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Physical Review A

Three-level atoms in phase-sensitive broadband correlated reservoirs

V. Buek, P. L. Knight, Igor K. Kudryavtsev

Published Aug 1, 1991• 64 citations
Publisher

Abstract

A three-level atom with two competing transitions can sense correlations between modes of an electromagnetic field with which it interacts. We examine the sensitivity of three-level atoms in ladder, \ensuremath{\Lambda}, and V configurations to correlations between modes in a broadband correlated reservoir of field modes. Our model of a correlated reservoir includes pairwise mode correlations around a center frequency. When such correlations are set to zero, the reservoir becomes a simple thermal heat bath, but in the opposite extreme when the modes are perfectly correlated, we recover a minimum-uncertainty broadband squeezed vacuum. We show that atomic populations are extremely sensitive to these correlations, and can, in the ladder system, become inverted as a result of the phase-sensitive noise. We also show how atomic population trapping is affected by mode correlations.

DOI
10.1103/physreva.44.1931

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Journal of Modern Optics•Mar 1, 1995•18 citations
A three-level atom with two competing transitions can sense correlations between modes of an electromagnetic field with which it interacts. We examine the sensitivity of three-level atoms in ladder, \ensuremath{\Lambda}, and V configurations to correlations between modes in a broadband correlated reservoir of field modes. Our model of a correlated reservoir includes pairwise mode correlations around a center frequency. When such correlations are set to zero, the reservoir becomes a simple thermal heat bath, but in the opposite extreme when the modes are perfectly correlated, we recover a minimum-uncertainty broadband squeezed vacuum. We show that atomic populations are extremely sensitive to these correlations, and can, in the ladder system, become inverted as a result of the phase-sensitive noise. We also show how atomic population trapping is affected by mode correlations.
We show that atoms interacting with a squeezed radiation field reservoir can exhibit phase-dependent population decay and relax into a highly correlated pure state, in striking difference to decay in a heat bath. We use a Heisenberg operator treatment of radiative transitions in a broadband squeezed light field described as a quantum white-noise field with correlated fluctuations to describe the modified decay of a single atom, and of two atoms cooperatively decaying in a squeezed vacuum. We compare this decay with that generated by a broadband thermal field which lacks the essential field-mode correlations characteristic of squeezing.
Using the formalism developed earlier, we treat spontaneous emission from a three-level atom (ladder system) interacting with a broadband squeezed vacuum field. We obtain expressions for the transient and steady-state populations of the atomic levels with the conditions that the atom interacts with either a multimode perfect squeezed vacuum field, or a three-dimensional vacuum field in which the squeezed modes lie within a solid angle over which squeezing is propagated. The results are compared with those obtained for the atom interacting with a thermal field. We show that in the perfect case the first excited state is not populated when the squeezed vacuum field is in a minimum-uncertainty squeezed state. Moreover, the second excited state can have a steady-state population larger than 1/2. These features are completely absent when the atom interacts with the thermal field. In addition, for a low-intensity squeezed vacuum field the population in the second excited state exhibits a linear rather than quadratic dependence on the intensity of the squeezed vacuum field. In the three-dimensional case the presence of unsqueezed modes considerably reduces the effect of squeezing on spontaneous emission. However, a significant reduction in a population of the first excited state and a population larger than 1/2 in the second excited state can be achieved provided the squeezing is propagated over a large solid angle. We also discuss the effect of the two-photon detuning between the double carrier frequency of the squeezing and atomic transition frequency ${\mathrm{\ensuremath{\omega}}}_{3}$ on the steady-state atomic population.
In this paper we investigate the sensitivity of coupled atomic transitions to correlations between field modes. In particular, we show that a three-level atom interacting with a cavity field supporting two quantized modes can be highly sensitive to the nature of the correlations between the modes. Correlated two-mode states include the two-mode squeezed state, whereas the SU(2) coherent state is an example of an anticorrelated state. We study in detail the dynamics of a three-level atom in the \ensuremath{\lambda} configuration, interacting with the two modes of an SU(2) coherent state. We show that for certain choices of the atom-field coupling constants, the generalized two-photon Rabi frequency for the system becomes independent of the photon number, leading to a purely periodic behavior in time of the atomic population probabilities; for other choices of the atom-field coupling constants, we observe the usual collapse and revival of the Rabi oscillations. We study also the dynamics of the field, in particular the correlations between the modes. Finally, for comparison purposes, we present a parallel study of the case in which the field modes are initially uncorrelated.
Light emitted from laser-driven atoms often has squeezed quadrature fluctuations reflecting the phase dependence of the atomic source excited into a coherent superposition by the driving field. In this paper, we study the maximum squeezing in the emitted light fields from three-level atoms, paying particular attention to the role of atomic coherences in governing the optimum squeezing which is possible. Some phase dependent nonlinear optical processes have the potential for substantial quantum noise reduction at useful intensities: for example, four-wave mixing involving atomic systems has already been used to generate quadrature-squeezed light. The threoretical description of such a source is generally complicated with damping processes, coherent and incoherent pumping, and so on, all needing to be taken into account. Fully quantum treatments are available, but the basic physics of the process is often difficult to grasp in the necessarily complicated analysis. Although less important from the point of view of efficient practical sources of squeezed light, studying the generation of squeezed light in simpler systems such as two- or three-level atoms interacting with one or two modes (as in Jaynes-Cummings models) or in spontaneous emission or resonance fluorescence gives greater insight into the fundamentals of the squeezing process. In particular, the relationship between the atomic coherences and the degree of squeezing in the generated fields can be explored. We study the maximum (optimized) squeezing that can be obtained in the emitted fields from the irreversible decay from three-level atoms for any choice of initial conditions, excitations and decay process, for all quadrature components and for all possible configurations (V, \ensuremath{\Lambda}, and ``ladder'' systems).We show that for V and \ensuremath{\Lambda} systems, optimum squeezing is actually associated with a two-level state (in a suitable basis) involving a single one-photon coherence, but for ladder systems the state for maximum noise reduction is not equivalent to a two-level system and involves a single two-photon coherence and no intermediate state population. We pay particular attention to whether the total field is in a minimum uncertainty state, and the nature of the atomic state associated with maximum squeezing, especially whether it is a mixed or pure state. In the case where the initial free field has a zero amplitude at the detector and the source atoms are confined to a region small compared to the wavelength (Dicke source) we show that the squeezing in the total field is given in terms of the squeezing in the source field, and hence related to atomic populations and atomic one-photon and two-photon coherences for the case of three level atom. Previously unconsidered source-free field interferences terms are shown to be zero. The choice of quadrature phase and frequency is optimized to minimize the source field normally ordered variance. We then minimize further with respect to the choice of atomic density matrix elements subject to the constraints that the density matrix is Hermitean, positive, and has a trace equal to unity. In all cases we find that the optimum squeezing is produced when the source field is in a minimum uncertainty state.
Master equation methods are used to investigate the effects of a broad-band squeezed vacuum on a three-level atom of the lambda configuration. The two-mode squeezed vacuum is treated as a Markovian reservoir in a non-stationary phase-dependent state. In addition to the squeezed vacuum the atom is driven by two coherent laser fields each of which, depending on the polarization, can couple to one or both of the atomic transitions. We show that in general the optical Bloch equations for the atomic density matrix elements have oscillatory coefficients, thereby necessitating the use of Floquet methods. For the case of equal laser frequencies, which are also equal to the carrier frequency of the squeezed vacuum, the coefficients of the Bloch equations become time independent and stationary solutions for the populations and coherences are obtained by standard matrix methods. For the ordinary vacuum the usual coherent population trapping effect at two-photon resonance is obtained, with the upper state population being zero. An unsqueezed thermal field partially destroys the trapping effect as the upper state population is no longer zero at two-photon resonance. The squeezed vacuum has the effect of improving the trapping in that the coherence hole becomes more pronounced for some values of the relative phase between the squeezed vacuum and the driving fields. The additional effects of a coherence transfer rate between the two optical coherences, which occurs for special choices of angular momentum quantum numbers are also studied. For the case of equal laser frequencies, the inclusion of this coherence transfer process destroys population trapping and reduces the lambda system to a two-level system. However, for the case of unequal laser frequencies, the coherence transfer process in combination with the squeezed vacuum can restore to some extent the population trapping. We show that other features that do not occur for two-level atoms, such as stationary population inversions between pairs of the atomic levels, also depend on the relative phase and can be enhanced in the squeezed vacuum. In the case of unequal frequencies of the driving fields the population in the upper state depends on the relative phase only when the carrier frequency of the squeezed vacuum is equal to one of the two frequencies of the driving fields. When the carrier frequency of the squeezed vacuum is slightly detuned from both frequencies of the driving fields, the population in the upper state is insensitive to the relative phase but is dependent on the degree of squeezing. For large detunings, the population does not show any dependence on the degree of squeezing and its distribution in function of the two-photon detuning is similar to that in the thermal vacuum field.