We study phase-conjugate degenerate four-wave mixing (DFWM) in an optically pumped, two-level atomic system (the
3s2S1∕2,
F=2, ${m}_{F}=2\ensuremath{\rightarrow}3p\phantom{\rule{0.2em}{0ex}}^{2}P_{3∕2}$,
F=3,
mF=3 transition in a diffuse, collision-free, thermal beam of sodium) using phase-modulated laser beams. In this investigation, we study the detailed line shape of the four-wave mixing signal as a function of the temporal delay between the probe field and the pump fields at different intensities of the cw pump waves and modulation frequencies. We show that phase modulation of the pump and probe beams leads to strong amplitude modulation of the phase-conjugate beam and report excellent agreement between our experimental observations of the DFWM spectra and the results of numerical calculations. Our numerical results suggest an enhancement of the ``local'' DFWM signal when the sidebands of the phase-modulated laser are resonant with dressed-state transitions, but that this resonance is less obvious in the total signal generated. We also show that the complex line shapes depend sensitively upon the delay of the probe beam, with the peak DFWM signal occurring when the probe beam is advanced compared to the pump beam.
We report on the enhancement of phase conjugation degenerate four-wave mixing (DFWM) in hot atomic Rb vapor by using a Bessel beam as the probe beam. The Bessel beam was generated using cross-phase modulation based on the thermal nonlinear optical effect. Our results demonstrated that the DFWM signal generated by the Bessel beam is about twice as large as that generated by the Gaussian beam, which can be attributed to the extended depth and tight focusing features of the Bessel beam. We also found that a DFWM signal with reasonable intensity can be detected even when the Bessel beam encounters an obstruction on its way, thanks to the self-healing property of the Bessel beam. This work not only indicates that DFWM using a Bessel beam would be of great potential in the fields of high-fidelity communication, adaptive optics, and so on, but also suggests that a Bessel beam would be of significance to enhance the nonlinear process, especially in thick and scattering media.