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Journal of the Optical Society of America B

A general theory of two-wave mixing in nonlinear media

Mingjun Chi, Jean‐Pierre Huignard, Paul Michael Petersen

Published Jul 14, 2009• 29 citations
Publisher

Abstract

A general theory of two-wave mixing (TWM) in nonlinear media is presented. Assuming a gain (or absorption) grating and a refractive index grating are generated because of the nonlinear process in a nonlinear medium, the coupled-wave equations of TWM are derived based on Maxwell's wave equation. The coupled-wave equations can be decoupled as coupled equations for the intensity and coupled equations for the phase of both beams, and these two sets of coupled equations can be solved analytically by using average total intensity in the medium instead of using the total intensity. Compared with the previous theory of TWM, the theory presented here is more general, and the applications of the theory to photorefractive materials, Kerr media, and semiconductor broad-area amplifiers are described.

DOI
10.1364/josab.26.001578

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A general theory of two-wave mixing (TWM) in nonlinear media is presented. Assuming a gain (or absorption) grating and a refractive index grating are generated because of the nonlinear process in a nonlinear medium, the coupled-wave equations of TWM are derived based on Maxwell's wave equation. The coupled-wave equations can be decoupled as coupled equations for the intensity and coupled equations for the phase of both beams, and these two sets of coupled equations can be solved analytically by using average total intensity in the medium instead of using the total intensity. Compared with the previous theory of TWM, the theory presented here is more general, and the applications of the theory to photorefractive materials, Kerr media, and semiconductor broad-area amplifiers are described.
The solution of the nondegenerate two-wave-mixing problem in an absorptive Kerr medium including the contribution from nonlinear absorption is obtained for the first time to our knowledge. This solution enables us to analyze the influence of nonlinear absorption on the two-wave-mixing gain and account for previously unexplained results reported for ruby and Cr3+:YAlO3. The effect of nonlinear absorption of a pump beam on the gain of a probe beam is shown to be minimized when incident intensities of the interacting beams are equal. The intensity dependence of the two-wave-mixing gain for dispersive (ruby and Cr3+:YAlO3) media and the gain measurements for absorptive (fluorescein-doped glass) media are also in agreement with the new theory.
The theory of probe beam amplification via degenerate optical wave mixing in a Kerr medium is presented. This theory includes consideration of the self-phase modulation, two-wave mixing, and multiwave mixing terms in the coupled-wave equations. Both analytical solutions, under the assumptions of a nondepleted pump beam and a transparent Kerr medium, and numerical solutions with these assumptions removed are presented. Our solutions show that under certain conditions, phase matching can be satisfied and a high probe beam gain is possible, even for a zero phase shift between the refractive index and the intensity gratings.
Nonlinear optics normally involves the change in the susceptibility of a material due to the presence of optical radiation. In many cases, the light-matter interaction produces a change in the refractive index of the medium, as occurs in photorefractive media, as well as in Kerr-like media, Brillouin-active media and absorbing media with thermallyinduced refractive index changes. Such nonlinear refractive index variation corresponds to a change in the real part of the optical susceptibility %. In resonant materials, the optical radiation induces stimulated emission (or absorption) causing transfer of population between different energy states of the medium. This can lead to saturation of the amplification (or absorption) corresponding to changes in the imaginary part of the susceptibility x= i2odk where the amplitude gain coefficient a(I) is a saturable function of the intensity /, and k is the magnitude of the wavevector of the optical radiation. The interference of two (or more) coherent beams I(x) in the laser amplifier can cause a modulation of the population inversion N(x). This modulation of the inversion is commonly known as spatial hole burning in lasers and leads to formation of a gain-grating a(x) = 1/2GN(X) where G is the stimulated emission cross-section. The gain grating can act as a very efficient diffractive optical element exhibiting high diffraction efficiency that may be even greater than unity [16] and also very high phase conjugate reflectivity using four-wave mixing (FWM) geometries [5-7].
In conclusion, the TWM in broad-area semiconductor amplifier in nondegenerate condition is investigated theoretically. The coupled-wave equations are derived and analytical solutions are obtained when the intensity of the pump is much larger than that of the signal, but much less than the saturation intensity of the amplifier. A special case of TWM, degenerate TWM, is investigated experimentally in a GaAlAs broad-area semiconductor amplifier. The experimental results show good agreement with the theory, and the validity of the theory for this experiment is discussed. A diffusion length of 2.0 m is determined from the experiment. The TWM gain in broad-area semiconductor amplifier is calculated as a function of the frequency difference between the pump and the signal based on the data obtained from the degenerate TWM experiment; and the calculated results are discussed based on the different contributions from the refractive index grating and the gain grating to the TWM gain. Depending on and , the TWM gain in semiconductor broad-area amplifier can be positive or negative. The energy exchange between the pump and signal beams occurs when 0.