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Physical Review A

Calculation of laser intensity fluctuations from the density-matrix equation of motion

Wallace Arden Smith

Published Jun 1, 1975• 5 citations
Publisher

Abstract

Intensity fluctuations for a single-mode laser near threshold are calculated from the Scully-Lamb equation of motion for the reduced density matrix of the radiation field. The magnitude and correlation time of the intensity fluctuations are contrasted with the results obtained from the usual Fokker-Planck analysis of the rotating-wave, Van-der-Pol (RWVP) model. When the photon number at threshold is not large, these calculations predict measurable differences from the RWVP Fokker-Planck results. Two methods are used to calculate the dynamics. One is a direct eigenfunction expansion of the Green's function of the equation of motion. The other is based on the calculation of the initial derivatives of the correlation function.

DOI
10.1103/physreva.11.2025

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Intensity fluctuations for a single-mode laser near threshold are calculated from the Scully-Lamb equation of motion for the reduced density matrix of the radiation field. The magnitude and correlation time of the intensity fluctuations are contrasted with the results obtained from the usual Fokker-Planck analysis of the rotating-wave, Van-der-Pol (RWVP) model. When the photon number at threshold is not large, these calculations predict measurable differences from the RWVP Fokker-Planck results. Two methods are used to calculate the dynamics. One is a direct eigenfunction expansion of the Green's function of the equation of motion. The other is based on the calculation of the initial derivatives of the correlation function.
A dynamic correspondence is set up between the density matrix of the electromagnetic field and an associated classical function. Means of one and two time quantum operators are shown to be obtainable from the corresponding averages of the associated classical random problem. When all atomic response rates are fast compared to photon rates, the equation of motion is obtained for the field density matrix. The associated classical problem is shown to obey a Fokker-Planck equation. Over a broad region that includes the threshold region, the Fokker-Planck equation is reduced to that for the rotating-wave van der Pol oscillator for which exact numerical solutions have been previously obtained by Hempstead and Lax.
We have calculated the third- and higher-order (multitime) cumulants of the intensity of single-mode laser light using the rotating-wave van der Pol (RWVP) model. Our results indicate a distinctly nonexponential time dependence of the cumulants slightly below threshold and an oscillatory time dependence somewhat above threshold. One can interpret this oscillatory behavior as showing that the larger fluctuations above the mean decay more rapidly than those below the mean. Measurements of the third-order intensity cumulants above threshold would be desirable to check for this behavior and to provide a more rigorous test of the RWVP model than the second-order intensity correlation.
The effect of counter-rotating terms in the interaction Hamiltonian on the photon statistics is investigated for a single-mode laser. The treatment is based on the Scully-Lamb model. A perturbation expansion is used to derive an equation of motion for the field-density matrix. The counter-rotating terms are found to lead to both transient and secular effects. With some reasonable approximations the steady-state photon-number distribution is derived and it is shown that the counter-rotating terms tend to raise the threshold of laser action and broaden the photon-number distribution. The relative size of these effects is found to be very small and depends on the square of the ratio of the atomic linewidth and the transition frequency.
A previously constructed laser model with quantum (noncommuting) noise sources was shown to lead near threshold to a quantum rotating-wave Van der Pol oscillator. A full dynamical correspondence between quantum and classical random processes allows one to compute the average of any time-ordered, normal-ordered operator function by averaging the associated function of classical random variables. Numerical calculations for the associated classical Van der Pol oscillator of the steady-state distribution, the total intensity fluctuations, and the linewidth versus operating point were amply confirmed experimentally. Measurements (and calculations) of higher than two-time correlations were sparse and contradictory. Photocount distributions, at times short compared to the intensity correlation time, confirm only the steady state of the laser. Photocount distributions at intermediate and longer times are difficult to compute because they involve multitime correlations of high ($\ensuremath{\infty}$) order. By providing an exact solution for photocount distributions and their moments for all times, we expected to stimulate measurements near threshold which would provide an adequate test of the Van der Pol laser model. Comparison of the results reported here with recent photocount experiments of Meltzer, Davis, and Mandel and of Jakeman, Oliver, and Pike provides gratifying agreement and confirmation of our statistical understanding of laser fluctuations near threshold.
In this study, we measured the temporal correlations in the electromagnetic field radiated by a laser in the threshold region of oscillation, from 110\frac{1}{10}101​ to 10 times threshold intensity. The experimental results are compared with theoretical predictions based on solutions of a Fokker-Planck equation. We stabilized the intensity of a He-Ne cw gas laser by means of a long-time-constant servo system which controlled the cavity length. Using a fast photomultiplier as detector, we recorded the photoelectron count distribution within a short counting time (3 \ensuremath{\mu}sec) while the photomultiplier was exposed to the laser light. From the photoelectron count distribution measurement, we calculated second, third, and fourth normalized cumulants of the intensity probability density function of the light field. The normalized cumulant is a measure of "pure" correlations among photons because the contributions from lower-order correlations are removed. The statistics of the photoelectron count distribution shows that the intensity fluctuations at about 110\frac{1}{10}101​ threshold are nearly those of a Gaussian field, and continuously approach those of a constant-amplitude field as the intensity is raised to about 10 times threshold. The normalized second, third, and fourth cumulants of the intensity probability density function of the laser light were also measured at 17 and 42% of threshold intensity as the counting time was increased from 3 to 1000 \ensuremath{\mu}sec. The results agree with predictions computed under the assumption that the dependence of the correlation functions on the time variables is the same as for Gaussian light.
The steady-state intensity correlation functions C(t) of the single-mode laser are analyzed with the generalized-moment-expansion method proposed by Nadler and Schulten [Z. Phys. B 59, 53 (1985); J. Chem. Phys. 82, 151 (1985)]. This method approximates C(t) by a superposition of N exponentials that exactly reproduces n derivatives of C(t) at t=0 and m relaxation moments (n+m+1=2N). In this way, the short- and long-time regimes of C(t) are well described even near threshold. With the use of relaxation moments we develop a method to obtain the eigenvalues of the Fokker-Planck operator. This method is applied to the single-mode laser. We show that the knowledge of only two relaxation moments is enough to obtain good results for the two first eigenvalues. The method gives excellent results when the eigenvalues are well separated (below threshold).