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Journal of Physics B Atomic Molecular and Optical Physics

Multimode entanglement and squeezing from coupled four-wave mixing oscillators

Huatang Tan, Wenwu Deng, He Huang

Published Oct 22, 2010• 2 citations
Publisher

Abstract

In this paper, we investigate the generation of multimode entanglement and squeezing of an optical field via coupled four-wave mixing interactions in a Kerr nonlinear medium pumped at multiple well-separated frequencies. We show that genuine multimode entanglement can be obtained and this entanglement can be verified with the measurable multimode squeezing present in the system. This scheme may be used to achieve entangled frequency combs which are useful in continuous-variable quantum communication networks.

DOI
10.1088/0953-4075/43/21/215507

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In this paper, we investigate the generation of multimode entanglement and squeezing of an optical field via coupled four-wave mixing interactions in a Kerr nonlinear medium pumped at multiple well-separated frequencies. We show that genuine multimode entanglement can be obtained and this entanglement can be verified with the measurable multimode squeezing present in the system. This scheme may be used to achieve entangled frequency combs which are useful in continuous-variable quantum communication networks.
The dynamical behavior of Kerr optical frequency combs is very well understood today from the perspective of the semiclassical approximation. These combs are obtained by pumping an ultrahigh-QQQ whispering-gallery mode resonator with a continuous-wave laser. The long-lifetime photons are trapped within the toruslike eigenmodes of the resonator, where they interact nonlinearly via the Kerr effect. In this article, we use quantum Langevin equations to provide a theoretical understanding of the nonclassical behavior of these combs when pumped below and above threshold. In the configuration where the system is under threshold, the pump field is the unique oscillating mode inside the resonator, and it triggers the phenomenon of spontaneous four-wave mixing, where two photons from the pump are symmetrically up- and down-converted in the Fourier domain. This phenomenon, also referred to as parametric fluorescence, can only be understood and analyzed from a fully quantum perspective as a consequence of the coupling between the field of the central (pumped) mode and the vacuum fluctuations of the various side modes. We analytically calculate the power spectra of the spontaneous emission noise, and we show that these spectra can be either single- or double-peaked depending on the value of the laser frequency, chromatic dispersion, pump power, and spectral distance between the central mode and the side mode of interest. We also calculate as well the overall spontaneous noise power per side mode and propose simplified analytical expressions for some particular cases. In the configuration where the system is pumped above threshold, we investigate the phenomena of quantum correlations and multimode squeezed states of light that can occur in the Kerr frequency combs originating from stimulated four-wave mixing. We show that for all stationary spatiotemporal patterns, the side modes that are symmetrical relative to the pumped mode in the frequency domain display quantum correlations that can lead to squeezed states of light under some optimal conditions that are analytically determined. These quantum correlations can persist regardless the dynamical state of the system (rolls or solitons), regardless of the spectral extension of the comb (number side modes) and regardless of the dispersion regime (normal or anomalous). We also explicitly determine the phase quadratures leading to photon entanglement and analytically calculate their quantum-noise spectra. For both the below- and above-threshold cases, we study with particular emphasis the two principal architectures for Kerr comb generation, namely the add-through and add-drop configurations. It is found that regardless of the configuration, an essential parameter is the ratio between out-coupling and total losses, which plays a key role as it directly determines the efficiency of the detected fluorescence or squeezing spectra. We finally discuss the relevance of Kerr combs for quantum information systems at optical telecommunication wavelengths below and above threshold.
Frequency combs are multimode photonic systems that underlie countless precision sensing and metrology applications. Since their invention over two decades ago, numerous efforts have pushed frequency combs to broader bandwidths and more stable operation. More recently, quantum squeezing and entanglement have been explored in single frequency comb systems for quantum advantages in sensing and signal multiplexing. However, the production of quantum light across multiple frequency combs remains unexplored. In this work, we theoretically explore a mechanism that generates a series of nonlinearly coupled frequency combs through cascaded three-wave upconversion and downconversion processes mediated by a single idler comb. We show how this system generates inter- and intracomb two-mode squeezing and entanglement spanning a very large spectral range, from ultraviolet to mid-IR frequencies. Finally, we show how this system can be engineered to produce on-demand multimode quantum light through covariance matrix optimization. Our findings could enable tunable broadband ghost spectroscopy protocols, squeezing-enhanced pump-probe measurements, and broadband entanglement between spectrally-multiplexed quanta of information.
We report on our research effort to generate large-scale multipartite optical-mode entanglement using as few physical resources as possible. We have previously shown that cluster-and GHZ-type N-partite continuous-variable entanglement can be obtained in an optical resonator that contains a suitably designed second-order nonlinear optical medium, pumped by at most O \mathcal{O} O (N 2) fields. In this paper, we show that the frequency comb of such a resonator can be entangled in an arbitrary number of independent 2 × 2 and 2 × 3 continuousvariable cluster states by a single optical parametric oscillator pumped by just a few optical modes.
Multimode nonclassical states of light are an essential resource in quantum computation with continuous variables [1]. They can be generated either by mixing different squeezed light sources using linear optical operations [2], or directly in a multimode optical device [3, 4]. Synchronously Pumped Optical Parametric Oscillators (SPOPO) — which correspond to an OPO pumped by a train of ultrashort pulses that are synchronized with the cavity round-trip time — have been theoretically shown to be promising devices for the generation of multimode nonclassical frequency combs, since a SPOPO is a sole optical cavity acting as an assembly of independent squeezers in a particular basis called the supermodes basis [5]. The supermodes are optical frequency combs with specific spectrum and phase profiles that are determined by the length of the intracavity nonlinear crystal and the pulse shape of the pump.
We describe the effects of Raman interactions on the quantum correlations of multimode optical fields. It is shown that both quantum beats and four-wave mixing processes exist in the Raman interactions of multimode fields with atomic reservoirs. These two mechanisms combine to lead to emission in pairs into multiple cavity modes. For four fields taken as examples, we find that the four-mode squeezed state can be created at steady state. From this we can obtain the Greenberger–Horne–Zeilinger entangled state, and the linear and square cluster entangled states. This scheme does not need the preparation of the initial states of atoms and cavity modes, and is robust against atomic spontaneous decay.