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Physical Review E

Critical wetting transitions in two-dimensional systems subject to long-ranged boundary fields

A. Drzewiński, Anna Maciołek, Artur Barasiński, S. Dietrich

Published Apr 28, 2009• 5 citations
Publisher

Abstract

Using the quasiexact density-matrix renormalization-group method and ground-state analysis we study interface delocalization transitions in wide two-dimensional Ising strips subject to long-ranged boundary fields with opposite signs at the two surfaces. Based on this approach, our explicit calculations demonstrate that critical wetting transitions do exist for semi-infinite two-dimensional systems even if the corresponding effective interface potentials decay asymptotically for large l as slow as l(-delta) with delta<2, where l is the distance of the mean interface position from the one-dimensional surface. This supersedes opposite claims by Kroll and Lipowsky [Phys. Rev. B 28, 5273 (1983)] and by Privman and Svrakić [Phys. Rev. B 37, 5974 (1988)] obtained within effective interface models. The corresponding wetting phase diagram is determined, including the cases delta=2 and delta=49 with the latter mimicking short-ranged surface fields. Our analysis highlights the limits of reliability of effective interface models.

DOI
10.1103/physreve.79.041144

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Physical review. E•Feb 1, 2017•0 citations
Using the quasiexact density-matrix renormalization-group method and ground-state analysis we study interface delocalization transitions in wide two-dimensional Ising strips subject to long-ranged boundary fields with opposite signs at the two surfaces. Based on this approach, our explicit calculations demonstrate that critical wetting transitions do exist for semi-infinite two-dimensional systems even if the corresponding effective interface potentials decay asymptotically for large l as slow as l(-delta) with delta<2, where l is the distance of the mean interface position from the one-dimensional surface. This supersedes opposite claims by Kroll and Lipowsky [Phys. Rev. B 28, 5273 (1983)] and by Privman and Svrakić [Phys. Rev. B 37, 5974 (1988)] obtained within effective interface models. The corresponding wetting phase diagram is determined, including the cases delta=2 and delta=49 with the latter mimicking short-ranged surface fields. Our analysis highlights the limits of reliability of effective interface models.
Effective Hamiltonian models predict nonuniversal critical singularities for two-dimensional wetting transitions with marginal long-ranged forces. We test these predictions by studying interfacial delocalization transitions in an infinitely long Ising strip, of width L (lattice spacings), with external fields that are long ranged and have opposite signs at each surface. Finite-size scaling suggests that the shift of the delocalization temperature T(c)(L) below the (semi-infinite) wetting temperature T(w) scales as L(-1/beta(s)) with beta(s) the adsorption critical exponent. Density-matrix renormalization-group methods allow us to study the behavior of T(c)(L) for L up to several hundred lattice spacings. For short-ranged forces the method recovers the universal value of beta(s)=1 known from the exact solution. While marginal long-ranged forces strongly influence the finite-size scaling of T(c)(L) , the extrapolated asymptotic value for the exponent beta(s) does not appear to confirm the predicted nonuniversality, but instead approaches the same universal value representative of systems with short-ranged forces.
Abstract. Effective Hamiltonian models predict non-universal critical singularities for two--dimensional wetting transitions with long-ranged forces. We verify these predictions by studying delocalization transitions in an infinitely long Ising strip, of width L (lattice spacings), with long-ranged surface fields that have opposite sign at each surface. The extrapolated asymptotic value for the exponent βs does not confirm to the predicted non-universality but instead approaches the same universal value representative of systems with short-ranged forces. The crossover of the scaling behaviour of the transition lines is presented. Moreover, contrary to the existing predictions, the critical wetting transition for p = 2 has been found.
The excess adsorption Gamma in two-dimensional Ising strips (infinityxL), subject to identical boundary fields at both one-dimensional surfaces decaying in the orthogonal direction j as -h1j(-p), is studied for various values of p and along various thermodynamic paths below the bulk critical point by means of the density-matrix renormalization-group method. The crossover behavior between the complete-wetting and critical-adsorption regimes, occurring in semi-infinite systems, is strongly influenced by confinement effects. Along isotherms T=const the asymptotic power-law dependences on the external bulk field, which characterize these two regimes, are pre-empted by capillary condensation. Along the pseudo-first-order phase-coexistence line of the strips, which varies with temperature, we find a broad crossover regime in which both the thickness of the wetting film and Gamma increase as functions of the reduced temperature tau but do not follow any power law. Above the wetting temperature the order-parameter profiles are not slablike but exhibit wide interfacial variations and pronounced tails.
The theory of interface localization in near-critical planar systems at phase coexistence is formulated from first principles. We show that mutual delocalization of two interfaces, amounting to interfacial wetting, occurs when the bulk correlation length critical exponent ν is larger than or equal to 1. Interaction with a boundary or defect line involves an additional scale and a dependence of the localization strength on the distance from criticality. The implications are particularly rich in the boundary case, where delocalization proceeds through different renormalization patterns sharing the feature that the boundary field becomes irrelevant in the delocalized regime. The boundary delocalization (wetting) transition is shown to be continuous, with surface specific heat and layer thickness exponents which can take values that we determine.
We performed extensive simulations of the random-bond Ising model confined between walls where competitive surface fields act. By properly taking the thermodynamic limit we unambiguously determined wetting transition points of the system, as extrapolation of localization-delocalization transitions of the interface between domains of different orientation driven by the respective fields. The finite-size scaling theory for wetting with short-range fields [E. V. Albano and K. Binder, Phys. Rev. Lett. 109, 036101 (2012)] establishes that the average magnetization of the sample, with critical exponent $\ensuremath{\beta}$, is the proper order parameter for the study of wetting. While the hyperscaling relationship given by $\ensuremath{\gamma}+2\ensuremath{\beta}={\ensuremath{\nu}}_{\ensuremath{\parallel}}+{\ensuremath{\nu}}_{\ensuremath{\perp}}$ requires $\ensuremath{\beta}=1/2$ ($\ensuremath{\gamma}=4, {\ensuremath{\nu}}_{\ensuremath{\parallel}}=3$, and ${\ensuremath{\nu}}_{\ensuremath{\perp}}=2$), the thermodynamic scaling establishes that ${\mathrm{\ensuremath{\Delta}}}_{s}=\ensuremath{\gamma}+\ensuremath{\beta}$, which in contrast requires $\ensuremath{\beta}=0$ (${\mathrm{\ensuremath{\Delta}}}_{s}=4$), where $\ensuremath{\gamma}, {\ensuremath{\nu}}_{\ensuremath{\parallel}}, {\ensuremath{\nu}}_{\ensuremath{\perp}}$, and ${\mathrm{\ensuremath{\Delta}}}_{s}$ are the critical exponents of the susceptibility, the correlation lengths parallel and perpendicular to the interface, and the gap exponent, respectively. So, we formulate a finite-size scaling theory for wetting without hyperscaling and perform numerical simulations that provide strong evidence of hyperscaling violation (i.e., $\ensuremath{\beta}=0$) and a direct measurement of the susceptibility critical exponent $\ensuremath{\gamma}/{\ensuremath{\nu}}_{\ensuremath{\perp}}=2.0\ifmmode\pm\else\textpm\fi{}0.2$, in agreement with theoretical results for the strong fluctuation regime of wetting transitions with quenched noise.