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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Velocity-selective optical pumping and interference oscillations in the absorption of Rb atoms in a weak magnetic field

Igor M. Beterov, A. Dudnikov, Vasily M. Entin, I. I. Ryabtsev

Published Oct 21, 1998• 0 citations
Publisher

Abstract

The experiments on transient phenomena in pulsed optical orientation of Rb atoms by the emissions of semiconductor lasers are presented. With using probe field method it was found that macroscopic magnetic momentum induced by strong pulsed laser field is processing in weak magnetic field causing Larmor oscillations of the absorption coefficient of probe field. The same effect was observed at fast changing of direction of the magnetic field.

DOI
10.1117/12.328274

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The experiments on transient phenomena in pulsed optical orientation of Rb atoms by the emissions of semiconductor lasers are presented. With using probe field method it was found that macroscopic magnetic momentum induced by strong pulsed laser field is processing in weak magnetic field causing Larmor oscillations of the absorption coefficient of probe field. The same effect was observed at fast changing of direction of the magnetic field.
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Abstract We report experimental studies of electro magnetically induced transparency and enhancement of third‐order optical nonlinearities in A‐type atomic systems realized in 87Rb atoms cooled and confined in a magneto‐optical trap. We observed complete transparency of a weak probe laser in the A type Rb system with a moderate coupling field. With a third pump laser tuned to a fourth atomic state, the atomic system exhibits the interference‐enhanced third‐order susceptibility and only absorbs two photons, but not one photon. Our experiment demonstrates large nonlinear absorption of the weak probe laser, from which greatly enhanced Kerr nonlinearity in the Rb system is inferred.
Abstract The quantum dynamics of a system of Rb atoms, modeled by a V -type three-level system interacting with intense probe and pump pulses, are studied. The time-delay-dependent transient-absorption spectrum of an intense probe pulse is thus predicted, simulating pump-probe experiments in which this is preceded or followed by a strong pump pulse. Numerical results are interpreted in terms of an analytical model based on interaction operators , which quantify the transformation undergone by the system under the action of an intense pulse. The oscillating features of the resulting transient-absorption spectra, due to the coupling of several excited states, are thus interpreted in terms of the atomic population and phase changes imposed by the pump and probe pulses. Strong-field-induced phases and their influence on the resulting transient-absorption spectra are thereby investigated for different values of pump and probe intensities and frequencies, focusing on the atomic properties which are encoded in the absorption line shapes for positive and negative time delays.
This article reviews the early investigations of Series on the resonance absorption and fluorescence of light by samples of oriented atoms dagger subjected to static and oscillatory magnetic fields. These investigations include experiments on optical-radiofrequency double resonance, light beats in double resonance, circulation of coherence in optical pumping, and time-biasing in level-crossing spectroscopy. It then describes some selected laser spectroscopy experiments involving the interaction of optically oriented atoms with static magnetic fields that were stimulated by the earlier work of Series, including experiments on hyperfine structure quantum beats, cascade quantum beats, ground-state quantum beats in transmission, and optogalvanic detection of atomic coherences. Finally, it describes some current work which uses static magnetic fields to manipulate the external variables (momentum and position) of laser-cooled oriented atoms, with applications in the rapidly developing field of atom optics and atom interferometry.
We have experimentally and theoretically investigated the behavior of Na atoms under the combined influence of resonant laser light and a magnetic field. Linearly polarized light was tuned to the (3s) 2{\mathrm{}}^{2}2S1/2{S}_{1/2}S1/2​ (F=2)\ensuremath{\rightarrow}(3p) 2{\mathrm{}}^{2}2P1/2{P}_{1/2}P1/2​ (F'=1) component of the D1{D}_{1}D1​ line. The intensity of fluorescent light was observed as a function of the laser intensity for various strengths of the magnetic field B. Trapping in the MF{M}_{F}MF​=\ifmmode\pm\else\textpm\fi{}2 levels of the ground state could be observed to be of decreasing importance for an increasing component of B perpendicular to the laser polarization \ensuremath{\epsilon}^. For laser intensities increasing beyond certain critical values, however, the fluorescence decreased and trapping seemed to become again important. For a quantitative explanation of the observed behavior we describe the system by generalized rate equations for the density matrix. We find that stimulated absorption and emission processes effectively inhibit the Larmor precession, thereby enforcing the trapping effect. Precession can only take place at sufficiently low light intensities.