A method is proposed for generating conditional single-photon states with a high degree of purity in a single-mode cavity by successive discrete photodetection. The cavity is pumped by resonance fluorescence emission from a source atom driven by a classical field. The cavity is tuned to a Mollow sideband. A relation between detector parameters is found that makes it possible to interpret the detection of a probe atom in the excited state as unambiguous evidence that a pure single-photon state has been prepared in the cavity. An expression is derived for the prior probability of such an event, and dependence of the one-photon state population of the cavity field on detuning, relaxation rate, and time is examined.
A method is proposed for generating conditional single-photon states with a high degree of purity in a single-mode cavity by successive discrete photodetection. The cavity is pumped by resonance fluorescence emission from a source atom driven by a classical field. The cavity is tuned to a Mollow sideband. A relation between detector parameters is found that makes it possible to interpret the detection of a probe atom in the excited state as unambiguous evidence that a pure single-photon state has been prepared in the cavity. An expression is derived for the prior probability of such an event, and dependence of the one-photon state population of the cavity field on detuning, relaxation rate, and time is examined.
We investigate properties of a two-level atom coupled to a single cavity mode, and driven by a strong, in general off-resonance, external field. The cavity field is tuned to resonance with a Mollow sideband. We show that the steady-state atomic population may be highly (nearly totally) inverted, a phenomenon forbidden in semiclassical theory, and that a strong enhancement of the resonance fluorescence results. This system is suggested as an alternative approach to create the atomic inversion necessary for laser or maser generation without using additional atomic levels. We also investigate properties of the cavity field, derive an analytical expression for the photon number distribution in the good cavity or strong-coupling limit, and discuss the conditions under which this system acts as a single-atom dressed-state laser.
A theory of the discrete photodetection of quantum jumps on the V configuration of atomic levels has been developed. A three-level source atom is placed in a cavity excited by a resonance fluorescence field. The cavity is tuned to exact resonance with an atomic transition. The cavity mode state is tested by a flux of unexcited (at the entrance) probe atoms passing through the cavity. The energy states of the outgoing probe atoms are detected by ionization chambers, which are assumed ideal. This a posteriori statistical information is indirectly related to the numerical characteristics of a measured quantum system consisting of the source atom and cavity mode. The “tuning” conditions for a discrete photodetector, i.e., the rules for choosing the parameters and durations of the interactions of the cavity mode with the probe and source atoms, intensities of the pump and probe fields that are necessary for observing quantum jumps from the “bright” state to the “dark” one and vice versa, have been determined. A two-state model that describes the dynamics of a quantum jump has been analyzed. The formulas have been obtained for the observable characteristics of quantum jumps: the mean residence time of the quantum system in quasistationary states (durations of the bright and dark periods), probabilities of quantum jumps, mean excitation levels of the quantized cavity mode, etc.
We present a quantum theory of a coherently pumped two-level atom in a photonic crystal, coupled to both a multi-mode wave-guide channel and a high quality micro-cavity embedded within the photonic crystal. The cavity field characteristics are highly distinct from that of a corresponding high Q cavity in ordinary vacuum. If the cavity field mode is resonant with the central component of the Mollow spectrum of atomic resonance fluorescence, enhanced, inversionless, nearly coherent light generation occurs when the photon density of states jump between the Mollow spectral components is large. The spectrum of the cavity field is also investigated and showed to be narrower than in the case of a conventional cavity. Moreover, enhanced, non-classical light generation is possible, if the cavity field is tuned on resonance with a Mollow sideband.
Abstract Frequency-resolved photon statistics of resonance fluorescence generated from a two-level system driven by a strong laser field and a weak laser field with equal frequencies are studied. The frequency resolution of fluorescent radiation is described by quantum filtering dynamics, which is simulated theoretically by two single-mode quantum optical cavities with tunable frequencies to scan the incident fluorescent radiation. By calculating the two-photon intensity–intensity correlation functions in terms of the cavity modes, we demonstrate that two-color strong correlations of resonance fluorescence can be generated not only between the opposite sidebands, but also between the central band and one of the sidebands: although both sidebands are broadened due to the perturbation of the weak laser field on the strong-field dressed atom. We emphasize that these properties are in contrast to the conventional case of the standard single-atom Mollow triplet. Moreover, if the resonance frequencies of the two filtering cavities are tuned appropriately, broadband two-color strong correlations are predicted, and the physical origin is revealed from the perspective of quantum interference of photon emission dynamics. This can be considered as a feasible scheme for the design of broadband non-classical light sources, and may be beneficial to the quantum precise detection of atomic and molecular dynamics via quantum optical spectroscopy.
A cavity-modified master equation is derived for a coherently driven two-level atom coupled to a single-mode cavity in the bad cavity limit, in which the cavity frequency is tuned to either the center or one of the sidebands of the Mollow triplet. The atomic populations in both the bare- and dressed-state representations are analyzed in terms of the cavity-modified transition rates. In the bare-state basis, the role of the cavity may be interpreted as enhancing the stimulated absorption of the atom while suppressing the stimulated emission. The bare-state population may thus be inverted under appropriate conditions. The dressed-state inversion, however, originates from the enhancement of the atom-cavity interaction when the cavity is resonant with the atomic dressed-state transition. We show that two-phase quadratures of the atomic polarization decay at different rates. The decay of the in-phase (or out-of-phase) quadrature may be greatly inhibited as the driving intensity increases, depending on the cavity resonant frequency. The spectrum of the atomic fluorescence emitted out the side of the cavity is also studied. The spectral profiles are sensitive to the cavity frequency. When the cavity frequency is tuned to the center of the Mollow resonances, the fluorescence spectrum is symmetrical with three peaks whose linewidths and heights are intensity dependent. When the cavity frequency is tuned to one of the Mollow sidebands, however, it is asymmetric, and the central peak and the sideband on resonance with the cavity can be significantly suppressed for strong driving fields. All three spectral lines can be narrowed by increasing the Rabi frequency. The physics of these striking spectral features is explored in the dressed-state basis. We also investigate the probe absorption spectrum. When the cavity frequency is tuned to the center of the Mollow fluorescence triplet, the central component exhibits a Lorentzian line shape, while the side bands show the Rayleigh-wing line shape. Probe gain may occur at line center due to cavity-induced, bare-state population inversion. When the cavity is tuned to resonance with one sideband, only two sidebands, with Lorentzian profiles, dominate. Gain can occur at the sideband far off resonant with the cavity. The sideband gain is a consequence of an unbalanced dressed-state population distribution.
Abstract The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.