Physical Review A

Stark-induced phase modulation in coherent Raman spectroscopy

Hans Moosmüller, D A Krueger, C. Y. She

Published Dec 1, 1988• 3 citations

Abstract

The phase of molecular motion is modulated by the optical Stark effect due to high-intensity laser beams. This is shown to lead to modulation in coherent Raman spectra. The spectral modulation is more pronounced in stimulated Raman spectroscopy than in four-wave-mixing Raman spectroscopy. Increased damping reduces the phase modulation leading to the commonly known spectra.

DOI: 10.1103/physreva.38.6210

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