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Physical Review A

Transient coherence oscillation induced by a detuned Raman field in a rubidium Λ system

Sung Jong Park, Hyuck Cho, Taeg Yong Kwon, Ho Seong Lee

Published Feb 17, 2004• 35 citations
Publisher

Abstract

The temporal evolution of coherent population trapping (CPT) was observed in rubidium atomic vapor when sudden changes were made to the detuning of a weak Raman field. The subsequent creation and destruction of CPT are caused by the temporal oscillations of optically induced Raman coherence, with their period depending on the Raman detuning. The oscillating signal was observed over a time of order of tens of milliseconds, and the dependence of the relaxation time on the cell temperature and laser power were investigated. The main features of the experimental observations were well explained by the time-dependent density-matrix equations.

DOI
10.1103/physreva.69.023806

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•Mar 23, 2001•0 citations
The temporal evolution of coherent population trapping (CPT) was observed in rubidium atomic vapor when sudden changes were made to the detuning of a weak Raman field. The subsequent creation and destruction of CPT are caused by the temporal oscillations of optically induced Raman coherence, with their period depending on the Raman detuning. The oscillating signal was observed over a time of order of tens of milliseconds, and the dependence of the relaxation time on the cell temperature and laser power were investigated. The main features of the experimental observations were well explained by the time-dependent density-matrix equations.
Coherent population trapping (CPT) oscillation is a transient oscillation phenomenon based on the CPT effect, which is related to the Raman detuning of the coherent bichromatic laser fields from the hyperfine ground-states of three-level Λ system. In this work, sawtooth wave is adopted to modulate the frequency of microwave signal to make Raman detuning change uniformly and stepping. Meanwhile, by building the relationship between the microwave frequency modulation rate and the change rate of Raman detuning, the effects of the change rate and mode of Raman detuning on CPT oscillation are analyzed respectively. The results reveal that when the Raman detuning changes uniformly, the CPT oscillation will occur on condition that the change rate is high enough, and the excited oscillations show non-harmonic oscillation behavior. When the Raman detuning is triggered off by step change, the excited CPT oscillation is a damping oscillation, and the oscillation frequency is equal to the frequency of Raman detuning. The modulation of Raman detuning is realized by using sawtooth wave to modulate the microwave frequency, and then the complete establishment of CPT state and the complete attenuation of CPT oscillation process are achieved. This work presents a new modulation method to realize the CPT oscillation, which shows great application potential in the field of weak magnetic measurements and atomic clocks.
We observe the transient evolution of the laser pumped magnetic resonance in a paraffin-coated rubidium vapor cell and analyze the phenomena numerically by using the four-level density matrix. With the increased radio frequency (RF) sweep rate, the traditional Lorentz signal turns to an asymmetric shape at low sweep rate and starts to oscillate at a high sweep rate. The transient oscillation's features, including frequency and the decay time, are studied by suddenly turning on the RF field to the resonance Larmor precession frequency under the different RF field and light field parameters. The experimental result reveals the transient signals' strong dependence on the RF field power and light power. Especially, the transient oscillation frequency primarily depends on the RF field's power and whatever power the laser light is. When the laser power is lower, the transient oscillation frequency is proportional to the RF field's amplitude. These transient evolution signals are also confirmed with the numerical calculations based on the density-matrix equation of motion.
Coherent population trapping (CPT) resonance formation is modeled numerically in a three-level Λ -system with one of the near-resonance fields being frequency-modulated. The model is based on density matrix equations in RW approximation with atomic relaxation properly taken into account. Slow modulation is shown to be equivalent to CW excitation with the frequency changed point by point. As the modulation period approaches the relaxation times, the delayed response of the system is shown to cause the CPT resonance shift and reshaping, as well as the appearance of transient oscillations of the energy level populations.
We investigated the existence of coherent population trapping (CPT) as a transient effect dependent on the rate of change of interaction parameters between an atom and light waves. For that purpose we exploited the phase dependence of CPT in a closed double-\ensuremath{\Lambda} interaction scheme, varying the total phase of the atomic transition loop linearly in time by detuning the light waves from exact four-photon resonance. For a slowly changing phase (that is, for small detunings) we observed the subsequent creation and destruction of CPT depending on the varying phase, while for higher speed of phase change CPT disappears. An analytical solution for a special case for a double-\ensuremath{\Lambda} interaction scheme that can be used to understand the principles of this phenomenon is presented. A qualitative comparison with our experiment shows good agreement within the limits of our theoretical considerations, confirming the validity of the basic idea. \textcopyright{} 1996 The American Physical Society.
Raman pulse atom interferometry is an important modality for precision measurements of inertial forces and tests of fundamental physics. Typical Raman atom optics use two coherent laser fields applied at gigahertz-scale detunings from optical resonance, so that spontaneous emission produces a minor or negligible source of decoherence. An additional consequence of spontaneous emission is coherent population trapping (CPT). We show that CPT produces coherences and population differences which induce systematic effects in Raman pulse atom interferometers. We do not believe that CPT has been previously identified as an error mechanism in Raman pulse atom interferometry. We present an experimental characterization of CPT coherences and population differences induced in laser-cooled cesium atoms by application of Raman pulses at detunings near 1 GHz, commensurate with detunings used in several precision measurement experiments. We are not aware of previous demonstrations of CPT-induced population difference. We argue that CPT effects could induce phase shifts of several milliradians in magnitude for typical experimental parameters and stipulate that these errors can be suppressed by propagation direction reversal in Raman interferometer-based precision measurements.
We study the features of spatial and temporal evolution of two powerful short different-wavelength laser pulses interacting with optical dense three-level Lambda-type medium under condition of coherent population trapping for the general case of unequal transition oscillator strengths. The pulses are simultaneously sent into an atom. The durations of probe and coupling pulses T1,2T_{1,2}T1,2​ (T2>T1T_2>T_1T2​>T1​) are supposed to be shorter than all relaxation times in the medium. We present analytical and numerical solutions of the self-consistent set of coupled Schr\\"{o}dinger equations and reduced wave equations in adiabatic limit with taking into account the first non-adiabatic correction. The adiabaticity criterion with account of pulse propagation is studied. We find that propagation dynamics depends on the relationship between the transition oscillator strengths. It is shown that at the initial stage of propagation the envelopes of the pulses slightly change along the length of the medium. This distance can be large compared to one-photon resonant absorption length of the medium. Also it is possible a regime of complete reemitting of the probe pulse into the coupling one during propagation. A spatial evolution of the atomic Raman coherence is investigated in detail too.