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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Boundary effects in the process of spontaneous emission in a one-dimensional chain of atoms

Konstantin V. Krutitsky, Oleg N. Gadomsky

Published Sep 26, 1997• 0 citations
Publisher

Abstract

Boundary problem of quantum optics for spontaneous emission of atom embedded in one-dimensional chain of discrete dipoles is solved. The role of boundary effects caused by violation of translational symmetry in atomic spatial distribution is investigated. Life time of excited state and frequency shift of atomic transition are calculated. It is shown that these spectral characteristics significantly depend on atomic position in the chain. Angular distribution of spontaneous photons is also investigated. Theoretical analysis is based on the system of Heisenberg equations for atomic and field operators. For the calculation of the mode functions it is employed as the method of integro-differential equations.

DOI
10.1117/12.287675

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Boundary problem of quantum optics for spontaneous emission of atom embedded in one-dimensional chain of discrete dipoles is solved. The role of boundary effects caused by violation of translational symmetry in atomic spatial distribution is investigated. Life time of excited state and frequency shift of atomic transition are calculated. It is shown that these spectral characteristics significantly depend on atomic position in the chain. Angular distribution of spontaneous photons is also investigated. Theoretical analysis is based on the system of Heisenberg equations for atomic and field operators. For the calculation of the mode functions it is employed as the method of integro-differential equations.
As a contribution to quantum optics in the vicinity of surfaces we study the single atom spontaneous emission in a linear chain of two-level atoms. The electromagnetic field is thereby treated with the help of integro-differential equations which take into account the interaction with the other atoms in the chain. The life time of the excited atom, the frequency shift of the atomic transition and the angular distribution of emitted photons are worked out. They depend on the position of the emitting atom. As compared with the single atom in free space, considerable modifications occur for atoms a few interatomic distances away from the ends of the chain.
We have theoretically investigated the process of spontaneous emission of initially excited two-level atom inside and outside of ultra-thin dielectric film. Dielectric medium is considered as discrete-continuous system of interacting dipoles. For the solution of this boundary problem of quantum optics we use Heisenberg equations for atomic operators. Mode functions of ultra-thin film are calculated by direct solution of integro-differential field equation. Coordinate dependences of excited state life time are analyzed and it is shown that consideration of near-field effect may essentially change spectral properties of the atoms located at small distances from the surface.
We study the spontaneous emission of an atom embedded in a one-dimensional photonic crystal or superlattice using a classical electrodynamic theory of radiation. The rate of emission is a function of the frequency of the emitted photon, the dipole's position and orientation, as well as the geometric and material parameters of the superlattice. The emission spectrum shows an oscillatory behavior which follows the photonic band structure. For TE modes, there are frequency regions where radiative emission is completely prohibited due to the absence of modes with k//>omega/c; the radiation is then TM polarized. In addition to the radiative modes, there are always evanescent modes with k//>omega/c which are waveguided by the dielectric layers. The evanescent contribution to the spontaneous emission is dominant if a dielectric layer is in the near field region of the dipole. For TM modes, emission rates greatly vary for parallel and perpendicular dipole moments. In a photonic crystal with a high filling fraction of the dielectric and perpendicular dipoles located in the low-index layer, the decay rate can be as much as 76 times the free space value for a single atom and 50 times for a gas of atoms. We also find that the rate of emission presents a strong dependence on the atom's position.
Spontaneous emission competes with stimulated emission in many interactions of light with matter. In the usual analyses which describe the interaction of an atom with a coherent optical field, the spontaneous emission characteristics, e.g., probability and spectral distribution, are not determined. The spontaneous emission from an atom which interacts with a coherent light wave is considered. The competition between coherent photons and spontaneous photons is treated in detail for a system consisting of a stationary atom, an open cavity and spatial fields. In the model chosen, a multilevel atom which spontaneously decays by interacting with spatial fields has two nondegenerate states coupled by an interaction with a single mode of the cavity. The Laplace-transformed Schrodinger equation is solved for specified initial conditions of the system. It is found that the interaction with the coherent field modifies the spectral distribution of spontaneous radiation from the atom. For spontaneous transitions involving an atomic state which interacts with the coherent field, the spectral distributions can no longer be described by Lorentzian functions. The new distributions exhibit a broadening and splitting for strong interactions between the atom and the coherent field. It is shown that the qualitative features of these distributions can be predicted from the energy-level diagram of the atom-cavity system. The net probability of the system gaining a coherent or cavity photon is calculated by integrating over the emitted spontaneous frequencies. The equivalence of this approach to the method of computing probabilities by integrating over time is demonstrated by using Parseval's theorem.
The dynamic evolution of atomic spontaneous emission in one-dimensional photonic crystals (1DPC) is investigated by using mode functions for the 1DPC. Our attention is focused on the non-Markovian processes in the first several optical cycles of the spontaneous emission decay. The integral-differential dynamic equation is directly solved by numerical calculation without using the Markovian approximation. The interference of the multireflected fields plays an important role in the non-Markovian processes. Due to the interference of the fields successive arrived at the atom due to the reflection at the interfaces, the decay rate shows a series of pulselike peaks. If the interference is constructive, the spontaneous decay is enhanced, while if the interference is destructive, the spontaneous decay is suppressed. The steady decay rate is approximately equal to the vacuum decay rate, when the atomic transition frequency corresponds to an allowed normal mode of the 1DPC. The spontaneous emission decay is suppressed if the atomic transition frequency is within the forbidden gap of the 1DPC.
A quantum theory of spontaneous emission from an initially excited two-level atom in a one-dimensional optical cavity with output coupling from both sides is developed. Orthonormal mode functions with a continuous spectrum are employed, which are derived by imposing a periodic boundary condition on the whole space with a period much larger than the cavity length. The delay differential equation of the atomic state of Cook and Milonni [Phys. Rev. A 35, 5081 (1987)] is re-derived in a strict manner, where the reflectivity of the cavity mirrors is included naturally in the mode functions. An approximate solution at a single-resonant-mode limit shows the results of ``vacuum'' Rabi oscillation in an underdamped cavity and enhanced spontaneous emission rate in an overdamped cavity. For the latter case, it is found that in the optical range the spontaneous emission rate is enhanced by a factor F (finesse of the cavity).