Journal of the Physical Society of Japan
Collision-Induced Two-Photon Absorption of Ultrashort Light Pulses
Kenji Torizuka, Norio Morita, Tatsuo Yajima
Abstract
The relation between the spectral character of a completely off-resonant two-photon absorption and the non-impact collision dynamics of a three-level atomic system is studied. A collisionally induced resonance character in the spectral dependence of the absorption probability is shown theoretically. Measured results about the dependence of fluorescence intensity on the incident light frequencies are ingood agreement with the theory. The interatomic potential between the sodium 4D state and argon is also estimated from experimental results.