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Physics Letters A

Raman coupling between dressed states in resonant multiphoton ionization

Piers Coleman, P. L. Knight

Published Feb 1, 1981• 9 citations
Publisher
DOI
10.1016/0375-9601(81)90095-5

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Abstract Resonance‐enhanced multiphoton ionization (REMPI) in potassium atom is investigated within the strong coupling regime using photoelectron momentum imaging techniques. The kinetic energy distribution of the ionized electrons reveals the eigenenergies of the dressed states, which exhibit Autler–Townes (AT) splitting. This splitting is proportional to the laser field strength. Partial wave analysis of the photoelectrons angular distributions (PAD) uncovers relative phase shifts between the dressed states, shedding light on attosecond ionization time delays. The observed phase shift between the two electron wave packets by the AT splitting arises from the combined effects of the Coulomb phase and the quantum defect phase.
The resonance enhancements marking the ATI spectrum of argon are discussed in the light of a recently compiled map of the quasienergies of this atom. Many of the dressed excited states of interest shift nonponderomotively in complicated ways, but keep an ionization width narrow enough to produce sharp substructures of both low and high ATI peaks through Stark-shift induced resonances. The most prominent enhancement observed in the high-order ATI peaks originates from ionization from the dressed ground state perturbed by the influence of neighbouring resonant dressed states.