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Optics Letters

Tunable resonance fluorescence monochromator with sub-Doppler spectral resolution

Nathan C. Pixley, Tiffany L. Correll, Dimitri Pappas, Oleg I. Matveev, Benjamin W. Smith, James D. Winefordner

Published Dec 15, 2001• 15 citations
Publisher

Abstract

A cesium-based resonance fluorescence monochromator with a spectral resolution of 200 MHz and a tunable response over the D(2) absorption line of cesium (380 MHz) is described. The narrow spectral response is achieved through excitation of a monokinetic population of the 6(2)P(3/2)( degrees ) state by arrangement of the excitation lasers in either a copropagating or a counterpropagating orientation. The narrow spectral response of the detector allows for excitation of specific hyperfine components involved in the 6(2)P(3/2)( degrees ) (F=3-5) to 6(2)D(5/2) (F=2-6) transition (917.23 nm). The selectivity gained through resolving specific hyperfine transitions allows for a photon detector that is both spectrally tunable and narrow. We report the sub-Doppler linewidths achieved through various laser beam orientations. We also describe how these beam geometries can be applied to spectrally narrow and tunable image detection.

DOI
10.1364/ol.26.001946

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•Jan 1, 1991•0 citations
A cesium-based resonance fluorescence monochromator with a spectral resolution of 200 MHz and a tunable response over the D(2) absorption line of cesium (380 MHz) is described. The narrow spectral response is achieved through excitation of a monokinetic population of the 6(2)P(3/2)( degrees ) state by arrangement of the excitation lasers in either a copropagating or a counterpropagating orientation. The narrow spectral response of the detector allows for excitation of specific hyperfine components involved in the 6(2)P(3/2)( degrees ) (F=3-5) to 6(2)D(5/2) (F=2-6) transition (917.23 nm). The selectivity gained through resolving specific hyperfine transitions allows for a photon detector that is both spectrally tunable and narrow. We report the sub-Doppler linewidths achieved through various laser beam orientations. We also describe how these beam geometries can be applied to spectrally narrow and tunable image detection.
Improvements in spectral resolution and sensitivity of a cesium based resonance fluorescence imaging monochromator (RFIM) are described. Alignment of the two lasers used in the excitation scheme in a co-propagating geometry have resulted in a detector spectral bandpass (270 MHz) that is narrower than the Doppler broadened profile (380 MHz) of cesium vapor at room temperature. Improvements in the experimental design, namely the addition of an image intensifier and cooled charge-coupled device (CCD) camera, have resulted in increased sensitivity; we report a limit of detection of 10 8 photons per pixel limited by image intensifier noise. Images of the cesium D 2 line emission (852.12 nm) from a cesium hollow cathode lamp were compared to an argon emission line (4Sº 1/2 → 4P 3/2 ) at 852.14 nm from a silver/argon hollow cathode lamp as a demonstration of the spectral resolution. The ability of the RFIM to discriminate between photons exciting the F = 4 vs. F = 3 ground state hyperfine level (a frequency difference of 9.2 GHz) of the cesium 6 2 S 1/2 state was also investigated to further demonstrate the spectral selectivity. The potential use of the described RFIM for chemical imaging applications is discussed.
Sub-Doppler resonances in caesium vapours are studied in a laser field produced by counterpropagating two-frequency light beams with mutually orthogonal linear polarisations. The beams are in resonance with optical transitions in the D1 line, the frequency difference of the field spectral components being equal to the hyperfine ground-state splitting in the Cs atom (≈9.2 GHz). It has already been shown that in this configuration, the hypercontrast effect can be observed for sub-Doppler resonances, which makes this configuration promising for the employment in newgeneration miniature optical frequency standards. In the present work, two different two-frequency configurations are compared with each other and with the single-frequency configuration widely used in practice for observing saturated absorption resonances. The parameters of nonlinear resonances are measured at various temperatures of caesium vapours and at different optical field intensities. The results of the investigations performed make it possible to find an optimal two-frequency scheme for exciting nonlinear resonances and to estimate a potential of the scheme for its applications in quantum metrology.
We report on the investigation of narrow sub-Doppler-width resonances observed at the D2 line of Cs atoms (Fg = 4 → Fe = 3, 4, 5 hyperfine transitions), confined in thin optical cells. These cells have a thickness of L = 6λ (λ = 852 nm) and L = 700 μm, and are irradiated by two narrow-band laser radiations (one with fixed and the other with scanned frequency). We show that for zero frequency detuning of the fixed-frequency laser from the Fg = 4 → Fe = 5 hyperfine transition, its absorption spectrum in the thin cell consists of resonances, centered at the respective hyperfine transitions. The spectral widths of these resonances range from 2 to 20 MHz, and they are characterized by a good contrast and extremely small Doppler background. This spectrum is highly sensitive to the frequency offset of the fixedfrequency laser. The analysis leads to the conclusion that the spatial restriction of Cs vapor suppresses the interaction of the light with atoms with significant velocity component along the direction of the laser beam propagation.
The absorption and fluorescence spectra of a submicron Cs vapour layer under resonant excitation on the D2 line are measured. Sub-Doppler features centered at the resonance frequency of the hyperfine (hf) transitions have been observed. Substantial changes in the amplitude and width of the sub-Doppler resonances for individual hf transitions were recorded in dependence on the intensity of the incident laser radiation. In the fluorescence spectra narrow dips due to the effects of saturation have been observed. We also report about the observation of coherence resonances in Hanle configuration obtained at cell thickness of the order of the wavelength of the laser light.
Abstract Sub-Doppler resonances in caesium vapours are studied in a laser field produced by counterpropagating two-frequency light beams with mutually orthogonal linear polarisations. The beams are in resonance with optical transitions in the D1 line, the frequency difference of the field spectral components being equal to the hyperfine ground-state splitting in the Cs atom (∼9.2 GHz). It has already been shown that in this configuration, the hypercontrast effect can be observed for sub-Doppler resonances, which makes this configuration promising for the employment in new-generation miniature optical frequency standards. In the present work, two different two-frequency configurations are compared with each other and with the single-frequency configuration widely used in practice for observing saturated absorption resonances. The parameters of nonlinear resonances are measured at various temperatures of caesium vapours and at different optical field intensities. The results of the investigations performed make it possible to find an optimal two-frequency scheme for exciting nonlinear resonances and to estimate a potential of the scheme for its applications in quantum metrology.
The resonant excitation of the sodium D2 transition by laser radiation was investigated experimentally in this thesis. Line polarization measurement of the resonance fluorescence was employed to investigate the excitation process. The sodium atoms, which were collimated in a very narrow beam, were excited by a monochromatic laser beam with the frequency tuned to resonance with the 32S 112(F=2) - 32P312 hyperfine transition. The direction of the laser beam was perpendicular to the atomic beam and the fluorescence photons were detected along a direction perpendicular to both the laser and atomic beams. The experimental measurements were performed to determine the effect due to the variation of the laser intensity and frequency on the line polarization. A theoretical expression of the line polarization as a function of density matrix elements of the upper excited hyperfine sub -states was derived. A full quantum electrodynamic theory was used to derive an atomic operator equation of motion which was needed to calculate atomic operator elements. These elements then yielded the corresponding density matrix elements. The experimental results and the theoretical modelling were in a good agreement. The first experimental results for the line polarization of the highly excited states, 42D512 and 42D312, are also presented. The use of two lasers enabled these highly excited states to be excited. The line polarization of the fluorescence for transitions from the 4D level down to lower states is derived in terms of the density matrix elements of the upper excited states. Two limiting cases for the theoretical predictions of the line polarization are considered.