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Physical Review A

Detection of Rydberg-atom micromasers

L. Z. Wang

Published Jan 1, 1992• 5 citations
Publisher

Abstract

The lifetimes of Rydberg atoms have been considered in micromaser theory. The difference from the usual micromaser theory [P. Filipowicz, J. Javanainen, and P. Meystre, Phys. Rev. A 34, 3077 (1986)] without level decay rates is discussed. It is shown that when the atom-field interaction time is large, the quantum collapse and revival are significantly different from the prediction of the usual micromaser theory. The relation between the photon fluctuation and the fluctuation of the population of the lower level after interacting with a maser field is also discussed. We found that the consistency of the sub-Poisson statistics of the lower-level population and photon number is violated.

DOI
10.1103/physreva.45.r27

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Quantum revivals in micromasers

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A distinctive signature of the granulated nature of the electromagnetic field is the revivals known to occur in the dynamics of a two-level atom interacting with a single-field mode (Jaynes-Cummings model). The development of high-Q single-mode cavities combined with progress in Rydberg atom spectroscopy has led to a possibility of verifying these predictions. Revival experiments using micromasers have been performed by Walther et al. Here the cavity mode is first allowed to reach a steady state, and then probe atoms are injected into the resonator. By measuring their state as they exit the cavity, one can infer the state of the field. We show that the micromaser experiences Jaynes-Cummingslike revivals when the pump parameter θ is varied. However, in contrast to the conventional Jaynes-Cummings situation, which considers initially coherent fields, the micromaser photon statistics are usually not Poissonian and depend sensitively on θ. The micromaser revivals cannot be explained by a semiclassical theory or linearized quantum fluctuations about the semiclassical solution. Rather, an exact quantum treatment, considering fully the granularity of the cavity mode, is required.

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There are only fistful of systems in physics that can be described by an exact theory from first principles and, at the same time, can be investigated under experimental conditions approaching the idealized theoretical ones. The one-atom-maser or micromaser provides such an example, making a detailed study of the fundamental properties of the atom-field interaction possible. The situation realized in a micromaser is very close to the ideal case of a single two-level atom interacting with a single quantized mode of a cavity field. In the micromaser the atoms have a dual purpose of both pumping the field and also probing it via measurements of the outgoing atoms. Any other means of measuring the field inside the resonator has the detrimental effect of lowering its Q-factor and thereby the photon storage time. The long photon storage time of the resonator allows for the decay of the field to be negligible during the passage of an atom and its interaction with the field. The behavior of atoms in a cavity is governed by the oscillatory exchange of energy between the atoms and the field, which is called Rabi oscillation. For cavity fields in the vacuum and few photon number states (Fock states), Rabi oscillations have been measured in the past. To prevent thermal effects from polluting the pure number states these experiments were performed at low temperatures (below 1 K). However, the observed resolution of the Rabi oscillations measurements was quite disappointing (only about 2% of the predicted theoretical value) and precluded more ambitious experiments like atom-atom correlations or time resolved investigations of the maser field dynamics. The observed contrast of Rabi oscillations can be considered as a figure of merit for the experimental resolution of quantum features of a maser field. Therefore, a high resolution in the measurements of Rabi oscillations is crucial. This thesis describes the methods and improvements applied to enhance the resolution of Rabi oscillations by a factor of 8. The following upgrades and developments proved to be crucial in this work: 1) The base temperature of the cryogenic system was lowered to 0.3 K, i.e. one third of the original value. At the same time, the time during which the system remains at the base temperature was improved by almost of an order of magnitude (to more than 12 h). 2) For the promotion of the atoms to the Rydberg regime new three-step diode laser setup was constructed. The excitation efficiency compared to the old dye laser was increased by two orders. Using top-of-fringe stabilization with new spectroscopic methods, specially designed error detection and feedback schemes as well as state-of-the-art PID regulators the continuous locking of lasers is about 8 h (compared to about 20 min with the old dye laser system). 3) The flexibility of using the three step excitation allows to excite different maser states and for the first time to investigate pure maser transition. 4) Various improvements on the atomic oven and the channeltron detection unit led to the reliable and stable production and detection of the atomic beam. Observed distribution of the atomic beam statistics reaches to within 6% the Poisson limit which is expected in the absence of experimental imperfections. 5) New developed techniques in magnetic field compensation allow to perform such measurements with two orders of magnitude better accuracy compared to the previous experiments. To demonstrate the new capabilities of the apparatus and to apply its improved resolution of quantum fields we performed a previously impossible in-depth analysis of mean photon number and the atomic inversion produced by a micromaser for various detunings between the cavity- and atomic resonance frequency.

•Jan 1, 2009•0 citations

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A micromaser in standard operation produces entangled two-level atoms. This entanglement can be investigated in the correlations of atoms leaving the micromaser cavity in the upper and lower maser levels. The correlations contribute to the stabilization of the photon number in the cavity and are thus vital for the generation of sub-Poissonian statistics in the maser field. We review how various statistical signatures for this entanglement are calculated in micromaser theory, and report recent measurements that demonstrate the case. Ways are described leading to an optimal entanglement for the atoms in the micromaser.

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It is shown analytically that under certain experimental conditions the steady-state photon statistics of a micromaser field are directly connected to the fluctuation in number of the atoms in transition from the upper to the lower maser level under the influence of the maser field. The analytical results are compared to the results of a computer simulation of the maser process.

Physical Review A•Aug 1, 1990•134 citations
The lifetimes of Rydberg atoms have been considered in micromaser theory. The difference from the usual micromaser theory [P. Filipowicz, J. Javanainen, and P. Meystre, Phys. Rev. A 34, 3077 (1986)] without level decay rates is discussed. It is shown that when the atom-field interaction time is large, the quantum collapse and revival are significantly different from the prediction of the usual micromaser theory. The relation between the photon fluctuation and the fluctuation of the population of the lower level after interacting with a maser field is also discussed. We found that the consistency of the sub-Poisson statistics of the lower-level population and photon number is violated.
A distinctive signature of the granulated nature of the electromagnetic field is the revivals known to occur in the dynamics of a two-level atom interacting with a single-field mode (Jaynes-Cummings model). The development of high-Q single-mode cavities combined with progress in Rydberg atom spectroscopy has led to a possibility of verifying these predictions. Revival experiments using micromasers have been performed by Walther et al. Here the cavity mode is first allowed to reach a steady state, and then probe atoms are injected into the resonator. By measuring their state as they exit the cavity, one can infer the state of the field. We show that the micromaser experiences Jaynes-Cummingslike revivals when the pump parameter θ is varied. However, in contrast to the conventional Jaynes-Cummings situation, which considers initially coherent fields, the micromaser photon statistics are usually not Poissonian and depend sensitively on θ. The micromaser revivals cannot be explained by a semiclassical theory or linearized quantum fluctuations about the semiclassical solution. Rather, an exact quantum treatment, considering fully the granularity of the cavity mode, is required.
We describe the first investigation of the nonclassical radiation field of a micromaser. The maser cavity is cooled to 0.5 K to exclude thermal photons and has a quality factor 3\ifmmode\times\else\texttimes\fi{}1010{10}^{10}1010. Velocity-selected Rydberg atoms pump the maser. The photon statistics in the cavity are measured via the statistics of the atoms leaving the cavity in the lower maser level. Taking into account a detection efficiency of 10%, their fluctuations are reduced up to 40% below the Poisson level. This corresponds to photon-number fluctuations in the cavity of up to 70% below the vacuum-state limit.
The development of a single-atom maser or a micromaser allows a detailed study of the atom–field interaction. The situation realized is very close to the ideal case of a single two-level atom interacting with a single-mode quantized field as treated in Section 6.2. In a micromaser a stream of two-level atoms is injected into a superconducting cavity with a high quality factor. The injection rate can be such that only one atom is present inside the resonator at any time. Due to the high quality factor of the cavity, the radiation decay time is much larger than the characteristic time of the atom–field interaction, which is given by the inverse of the single-photon Rabi frequency. Therefore, a field is built up inside the cavity when the mean time between the atoms injected into the cavity is shorter than the cavity decay time. A micromaser, therefore, allows sustained oscillations with less than one atom on the average in the cavity. The realization of a single-atom maser or a micromaser has been made possible due to the enormous progress in the construction of superconducting cavities together with the laser preparation of highly excited atoms called Rydberg atoms. The quality factor of the superconducting cavities is high enough for periodic energy exchanges between atom and cavity field to be observed. The interesting properties of the Rydberg atoms make them ideal for micromasers. In Rydberg atoms the probability of induced transitions between adjacent states becomes very large and scales as n 4 , where n denotes the principle quantum number.
There are only fistful of systems in physics that can be described by an exact theory from first principles and, at the same time, can be investigated under experimental conditions approaching the idealized theoretical ones. The one-atom-maser or micromaser provides such an example, making a detailed study of the fundamental properties of the atom-field interaction possible. The situation realized in a micromaser is very close to the ideal case of a single two-level atom interacting with a single quantized mode of a cavity field. In the micromaser the atoms have a dual purpose of both pumping the field and also probing it via measurements of the outgoing atoms. Any other means of measuring the field inside the resonator has the detrimental effect of lowering its Q-factor and thereby the photon storage time. The long photon storage time of the resonator allows for the decay of the field to be negligible during the passage of an atom and its interaction with the field. The behavior of atoms in a cavity is governed by the oscillatory exchange of energy between the atoms and the field, which is called Rabi oscillation. For cavity fields in the vacuum and few photon number states (Fock states), Rabi oscillations have been measured in the past. To prevent thermal effects from polluting the pure number states these experiments were performed at low temperatures (below 1 K). However, the observed resolution of the Rabi oscillations measurements was quite disappointing (only about 2% of the predicted theoretical value) and precluded more ambitious experiments like atom-atom correlations or time resolved investigations of the maser field dynamics. The observed contrast of Rabi oscillations can be considered as a figure of merit for the experimental resolution of quantum features of a maser field. Therefore, a high resolution in the measurements of Rabi oscillations is crucial. This thesis describes the methods and improvements applied to enhance the resolution of Rabi oscillations by a factor of 8. The following upgrades and developments proved to be crucial in this work: 1) The base temperature of the cryogenic system was lowered to 0.3 K, i.e. one third of the original value. At the same time, the time during which the system remains at the base temperature was improved by almost of an order of magnitude (to more than 12 h). 2) For the promotion of the atoms to the Rydberg regime new three-step diode laser setup was constructed. The excitation efficiency compared to the old dye laser was increased by two orders. Using top-of-fringe stabilization with new spectroscopic methods, specially designed error detection and feedback schemes as well as state-of-the-art PID regulators the continuous locking of lasers is about 8 h (compared to about 20 min with the old dye laser system). 3) The flexibility of using the three step excitation allows to excite different maser states and for the first time to investigate pure maser transition. 4) Various improvements on the atomic oven and the channeltron detection unit led to the reliable and stable production and detection of the atomic beam. Observed distribution of the atomic beam statistics reaches to within 6% the Poisson limit which is expected in the absence of experimental imperfections. 5) New developed techniques in magnetic field compensation allow to perform such measurements with two orders of magnitude better accuracy compared to the previous experiments. To demonstrate the new capabilities of the apparatus and to apply its improved resolution of quantum fields we performed a previously impossible in-depth analysis of mean photon number and the atomic inversion produced by a micromaser for various detunings between the cavity- and atomic resonance frequency.
A micromaser in standard operation produces entangled two-level atoms. This entanglement can be investigated in the correlations of atoms leaving the micromaser cavity in the upper and lower maser levels. The correlations contribute to the stabilization of the photon number in the cavity and are thus vital for the generation of sub-Poissonian statistics in the maser field. We review how various statistical signatures for this entanglement are calculated in micromaser theory, and report recent measurements that demonstrate the case. Ways are described leading to an optimal entanglement for the atoms in the micromaser.