous-wave phase-conjugate mirror (PCM) formed using backward-four-wave mixing in potassium vapor. We characterize the quantum-noise properties of the PCM as functions of the vapor density, pump detuning from resonance, and relative frequency detuning of the signal beam from the probe beam. We compare the noise measurements of the PCM with the predicted noise of an ideal quantum-noise-limited PCM and determine the value of the minimum signal that can be used to perform phase conjugation with unity signal-to-noise ratio. For the range of vapor densities studied, we find that the PCM operates nearest the quantum-noise limit and that the value of the minimum signal is lowest under conditions in which the reflectivity is maximized. These results demonstrate that it is possible to perform phase conjugation with signals as weak as 14 fW with near-unity reflectivity. Our measurements are in qualitative agreement with the predictions of a quantum theory of phase conjugation via nearly degenerate four-wave mixing in a two-level system.
Summary form only given. We use a high-reflectivity phase-conjugate mirror (PCM) to demonstrate that optical phase conjugation can be performed on continuous-wave signal beams having power spectral densities as low as 5 x 10/sup -18/ W/Hz (i.e., 19 photons/sec.Hz). Our high-reflectivity (>600%), wide-bandwidth (90 MHz) PCM is formed by performing four-wave mixing in a potassium vapor cell using a frequency-stabilized Ti:sapphire laser that is tuned near the D/sub 2/ line. We have measured the noise spectra of the conjugate beam as functions of pump detuning from resonance, probe-pump detuning, pump-probe angular separation, and the number density of potassium atoms.
A quantum theory of nearly degenerate backward four-wave mixing in a two-level atomic system is developed. The theory is used to calculate the quantum noise produced by a phase-conjugate mirror based on this system. The results indicate that in the case of pure radiative broadening the ideal quantum-noise limit is reached for relatively small pump-wave strengths and for relatively large probe-pump and pump-resonance detunings, so that the phase-conjugate reflectivity is far from its maximum value. Conversely, in the collisionally broadened case, operation closest to the quantum-noise limit occurs near the point of maximum reflectivity.
We investigate theoretically the quantum-noise properties of optical phase conjugation via four-wave mixing of nonclassical signal fields. We show that while the field generated at a phase-conjugate mirror (PCM) can be in a nonclassical state, the generated field is not necessarily useful within the context of phase conjugation. For the case in which a quadrature-squeezed signal field is incident at a PCM, we determine that the signal-to-noise ratio of one of the quadrature components of the generated field can approach the signal-to-noise ratio of the corresponding quadrature component of the signal field as the amount of squeezing of the vacuum field injected at the rear of the PCM is increased. For the case in which the signal field is amplitude squeezed, we determine that the signal-to-noise ratio of the conjugate field is always much smaller than that of the signal field. These results demonstrate that the phase-conjugation process can preserve the desirable quantum-noise properties of quadrature-squeezed fields but not those of amplitude-squeezed fields.
We report on a high-reflectivity (up to 670%) wide-bandwidth (up to 230 MHz) phase-conjugate mirror formed using backward-four-wave mixing with continuous-wave pump beams in a 2-mm potassium vapor cell. The reflectivities and bandwidths are significantly larger than have been measured previously, and the bandwidth is ten times greater than is predicted theoretically. The reflectivity-bandwidth product is more than an order of magnitude improvement over those previously achieved with other continuous-wave phase-conjugate systems.
We observe optical phase conjugation using the surface nonlinearity of a dense atomic potassium vapor. For an atomic number density of 1.5\ifmmode\times\else\texttimes\fi{}1017{10}^{17}1017 ${\mathrm{cm}}^{\mathrm{\ensuremath{-}}3}$, phase-conjugate reflectivities of 4\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}5}$ are measured for pump intensities approaching the saturation intensity of 10 W ${\mathrm{cm}}^{\mathrm{\ensuremath{-}}2}$. We also demonstrate aberration correction using surface phase conjugation. The measured properties of the surface-phase-conjugate signal are in excellent agreement with the predictions of a theory of surface phase conjugation by degenerate four-wave mixing, in which the origin of the nonlinear response is saturated absorption.