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Journal of Physics A Mathematical and General

Lop-sided diffraction by absorbing crystals

Michael Berry

Published Apr 17, 1998• 84 citations
Publisher

Abstract

Diffraction of atoms by a particular absorbing `crystal of light', that has been studied experimentally, is described by the complex potential . The diffracted beam intensities can be calculated exactly, as a function of (dimensionless) potential strength , angle of incidence , and crystal thickness . Only the beams have nonzero intensity; this `lop-sidedness' is a dramatic violation of Friedel's law. The n th beam is strong at Bragg angles , and the peaks get sharper with increasing ; they correspond to degeneracies of the (non-Hermitian) governing matrix. For normal incidence , the are periodic in , and as n increases they approach a self-similar function of .

DOI
10.1088/0305-4470/31/15/014

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Diffraction of atoms by a particular absorbing crystal of light', that has been studied experimentally, is described by the complex potential . The diffracted beam intensities can be calculated exactly, as a function of (dimensionless) potential strength , angle of incidence , and crystal thickness . Only the beams have nonzero intensity; this lop-sidedness' is a dramatic violation of Friedel's law. The n th beam is strong at Bragg angles , and the peaks get sharper with increasing ; they correspond to degeneracies of the (non-Hermitian) governing matrix. For normal incidence , the are periodic in , and as n increases they approach a self-similar function of .
A medium described by an imaginary potential (or imaginary (refractive index) ), that varies sinusoidally in one direction, acts as a volume grating for plane waves incident on it obliquely or normally. Two peculiar features are identified. First, if the potential is weak, so that there are only two significant diffracted beams near the Bragg angle, and three for normal incidence, diffraction is strongly affected by degeneracies of the non-Hermitian matrix generating the `Bloch waves' in the grating; the effect of these degeneracies is very different from that of the Hermitian degeneracies for transparent gratings. Second, if the potential is strong and the grating thick, the asymptotic distribution of intensities among the diffracted beams (momentum distribution) is a rather narrow Gaussian, and dominated by a single set of complex rays; this is very different from the semiclassical limit for transparent gratings, where the rays form families of caustics proliferating with thickness, and with a wider momentum distribution.
The diffraction of a coherent, stationary, beam of atoms from a standing wave of light is considered. Particular attention is paid to long interaction times for which the motion of the atoms inside the light field must be taken into account. This is the regime of dynamical diffraction, and is treated within the framework of a set of differential difference equations due to Raman and Nath. The popular Raman-Nath approximation, in which the kinetic energy imparted to the atoms by the light wave is ignored, is no longer valid and the full equations must be solved. When the interaction between the atoms and the light is very weak then few beams are produced. To describe spontaneous emission from the atom one can invoke a complex potential as a model for dissipation. If the atom beam is obliquely incident one finds anomalously high transmission close to the Bragg angles which is the physical manifestation of degeneracies in non-Hermitian matrices. The classical limit is approached when the atom-light interaction is strong, producing many beams. The classical dynamics (geometrical rays) reveal that the farfield intensity pattern is dominated by caustics. These proliferate with increasing interaction distance. Two methods are presented for analytically treating the semiclassical limit of the wave mechanics. The first begins with W.K.B. solutions to the continuised Raman-Nath equations. Mapping onto parabolic cylinder functions removes the spurious divergences of the W.K.B. solutions, giving eigenvectors which are uniformly valid for all scattering angles and may be summed to give the wavefunction. The second method transforms the original W.K.B. eigensum, using the Poisson summation formula, giving a new sum, each term of which has classical significance. This method shows that wave theory decorates the classical caustics with an Airy function intensity profile, as predicted by catastrophe theory.
Atoms in light crystals formed by a standing light wave are a model system to study the propagation of matter waves in periodic potentials. The encountered phenomena can be described by dynamical diffraction theory which has been extensively studied for x-ray, electron, and neutron scattering from solid state crystals. In this paper we show that an atomic de Broglie wave traversing a standing light wave allows investigation of predictions of dynamical diffraction theory which were previously experimentally not accessible. We present standard diffraction efficiency characterizations for pure absorptive and pure refractive crystals. Additionally we were able to measure directly the total atomic wave field formed inside a refractive and an absorptive crystal and to confirm the predicted absolute position of the atomic wave field with respect to the lattice planes. By superposing two standing light waves of different frequency we tailored a new kind of crystal potential where Friedel's law about usual diffraction symmetries is maximally violated.
Bragg diffraction of atoms at thick standing light waves requires that the wave-matching condition is fulfilled. This usually means that the atomic beam crosses the light wave exactly at the Bragg angle. Nevertheless, our experiments also demonstrate Bragg diffraction at detuned angles if the amplitude of the standing light wave is temporally modulated with an appropriate frequency. If, on the other hand, the phase of the light wave is modulated no diffraction is observed. Both modulation processes produce frequency sidebands which set up `slowly travelling standing waves' in front of a retro-reflection mirror. Atoms are diffracted at these `almost standing' light waves in a similar way to photons at the travelling sound waves in an acousto-optic modulator. The frequency of the diffracted de Broglie waves is assumed to be shifted by the intensity modulation frequency. The different results using amplitude- and phase-modulated light waves are due to interference between the diffraction contributions of the individual frequency sidebands contained in the standing light wave.
The subject of the review is the diffraction of an electromagnetic wave on a periodic condensed matter where the Bragg condition is satisfied at the frequency of resonance excited in this medium. The Bragg systems known as resonant photonic crystals in general have been considered, and the propagation, reflection, transmission, and diffraction of electromagnetic radiation in different objects—(I) periodic quantum-well structures near the exciton resonance, (II) optical lattices of atoms cooled in a laser field, and (III) bulk crystals and multilayers with gamma-ray resonance intranuclear transitions—have been described in a unified context. The main attention has been paid to the steady-state linear diffraction, including resonant reflection and transmission, which is the best studied and allows a comparison of the three aforementioned systems with the aim of revealing specific characteristics and common features. A characteristic common property of the considered systems is the suppression of non-radiative channels and an inhomogeneous broadening of the resonance frequency. The second fundamental property of resonant photonic crystals is that the interaction of light with resonant excitation can occur in two regimes depending on the thickness of the sample. In the superradiant regime realized for a small number of resonant layers N (fine structures), the height of the peak and half-width of the reflection spectrum monotonically increase with increasing value of N. With a further increase in N, there occurs a transition to a photonic-crystal regime where the half-width of the reflection spectrum is saturated, which manifests itself in the form of an optical stop band. The theoretical description is illustrated by experimental spectra measured for all three resonant Bragg systems.