Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Journal of Physics B Atomic Molecular and Optical Physics

Spectral hole-burning in pump–probe studies of nonlinear selective reflection spectroscopy

Yanting Zhao, Jie Ma, Lirong Wang, Jianming Zhao, Liantuan Xiao, Suotang Jia

Published Aug 9, 2005• 4 citations
Publisher

Abstract

Special hole-burning effects on the spectrum of gas atoms near a glass–vapour interface were obtained by observing the reflection of a weak probe beam. Sub-Doppler reflection spectroscopy has been achieved and the unabsorption dip was measured for different pump laser power and detuning. The nonlinear optical properties of the atomic system were investigated by taking into account the collisions between the atoms and the walls of the cell. We also demonstrated the absorption reduction in a V-type energy level configuration with a linewidth of about 6.5 MHz. The experimental results agree with reasonable accuracy with the predictions derived from a theoretical explanation of the nonlinear optical susceptibility.

DOI
10.1088/0953-4075/38/16/014

Related papers

Nonlinear selective reflection in cascade three-level atomic systems

F. Schuller, O. Gorceix, M. Ducloy

We study the cascade three-level selective-reflection spectroscopy for normal incidence at a dielectric--atomic-vapor interface in a pump-probe scheme. Taking into account the effects of spatial dispersion arising from deexcitation by collisions with the interface and the transient response of atoms leaving the surface, we evaluate the modification of the probe-field reflection induced by the presence of the pump field in terms of a nonlocal nonlinear susceptibility. The dependence of this susceptibility on the probe frequency for various given pump frequencies is calculated. Sub-Doppler structures in the selective reflection spectrum are obtained and analyzed. Potential applications to the study of the interaction of highly excited atomic states with the surface are indicated.

Physical Review A•Jan 1, 1993•38 citations

Nonlinear Doppler-free spectroscopy of atoms near a surface

Pierre Simoneau, S. Le Boiteux, C. De Araujo +2 more

Up to now, Doppler-free nonlinear spectroscopy has been applied to atoms inside a gas medium (volume spectroscopy). We have extended these methods to atoms in the vicinity of a surface. The basic principle consists of monitoring reflectivity changes produced when a laser beam, incident on a glass–vapor interface, is brought into resonance with an atomic transition. For Doppler-free spectroscopy, two counterpropagating beams are used to operate velocity selection. If these two beams are under normal incidence in the glass—velocity selection perpendicular to the surface—one observes saturated dispersion (selective reflection sensitive to the real index). For incidence angles in the glass (prism) larger than the critical angle (total internal reflection), a standing evanescent wave is produced in the gas (velocity selection along the surface), and saturated absorption is detected. Experimental demonstration was performed on the Na resonance line; high sensitivity (10−4 relative reflectivity change) and spectral resolution as good as 20 MHz were obtained. The main limitation to better resolution comes from the short atomic transit time in the evanescent wave (typical extension ~λ). Relevant applications of these techniques should also concern the diagnostics of optically thick media, as analysis of interaction between gas-phase atoms and the surface, notably atom–wall collisions, and modification of the spontaneous emission characteristics.

International Laser Science Conference•Jan 1, 1986•0 citations

Three-level nonlinear selective reflection at a glass–Cs-vapor interface

Anne Amy‐Klein, Solomon M. Saltiel, O. A. Rabi +1 more

We present an experimental study of nonlinear selective reflection at a dielectric--Cs-vapor interface, in a three-level cascade-up scheme. The nonlinear reflection at the Cs ${\mathit{D}}_{2}$ resonance line is monitored in the presence of resonant irradiation at 621 nm or 658 nm (6${\mathit{P}}_{3/2}$\ensuremath{\rightarrow}8${\mathit{D}}_{5/2}$,9${\mathit{S}}_{1/2}$). Experimental reflection spectra with either counterpropagating or copropagating light beams are analyzed and compared with the theoretical predictions of F. Schuller et al. [Phys. Rev. A 47, 519 (1993)]. For a blue-detuned pump and copropagating geometry an alternative type of three-level coherent reflection resonances, specifically associated with desorbing atoms, is observed. Also observed is the nonlinear reflection associated with the off-resonant, two-photon dispersion of atoms moving parallel to the window surface. Probe beam saturation is responsible for the appearance of additional resonant features in reflection spectra. Finally we analyze crossover spectral resonances which arise from nondegenerate, four-wave-mixing processes induced by the combined influence of counterpropagating pump and probe beams, and the pump beam being partially reflected by the window.

Physical Review A•Oct 1, 1995•13 citations

Nonlinear selective reflection spectroscopy of V‐type atomic system at the gas‐solid interface

Tengfei Meng, Zhonghua Ji, Dianqiang Su +3 more

We theoretically present the nonlinear selective reflection spectroscopy of V‐type atomic system at gas‐solid interface in a pump‐probe scheme. The saturation and coherence effects are distinguished by solving Liouville equation in the absence and presence of reduced density matrix element between the two excited levels. When the coherence effect exists, two peaks appear in reflection spectroscopy with asymmetry lineshape. We investigate the dependence of reflection spectroscopy on pump field intensity, frequency detuning and coherent decay rate induced by collision between atoms. The lineshape can be explained based on reflection spectroscopy contributed from atoms with negative (before collision) and positive (after collision) velocities, single‐photon and two‐photon processes. This study is helpful for investigating quantum coherence and dynamic processes of atoms at gas‐solid interface.

arXiv:1503.04950•Annalen der Physik•Feb 11, 2016•3 citations

Doppler-free spectroscopy at a glass-vapour interface by saturated selective reflection at near normal incidence

S. Le Boiteux, Pierre Simoneau, Daniel Bloch +1 more

Doppler-free spectra of gas phase atoms near a glass-vapour interface are obtained by monitoring the reflection of a probe beam-instead of its transmission-in three-level saturation spectroscopy. Experiments performed on the 3S-3P-4D cascade system of Na have allowed the authors to monitor two-photon-induced saturated dispersion of Na atoms.

Journal of Physics B Atomic and Molecular Physics•Mar 14, 1987•22 citations

Excitation dependence of resonance line self-broadening at different atomic densities

Hebin Li, Vladimir A. Sautenkov, Yuri V. Rostovtsev +1 more

We study the dipole–dipole spectral broadening of a resonance line at high atomic densities when the self-broadening dominates. The selective reflection spectrum of a weak probe beam from the interface of the cell window and rubidium vapour is recorded in the presence of a far-detuned pump beam. The excitation due to the pump reduces the self-broadening. We found that the self-broadening reduction dependence on the pump power is atomic density independent. These results provide experimental evidence for the disordered exciton based theory of self-broadening, and can be useful for the description of the interaction of a strong optical field with a dense resonance medium.

arXiv:0811.0575•Journal of Physics B Atomic Molecular and Optical Physics•Mar 9, 2009•39 citations
Special hole-burning effects on the spectrum of gas atoms near a glass–vapour interface were obtained by observing the reflection of a weak probe beam. Sub-Doppler reflection spectroscopy has been achieved and the unabsorption dip was measured for different pump laser power and detuning. The nonlinear optical properties of the atomic system were investigated by taking into account the collisions between the atoms and the walls of the cell. We also demonstrated the absorption reduction in a V-type energy level configuration with a linewidth of about 6.5 MHz. The experimental results agree with reasonable accuracy with the predictions derived from a theoretical explanation of the nonlinear optical susceptibility.
We study the cascade three-level selective-reflection spectroscopy for normal incidence at a dielectric--atomic-vapor interface in a pump-probe scheme. Taking into account the effects of spatial dispersion arising from deexcitation by collisions with the interface and the transient response of atoms leaving the surface, we evaluate the modification of the probe-field reflection induced by the presence of the pump field in terms of a nonlocal nonlinear susceptibility. The dependence of this susceptibility on the probe frequency for various given pump frequencies is calculated. Sub-Doppler structures in the selective reflection spectrum are obtained and analyzed. Potential applications to the study of the interaction of highly excited atomic states with the surface are indicated.
Up to now, Doppler-free nonlinear spectroscopy has been applied to atoms inside a gas medium (volume spectroscopy). We have extended these methods to atoms in the vicinity of a surface. The basic principle consists of monitoring reflectivity changes produced when a laser beam, incident on a glass–vapor interface, is brought into resonance with an atomic transition. For Doppler-free spectroscopy, two counterpropagating beams are used to operate velocity selection. If these two beams are under normal incidence in the glass—velocity selection perpendicular to the surface—one observes saturated dispersion (selective reflection sensitive to the real index). For incidence angles in the glass (prism) larger than the critical angle (total internal reflection), a standing evanescent wave is produced in the gas (velocity selection along the surface), and saturated absorption is detected. Experimental demonstration was performed on the Na resonance line; high sensitivity (10−4 relative reflectivity change) and spectral resolution as good as 20 MHz were obtained. The main limitation to better resolution comes from the short atomic transit time in the evanescent wave (typical extension ~λ). Relevant applications of these techniques should also concern the diagnostics of optically thick media, as analysis of interaction between gas-phase atoms and the surface, notably atom–wall collisions, and modification of the spontaneous emission characteristics.
We present an experimental study of nonlinear selective reflection at a dielectric--Cs-vapor interface, in a three-level cascade-up scheme. The nonlinear reflection at the Cs D2{\mathit{D}}_{2}D2​ resonance line is monitored in the presence of resonant irradiation at 621 nm or 658 nm (6P3/2{\mathit{P}}_{3/2}P3/2​\ensuremath{\rightarrow}8D5/2{\mathit{D}}_{5/2}D5/2​,9S1/2{\mathit{S}}_{1/2}S1/2​). Experimental reflection spectra with either counterpropagating or copropagating light beams are analyzed and compared with the theoretical predictions of F. Schuller et al. [Phys. Rev. A 47, 519 (1993)]. For a blue-detuned pump and copropagating geometry an alternative type of three-level coherent reflection resonances, specifically associated with desorbing atoms, is observed. Also observed is the nonlinear reflection associated with the off-resonant, two-photon dispersion of atoms moving parallel to the window surface. Probe beam saturation is responsible for the appearance of additional resonant features in reflection spectra. Finally we analyze crossover spectral resonances which arise from nondegenerate, four-wave-mixing processes induced by the combined influence of counterpropagating pump and probe beams, and the pump beam being partially reflected by the window.
We theoretically present the nonlinear selective reflection spectroscopy of V‐type atomic system at gas‐solid interface in a pump‐probe scheme. The saturation and coherence effects are distinguished by solving Liouville equation in the absence and presence of reduced density matrix element between the two excited levels. When the coherence effect exists, two peaks appear in reflection spectroscopy with asymmetry lineshape. We investigate the dependence of reflection spectroscopy on pump field intensity, frequency detuning and coherent decay rate induced by collision between atoms. The lineshape can be explained based on reflection spectroscopy contributed from atoms with negative (before collision) and positive (after collision) velocities, single‐photon and two‐photon processes. This study is helpful for investigating quantum coherence and dynamic processes of atoms at gas‐solid interface.
We study the dipole–dipole spectral broadening of a resonance line at high atomic densities when the self-broadening dominates. The selective reflection spectrum of a weak probe beam from the interface of the cell window and rubidium vapour is recorded in the presence of a far-detuned pump beam. The excitation due to the pump reduces the self-broadening. We found that the self-broadening reduction dependence on the pump power is atomic density independent. These results provide experimental evidence for the disordered exciton based theory of self-broadening, and can be useful for the description of the interaction of a strong optical field with a dense resonance medium.