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Journal of Magnetism and Magnetic Materials

Spin dynamics in the BEC phase of the S=1/2 quantum spin system TlCuCl3

Christian Rüegg, N. Cavadini, A. Fürrer, K Krämer, Hans Ulrich Güdel, Peter Vorderwisch, Klaus Habicht, H. Mutka, Andrew R. Wildes

Published Jan 2, 2004• 5 citations
Publisher
DOI
10.1016/j.jmmm.2003.11.075

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Exploiting the analogy between ultracold atomic gases and the system of triplons, we study magneto-thermodynamic properties of dimerized quantum magnets in the framework of Bose–Einstein condensation (BEC). Particularly, introducing the inversion (or Joule–Thomson) temperature [Formula: see text] as the point where Joule–Thomson coefficient of an isenthalpic process changes its sign, we show that for a simple paramagnet, this temperature is infinite, while for three-dimensional (3D) dimerized quantum magnets it is finite and always larger than the critical temperature [Formula: see text] of BEC. Below the inversion temperature [Formula: see text], the system of triplons may be in a liquid phase, which undergoes a transition into a superfluid phase at [Formula: see text]. The dependence of the inversion temperature on the external magnetic field [Formula: see text] has been calculated for quantum magnets of TlCuCl3 and Sr3Cr2O8.