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The Journal of Physical Chemistry B

Nonclassical Effects of a Two-Level Spin System Interacting with a Two-Mode Cavity Field via Two-Photon Transition

Horacio Grinberg

Published Nov 20, 2008• 7 citations
Publisher

Abstract

The interaction of a two-level cyclic XY n-spin model with a two-mode cavity field involving two-photon transitions is investigated through a generalized Jaynes-Cummings model in the rotating-wave approximation. The two-photon interacting Hamiltonian becomes from the replacement of each single-mode field in the one-photon interacting Hamiltonian with the second-harmonic generation. It was assumed that initially the correlated field modes are in disentangled coherent states having the same photon distribution and that the spin system is in an excited state. At any time t > 0, the spin system and the field are in an entangled state, in this case, via a unitary time evolution operator. Thus, the spontaneous decay of a spin level was treated by considering the interaction of the two-level spin system with the modes of the universe in the vacuum state. The different cases of interest, characterized in terms of a detuning parameter for each mode, which emerge from nonvanishing commutation relations, were analytically implemented and numerically discussed for various values of the initial mean photon number and spin-photon coupling constants. Photon distribution, time evolution of the spin population inversion, as well as the statistical properties of the field leading to the possible production of nonclassical states, such as antibunched light, violations of the Cauchy-Schwartz inequality, and second- and fourth-order squeezing, are examined. The case of zero detuning of both modes was treated in terms of a linearization of the expansion of the time evolution operator, while in other three cases, the computations were conducted via second- and third-order Dyson perturbation expansion of the time evolution operator matrix elements for the excited and ground states of the spin system, respectively.

DOI
10.1021/jp8075244

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The interaction of a two-level cyclic XY n-spin model with a two-mode cavity field involving two-photon transitions is investigated through a generalized Jaynes-Cummings model in the rotating-wave approximation. The two-photon interacting Hamiltonian becomes from the replacement of each single-mode field in the one-photon interacting Hamiltonian with the second-harmonic generation. It was assumed that initially the correlated field modes are in disentangled coherent states having the same photon distribution and that the spin system is in an excited state. At any time t > 0, the spin system and the field are in an entangled state, in this case, via a unitary time evolution operator. Thus, the spontaneous decay of a spin level was treated by considering the interaction of the two-level spin system with the modes of the universe in the vacuum state. The different cases of interest, characterized in terms of a detuning parameter for each mode, which emerge from nonvanishing commutation relations, were analytically implemented and numerically discussed for various values of the initial mean photon number and spin-photon coupling constants. Photon distribution, time evolution of the spin population inversion, as well as the statistical properties of the field leading to the possible production of nonclassical states, such as antibunched light, violations of the Cauchy-Schwartz inequality, and second- and fourth-order squeezing, are examined. The case of zero detuning of both modes was treated in terms of a linearization of the expansion of the time evolution operator, while in other three cases, the computations were conducted via second- and third-order Dyson perturbation expansion of the time evolution operator matrix elements for the excited and ground states of the spin system, respectively.
The interaction of a two-level XYn-spin system with a two-mode cavity field is investigated through a generalized Jaynes-Cummings model in the rotating wave approximation. The spontaneous decay of a spin level was treated by considering the interaction of the two-level spin system with the modes of the universe in the vacuum state. The different cases of interest, characterized in terms of a detuning parameter for each mode, which emerge from the nonvanishing of certain commutation relations between interaction picture Hamiltonians associated with each mode, were analytically implemented and numerically discussed for various values of the initial mean photon number and spin-photon coupling constants. Photon distribution, time evolution of the spin population inversion, as well as the statistical properties of the field leading to the possible production of nonclassical states, such as antibunched light and violations of the Cauchy-Schwartz inequality are examined for an excited initial state. It was assumed that the two modes are initially in coherent states and have the same photon distribution. The case of zero detuning of both modes was treated in terms of a linearization of the expansion of the time evolution operator, while in other three cases, the computations were conducted via second- and third-order Dyson perturbation expansion of the time evolution operator matrix elements for the excited and ground states respectively.
Abstract The interaction of the XY n‐spin cyclic model with a two‐mode cavity field in the rotating‐wave approximation is investigated in the framework of a generalized Jaynes–Cummings two‐level system consisting of the vacuum state and a thermally averaged manifold of excited sates. Computation of the energy of this manifold allows this interaction to be examined in off‐resonant states. Time evolution of the population inversion, photon distribution, and temperature distribution for an excited initial state are computed via second‐ and third‐order perturbation expansion of the time evolution operator matrix elements for the excited and ground states, respectively and for an ideal squeezed initial coherent state of the cavity field. It was assumed that the two modes have initially the same photon distribution. The pattern of the spin population inversion appears as a manifestation of multiple and complicated inerferences, which is mathematically reflected in a double discrete summation that appears in the calculation of the dynamics. © 2007 Wiley Periodicals, Inc. Int J Quantum Chem, 2008
We present a two-mode squeezed Jaynes–Cummings model, built upon the formalism of pair coherent states (PCSs), to investigate the dynamics of a two-level atom interacting with a two-mode quantized field. By solving the time-dependent Schrödinger equation under the rotating-wave approximation, we elucidate the system’s quantum evolution, with particular emphasis on how the squeezing degree and photon number difference modulate atomic population inversion and entanglement. We further quantify the nonclassical traits of the two-mode squeezed PCSs via Mandel’s parameter and the violation of the Cauchy–Schwarz inequality, highlighting their sensitivity to model parameters. These findings illuminate the subtle interplay of squeezing, photon statistics, and entanglement in advanced quantum optical systems.
We study the quantum dynamics of a two-mode two-photon Jaynes–Cummings model of a two-level atom interacting with the correlated two-mode SU(1, 1) coherent states. The collapse and revival patterns in this case are noted to be quite different from those in the case of uncorrelated coherent states and correlated pair-coherent states. As an example of the time evolution of the field statistics we show that violation of the Cauchy–Schwartz inequality by the initial field states may be nullified. We also discuss the evolution of the variance of the two-mode field quadrature operator.
The aim of this study is to investigate an effective two-level atom coupled to a twomode f-deformed cavity field with and without the rotating wave approximation.The first section discusses the theoretical model of the interaction between a two-mode cavity-field and an effective two-level atom within the framework of an f-DJCM without the rotating wave approximation.After that, we obtain the reduced density matrix of the atom with and without the rotating-wave approximation.Then, we have investigated the effect of the counterterm on temporal evolution of various nonclassical properties of the atom, i.e., atomic population inversion, atomic dipole squeezing and atom-field entanglement.Particularly, we compare the numerical result for three different values of the deformation parameter q (q=1, q=1.1, q=1) with and without the rotating wave approximation.
Multiphoton interaction of single-mode squeezed-state light and a two-level atom is considered based on the K-photon Jaynes–Cummings model. Time evolution of quantum fluctuation and photon statistical properties of the initial squeezing light are discussed. It is found that through interaction with a two-level atom, larger squeezing levels cannot be achieved in one-photon or multiphoton processes. For photon antibunching behavior of the light field, it is shown that a smaller initial squeezing level and an appropriately larger coherent part of the initial average photon number of the radiation field favor the generation of this nonclassical behavior, especially in the lower-order interaction processes.