The frequency of the multimode instabilities recently observed on a passive cavity filled with 2-level molecules is compared to that given by a very simple model of side-mode gain.
We report the observation of an instability in a bistable optical system with a homogeneously broadened two-level medium involving the onset of the cavity side mode that is two modes away from the source frequency and three modes away from the molecular resonance frequency. These measurements extend the range of a recent report [Phys. Rev. A 39, 703 (1989)] of observations of the multimode instability in optical bistability predicted by Lugiato and Bonifacio [Lett. Nuovo Cimento 21, 505 (1978); 21, 510 (1978)], with the key difference being that the experimental observations in the previous report were limited to instabilities of the side mode adjacent to the source frequency.
We have recently observed a sinewave self-pulsing in the beam transmitted by a passive cavity containing 2-level molecules, driven by a continuous wave. In this experiment made at a wavelength λ ≅ 3.5 mm, the intracavity Rabi frequency is comparable to the free spectral range ( 830 kHz ) of the very long cavity used (l =182 m) {1} and much larger than the collisional linewidth (≅ 25 kHz) .The medium is then strongly saturated by the driving field ( saturation parameter > 1000) so that its absorption , heavy in the linear regime (αl > 100), is in fact quite moderate. We claim that the self-pulsing observed in these conditions is the first experimental evidence of the multimode instability, predicted a long time ago by Bonifacio and Lugiato {2} but not yet observed. This instability is the multimode counterpart of the single mode instability, recently observed by Orozco et al {3}.