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Optics Communications

Laser cooling of Er3+-doped solids

Galina A. Nemova, Raman Kashyap

Published May 28, 2010• 8 citations
Publisher
DOI
10.1016/j.optcom.2010.05.015

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Journal of the Optical Society of America B•Mar 13, 2013•18 citations
A strongly focused laser beam with high power density employed in optical tweezers typically results in photothermal damage and instability to the trapped nanoparticles or bio-targets. Here, we report an effective laser cooling of trapped Yb3+-Er3+ co-doped rare-earth nanoparticle by employing a new cooling channel provided by Er3+ and utilizing an enhancement of the anti-Stokes emission through energy transfer between Yb3+ and Er3+. Especially in high temperature conditions, the co-doped system demonstrates a high laser cooling performance, that enable the temperature to decrease from 500 K to around room temperature. But for the initial temperature of around room temperature, the cooling temperature does not drop below freezing, which can avoid not only thermal but also cold damage to bio-targets in optical tweezers. This work provides experimental evidence of the Yb3+-Er3+ co-doping rare-earth nanoparticle for laser cooling, which can hold a potential to address the challenge of precise measurements in optical tweezers. The high-power trapping lasers in optical tweezers generate damaging heat. Here, the authors demonstrate efficient laser cooling using an erbium-ytterbium co-doped nanoparticle, which cools targets from high temperatures to near room temperature while avoiding sub-zero cooling from ambient conditions, thus enabling safe trapping of biological specimens.
We report a theoretical scheme for realizing efficient and enhanced laser cooling in Ho3+-doped solids, based on ground-state absorption (GSA) of I58→I57 at around 2.07 μm and excited-state absorption (ESA) of I55→F55 at around 2.28 μm. The upconversion-quenching-induced heat that usually is found in Ho3+ optical refrigeration can be significantly alleviated by using the copumping scheme, so the cooling power density and the cooling efficiency are greatly improved. The scheme works at temperatures above 133 K, and can shorten the time needed to reach the minimum attainable temperature of the cooling system. Besides, the dopant concentration is allowed to be promoted to around 1%. The copumping scheme can also be applied to other multilevel (such as Tm3+ and Er3+) optical refrigeration systems to improve the cooling performance.
We report a theoretical scheme for laser cooling of solids based on energy transfer usually found in rare-earth codoped materials. The cooling scheme enables a large enhancement in the cooling efficiency with regard to the standard anti-Stokes fluorescence cooling. A Ho3+ and Tm3+-codoped low-phonon crystal (LiYF4) sample is investigated to find that the cooling efficiency increases, and then decreases with the increasing of the resonant absorption. The optimal cooling efficiency is predicted to exceed 5%. The maximum cooling power density could be promoted greatly by applying the codoped cooling scheme. The cooling scheme is also valid for other rare-earth (for example, Tm3+ and Er3+, or Er3+ and Yb3+) codoped materials.