Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Semiconductor Science and Technology

Coherent manipulation of biexcitonic transitions and other two-pair correlations

V. M. Axt

Published Mar 8, 2004• 5 citations
Publisher

Abstract

Two-pair correlations are shown to induce dependences of the nonlinear optical response of semiconductors that can be used for a coherent manipulation of the resulting emission. Influences of biexcitonic transitions as well as transitions to two-pair scattering states are discussed within a microscopic density matrix approach. It is shown that the coherent control of biexciton beats is selective with respect to the propagation direction of the emitted signal, in contrast to the control of beats where all beat partners are generated by single photon processes. Furthermore, it is demonstrated that memory structures induced by exciton?exciton scattering states enable coherent manipulations of the excitonic line shape that allow us to estimate lower bounds for the corresponding memory time from experimentally accessible data.

DOI
10.1088/0268-1242/19/4/073

Related papers

Coherent control of exciton–biexciton beats: direction selectivity of four‐wave‐mixing signals in experiment and microscopic theory

T. Voss, Ilja Rückmann, J. Gutowski +2 more

Abstract In experiments and simulations based on a microscopic theory the optical coherent control of exciton–biexciton beats in coherent four‐wave‐mixing signals from a semiconductor quantum well is demonstrated. It is found that a reduction of the beat amplitude for one four‐wave‐mixing direction may at the same time coincide with a large beat amplitude for the other direction. The results can be understood by considering that at least two‐photon processes are required to coherently excite biexcitonic transitions which are responsible for the occurrence of the beat structure in the four‐wave‐mixing signals. (© 2006 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)

physica status solidi (b)•Jul 12, 2006•1 citation

Coherent control of the exciton and exciton-biexciton transitions in the generation of nonlinear wave-mixing signals in a semiconductor quantum well

T. Voss, Ilja Rückmann, J. Gutowski +2 more

By use of an optical coherent-control technique we demonstrate and analyze the control of transitions involved in the generation of four-wave-mixing signals in a semiconductor quantum well for the two different four-wave-mixing directions and for different sequences of the excitation pulses. Results are presented for frequency- as well as for time-resolved signals. A doubling of the coherent switching frequency is found which occurs if the laser pulses performing the control process contribute quadratically to the wave-mixing signal. A direct comparison between experiment and microscopic theory reveals how the coherent-control process acts on the coherent polarization of the exciton-biexciton system in all different configurations. An additional interpretation of the experimental results based on a simplified few-level model is able to provide an intuitive understanding of the relevant processes which govern the coherent control of the excitonic and biexcitonic wave-mixing polarizations.

Physical Review B•Mar 9, 2006•31 citations

Influence of Two-Pair Continuum Correlations Following Resonant Excitation of Excitons

V. M. Axt, Björn Haase, U. Neukirch

The memory structure induced by coherent transitions to the exciton-exciton scattering continuum is shown to have significant influence on spectrally resolved four-wave-mixing signals even under selective excitation of 1s excitons. Comparisons between experiments and calculations that account nonperturbatively for these quantum kinetic Coulomb correlations demonstrate large compensations between mean-field contributions and transitions to the two-pair continuum. Experiments with different polarizations of the laser pulses show that two-pair continuum correlations are responsible for delay-time dependent shifts of the excitonic emission as well as for substantial deformations of the line shape.

Physical Review Letters•May 14, 2001•32 citations

Correlated Coulomb quantum kinetics in optically excited semiconductors

V. M. Axt, Björn Haase

Correlations due to biexcitons as well as to two-pair scattering states are direct manifestations of Coulomb quantum kinetics. Effects resulting from the memory structure of the corresponding contributions to the optical interband polarization are analyzed taking a ZnSe single-quantum well as model system. Our calculations are based on a microscopic density matrix description using the dynamics controlled truncation scheme for closing the hierarchy of higher-order density matrices. A detailed comparison between experiment and theory allows for the identification of numerous effects directly reflecting different aspects of pair-correlations. In particular, we demonstrate various influences of the two-pair scattering continuum on four-wave-mixing signals. Furthermore, we show that signals with a dynamically changing polarization sensitively monitor a competition between coherent parts of the dynamics and signal components induced by incoherent exciton densities. Surprisingly, the phase of these signals is found to be almost unaffected by the presence of incoherent densities. This result can be traced back to a compensation of the influences on the phases resulting from different incoherent parts of the dynamics. Six-particle correlations representing transitions from incoherent densities to two-pair correlations turn out to be indispensable for a proper description of this effect.© (2001) COPYRIGHT SPIE--The International Society for Optical Engineering. Downloading of the abstract is permitted for personal use only.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Apr 10, 2001•0 citations

Coherent control of the exciton-biexciton system demonstrated in four-wave-mixing experiments

T. Voss

Systematic measurements and microscopic simulations were performed to study the optical coherent control of the exciton‐biexciton systems in a ZnSe quantum well. Our results show that the spectral components in the four‐wave mixing signal at the exciton and the exciton‐biexciton transition, respectively, can be separately controlled in the coherent regime. This separate control also results in different beat structures on the real‐time transients of the nonlinear wave‐mixing polarization. With respect to all important features experiment and simulation are in excellent agreement.

AIP conference proceedings•Jan 1, 2005•0 citations

Optical Preparation and Coherent Control of Ultrafast Nonlinear Quantum Superpositions in Exciton Gases: A Case Study for Atomically Thin Semiconductors

Florian Katsch, Andreas Knorr

We report on the optical preparation of coherent superpositions of exciton and biexciton states manifested in temporal nonlinear oscillations in interacting exciton gases.The effect is illustrated for atomically thin semiconductors, where the reflected light reveals these interactions in a unique way.The occurring nonlinear coherent oscillations are counteracted by incoherent excitation-induced dephasing, a phenomenon which originates from a new type of quantum interference between excitons and the twoexciton scattering continuum.To improve the experimental accessibility, we discuss different methods to control the oscillation modulation depth by modifying the mutual interplay of the exciton-biexciton superposition and excitation-induced dephasing.We find that the coherent optical response can be manipulated by the polarization degree of the exciting light field, the laser detuning, external magnetic fields, and quantum coherent feedback.The extraordinary temporal behavior and its control distinguishes the nonlinear coherent oscillations from atomic Rabi oscillations and enables their engineering based on our proposed control schemes.

Physical Review X•Nov 24, 2020•17 citations
Two-pair correlations are shown to induce dependences of the nonlinear optical response of semiconductors that can be used for a coherent manipulation of the resulting emission. Influences of biexcitonic transitions as well as transitions to two-pair scattering states are discussed within a microscopic density matrix approach. It is shown that the coherent control of biexciton beats is selective with respect to the propagation direction of the emitted signal, in contrast to the control of beats where all beat partners are generated by single photon processes. Furthermore, it is demonstrated that memory structures induced by exciton?exciton scattering states enable coherent manipulations of the excitonic line shape that allow us to estimate lower bounds for the corresponding memory time from experimentally accessible data.
Abstract In experiments and simulations based on a microscopic theory the optical coherent control of exciton–biexciton beats in coherent four‐wave‐mixing signals from a semiconductor quantum well is demonstrated. It is found that a reduction of the beat amplitude for one four‐wave‐mixing direction may at the same time coincide with a large beat amplitude for the other direction. The results can be understood by considering that at least two‐photon processes are required to coherently excite biexcitonic transitions which are responsible for the occurrence of the beat structure in the four‐wave‐mixing signals. (© 2006 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)
By use of an optical coherent-control technique we demonstrate and analyze the control of transitions involved in the generation of four-wave-mixing signals in a semiconductor quantum well for the two different four-wave-mixing directions and for different sequences of the excitation pulses. Results are presented for frequency- as well as for time-resolved signals. A doubling of the coherent switching frequency is found which occurs if the laser pulses performing the control process contribute quadratically to the wave-mixing signal. A direct comparison between experiment and microscopic theory reveals how the coherent-control process acts on the coherent polarization of the exciton-biexciton system in all different configurations. An additional interpretation of the experimental results based on a simplified few-level model is able to provide an intuitive understanding of the relevant processes which govern the coherent control of the excitonic and biexcitonic wave-mixing polarizations.
The memory structure induced by coherent transitions to the exciton-exciton scattering continuum is shown to have significant influence on spectrally resolved four-wave-mixing signals even under selective excitation of 1s excitons. Comparisons between experiments and calculations that account nonperturbatively for these quantum kinetic Coulomb correlations demonstrate large compensations between mean-field contributions and transitions to the two-pair continuum. Experiments with different polarizations of the laser pulses show that two-pair continuum correlations are responsible for delay-time dependent shifts of the excitonic emission as well as for substantial deformations of the line shape.
Correlations due to biexcitons as well as to two-pair scattering states are direct manifestations of Coulomb quantum kinetics. Effects resulting from the memory structure of the corresponding contributions to the optical interband polarization are analyzed taking a ZnSe single-quantum well as model system. Our calculations are based on a microscopic density matrix description using the dynamics controlled truncation scheme for closing the hierarchy of higher-order density matrices. A detailed comparison between experiment and theory allows for the identification of numerous effects directly reflecting different aspects of pair-correlations. In particular, we demonstrate various influences of the two-pair scattering continuum on four-wave-mixing signals. Furthermore, we show that signals with a dynamically changing polarization sensitively monitor a competition between coherent parts of the dynamics and signal components induced by incoherent exciton densities. Surprisingly, the phase of these signals is found to be almost unaffected by the presence of incoherent densities. This result can be traced back to a compensation of the influences on the phases resulting from different incoherent parts of the dynamics. Six-particle correlations representing transitions from incoherent densities to two-pair correlations turn out to be indispensable for a proper description of this effect.© (2001) COPYRIGHT SPIE--The International Society for Optical Engineering. Downloading of the abstract is permitted for personal use only.
Systematic measurements and microscopic simulations were performed to study the optical coherent control of the exciton‐biexciton systems in a ZnSe quantum well. Our results show that the spectral components in the four‐wave mixing signal at the exciton and the exciton‐biexciton transition, respectively, can be separately controlled in the coherent regime. This separate control also results in different beat structures on the real‐time transients of the nonlinear wave‐mixing polarization. With respect to all important features experiment and simulation are in excellent agreement.
We report on the optical preparation of coherent superpositions of exciton and biexciton states manifested in temporal nonlinear oscillations in interacting exciton gases.The effect is illustrated for atomically thin semiconductors, where the reflected light reveals these interactions in a unique way.The occurring nonlinear coherent oscillations are counteracted by incoherent excitation-induced dephasing, a phenomenon which originates from a new type of quantum interference between excitons and the twoexciton scattering continuum.To improve the experimental accessibility, we discuss different methods to control the oscillation modulation depth by modifying the mutual interplay of the exciton-biexciton superposition and excitation-induced dephasing.We find that the coherent optical response can be manipulated by the polarization degree of the exciting light field, the laser detuning, external magnetic fields, and quantum coherent feedback.The extraordinary temporal behavior and its control distinguishes the nonlinear coherent oscillations from atomic Rabi oscillations and enables their engineering based on our proposed control schemes.