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Journal of the Physical Society of Japan

Dynamics of Five-Level Atoms in Two Standing Electromagnetic Waves

Soo Chang, B. M. Garraway, Vladimir G. Minogin

Published Sep 15, 1990• 3 citations
Publisher

Abstract

We examine the dynamics of five-level atoms interacting with two standing waves. In our approach we describe the motion of the atoms by a Fokker-Planck equation, including the effect of velocity-dependent two-photon Raman processes within the second order rate equation approximation. By using this procedure we numerically calculate the cooled temperatures of sodium atoms. We then find two principal types of behaviour; that of two-level and three-level atomic systems. We are also able to find detunings of the standing waves for which the atoms are cooled to temperatures below the “Doppler limit”.

DOI
10.1143/jpsj.59.3155

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Annual Meeting Optical Society of America•Jan 1, 1990•0 citations
We examine the dynamics of five-level atoms interacting with two standing waves. In our approach we describe the motion of the atoms by a Fokker-Planck equation, including the effect of velocity-dependent two-photon Raman processes within the second order rate equation approximation. By using this procedure we numerically calculate the cooled temperatures of sodium atoms. We then find two principal types of behaviour; that of two-level and three-level atomic systems. We are also able to find detunings of the standing waves for which the atoms are cooled to temperatures below the “Doppler limit”.
We examine the laser cooling of three-level (Lambda) -atoms in the field of two standing waves when frequency detunings are considerably greater than natural width of the excited state as well as the Rabi frequencies in the system. It is shown that at the difference of frequency detunings is small when compared to the Rabi frequencies sub-Doppler cooling of the (Lambda) -atom is possible. We present the dependence of the light pressure force on the atoms velocity and dependence of cooled atoms temperature on the parameters of the exciting waves.
A theory of deep laser cooling of atoms by counterpropagating circular polarized laser waves in multilevel interaction schemes is developed. Using a (3+5)-level atom as an example, we show that in multilevel interaction schemes two-photon processes are responsible for creating a narrow structure near zero velocity in the ground-state atomic coherence. This structure is in turn responsible for narrow velocity structures in atomic populations and optical coherences. A Fokker-Planck-type kinetic equation is derived for a model of a (3+5)-level interaction scheme. It is found that two-photon coherent processes considerably enhance the radiation force at low velocities and the friction produced by the force at a negative detuning, and considerably decrease the diffusion coefficient. Two-photon processes in multilevel interaction schemes are identified as the basic physical mechanism responsible for deep laser cooling of atoms. The temperature of laser-cooled atoms is derived for a model (3+5)-level atom, and found to be in good agreement with the experimentally observed temperature for laser-cooled cesium atoms.
We theoretically investigated the transverse and longitudinal velocity fluctuations of initially cooled Cs atoms below (or close to) the Doppler limit as the atoms were slowly accelerated in a travelling plane electromagnetic wave. We first derived a kinetic equation describing the atomic motion in the first order rate equation approximation and then numerically solved the equation. Increase or decrease in the longitudinal fluctuation was shown to depend upon the initial atom temperature and the detuning, while the tranverse fluctuation routinely increased with interaction time.
We report computational results for the time evolution of the velocity distribution P(V,t) for two-level and multilevel ``Doppler'' laser cooling. We compare results obtained from the semiclassical (SC) Fokker-Planck equation and from generalized optical Bloch equations applied to density matrices over a basis of products of internal and quantized translational states (QDM). Computer memory requirements are optimized to make large-scale QDM calculations feasible. QDM and SC agree well except for two cases: (a) atoms in the wells of the light-shift potential (with kinetic energy less than the well depth, U0{\mathit{U}}_{0}U0​), and (b) atoms with recoil energy ER{\mathit{E}}_{\mathit{R}}ER​ comparable to or greater than the natural linewidth \ensuremath{\Elzxh}\ensuremath{\Gamma}. Transient dips occur in P(V,t) at V=0 in QDM results due to slow cooling of atoms in the light-shift potential wells. Dips in P(V,t) occur at velocity-tuned-resonance (Doppleron) velocities but disappear over long interaction times as atoms accumulate near points where the force is zero. When ER{\mathit{E}}_{\mathit{R}}ER​\ensuremath{\approxeq}\ensuremath{\Elzxh}\ensuremath{\Gamma}, sharp peaks occur in P(V,T) at V=\ifmmode\pm\else\textpm\fi{}VR{\mathit{V}}_{\mathit{R}}VR​ from velocity-selective population quasitrapping not previously found in a two-level transition. Sharp features in P(V,t) occur also for J\ensuremath{\rightarrow}J+1 transitions with J>0, small U0{\mathit{U}}_{0}U0​/ER{\mathit{E}}_{\mathit{R}}ER​, and sufficiently large detuning, from transitions between individual quantum states in the periodic potential.
We present a general theoretical description of laser cooling of three-level atoms in a Λ configuration in two standing waves. Detunings, intensity, and spatial phase difference of the two waves are arbitrary. We demonstrate that, for a zero spatial phase shift, sub-Doppler cooling requires equal detunings. The basic mechanism is then coherent population trapping. For different detunings sub-Doppler cooling occurs only when the spatial phases of the two standing waves are different. This effect can be traced back to a mechanism of the Sisyphus type. These schemes of sub-Doppler cooling require neither polarization gradients nor magnetic fields.
In the limit of asymptotically small photon momentum, a Fokker–Planck equation for the center-of-mass Wigner function suffices to describe laser cooling of an atom. We have devised a procedure to compute the light pressure force and the diffusion tensor for an atom with an arbitrary level structure, traveling with an arbitrary velocity in any given three-dimensional light field. The scheme is based on solving a set of differential equations closely related to the density matrix equations of motion encountered in conventional recoilless laser spectroscopy. Computer programs have been written that automatically construct and solve the required equations from broad specifications of the problem, such as energies and angular momenta of the atomic levels. A Langevin equation stochastic simulation has been implemented to solve the Fokker-Planck equation of laser cooling using the computed force and diffusion. Comparisons of optical-molasses experiments and simulations carried out for a model sodium atom with a J = 2→J = 3 transition show qualitative similarities such as sub-Doppler limit temperatures, but the quantitative agreement of theory and experiment is not satisfactory.