Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Applied Physics Letters

Transient electromagnetically induced transparency in self-assembled quantum dots

S. Marcinkevičius, A. Gushterov, J.P. Reithmaier

Published Jan 28, 2008• 103 citations
Publisher

Abstract

A coherent absorption dip in pump-probe experiment performed on a ten layer optically thin InGaAs∕GaAs quantum dot (QD) structure has been observed. Measurements performed for different wavelengths, polarizations, pulse widths, and temperatures allow assigning the dip to electromagnetically induced transparency (EIT). The EIT scheme is based on coupling of excitons with different spins in asymmetric QDs. Using spectrally narrow pulses, detrimental effect of the inhomogeneous broadening is reduced since only the QDs with transitions resonant with the pulse wavelength are addressed and participate in the EIT. The effect has been observed at temperatures up to 140K.

DOI
10.1063/1.2840160

Related papers

Transient electromagnetically induced transparency in InGaAs quantum dots

S. Marcinkevičius, A. Gushterov, J.P. Reithmaier

Electromagnetically induced transparency (EIT) based on exciton spin transitions is observed in InGaAs quantum dots. Inhomogeneous broadening of the quantum dot ensemble, detrimental for EIT, is effectively reduced by using spectrally narrow pulses.

Conference on Lasers and Electro-Optics•May 4, 2008•0 citations

Electromagnetically Induced Transparency in Semiconductor Quantum Wells

Mark C. Phillips, Hailin Wang

This chapter discusses advantage of the many-body Coulomb interactions to generate and manipulate nonradiative quantum coherences. It describes theoretically, the manifestation and behavior of electromagnetically induced transparency (EIT) processes in transient regimes. The chapter also discusses experimental demonstrations of EIT using excitons in gallium arsenide quantum-well structures. It shows that many-body Coulomb interactions between excitons can be exploited for the generation and manipulation of exciton spin coherence and biexciton coherence. The chapter provides the similarities and especially the essential differences in EIT processes between atomic and excitonic systems. It focuses on the changes in the absorption spectrum induced by EIT; these changes are also accompanied by corresponding changes in the refractive index. The absorption spectrum features a distinct EIT dip similar to that observed for cw excitations. The experimental setup for transient EIT studies was based on a standard transient pump-probe configuration, but with different pump and probe pulse durations.

CRC Press eBooks•Oct 3, 2018•0 citations

Exciton spin coherence and electromagnetically induced transparency in the transient optical response of GaAs quantum wells

Mark C. Phillips, Hailin Wang

We report experimental studies of electromagnetically induced transparency (EIT) arising from exciton spin coherence in the transient optical response of GaAs quantum wells. The exciton spin coherence, which is a direct result of Coulomb correlations between excitons with opposite spins, is induced via bound or unbound two-exciton states. Theoretical analyses based on a three-level model illustrate the manifestation of EIT in a transient regime and provide qualitative guidance for understanding the transient behaviors observed in the EIT experiments. Additional studies of the effects of exciton energy renormalization on optical Stark splitting also provide insights on how exciton many-body interactions can lead to unusual time-dependent asymmetric EIT line shapes.

Physical Review B•Mar 30, 2004•73 citations

Numerical investigation of electromagnetically induced transparency in a quantum dot structure

P. Kaer Nielsen, Henri Thyrrestrup, Jesper Mørk +1 more

.A numerical investigation of pulse propagation in a quantum dot structure in the regime of electromagnetically induced transparency is reported. The quantum dot is described as a cone on top of a wetting layer and the calculated energy levels and dipole moments are used in an effective three-level model. Pulse propagation characteristics such as degree of slowdown, absorption, and pulse distortion are investigated with respect to their dependence on the dephasing rates and pulse width. It is seen how Rabi oscillations can seriously distort the pulse when the spectral width of the pulse becomes too large compared to the width of the EIT window.

Optics Express•Jan 1, 2007•83 citations

Ultrafast Nonlinear Spectroscopy of Strain-compensated Quantum Dots

Junko Ishi‐Hayase

We investigate the dephasing mechanism of optically-induced exciton coherence in an ensemble of InAs self-assembled quantum dots (QDs) using a two-pulse photon-echo (PE) technique. The sample was fabricated on an InP (311)B substrate using strain compensation to control the emission wavelength. This technique also enabled us to fabricate a 150-layer stacked QD structure for enhancing the PE signal intensity. We show the measured decay time of PE signal intensity for resonant excitation of ground-state transition is extremely long, which corresponds to ultralong coherence times of excitons in our QDs. We confirmed that non-radiative population relaxation and pure dephasing are considerably smaller than the radiative relaxation at low temperature. Furthermore, we demonstrate the ultrafast coherent control of QD exciton polarization by changing the pulse areas (Rabi oscillations) in the PE experiment. We also propose a new scheme for implementing QD quantum memory by using the PE technique.

Hyomen Kagaku•Jan 1, 2011•0 citations

Transient nonlinear spectroscopy of indium arsenide quantum dots: Coherent and incoherent dynamics of confined excitons.

Anthony S. Lenihan

The three-dimensional confinement created by the ultrasmall semiconductor structures known as quantum dots greatly modifies the optical properties of the spatially localized carriers. These systems are presently of great interest to the research community, both for the improved understanding of the physics of confined structures, and for the potential applications of these systems to areas such as optoelectronics and quantum computing. Here, the techniques of transient coherent nonlinear optical spectroscopy are applied to the investigation of excitons confined within InAs/GaAs self-assembled quantum dots. These methods provide a powerful tool for the study of dynamic processes in these novel materials. The nonlinear measurements are based on the differential transmission experimental geometry, and utilize ultrafast pulsed lasers in order to temporally resolve the carrier dynamics after excitation. The experiments performed here are resonant with the ground state absorption of the quantum dots, as evidenced by comparison with the photoluminescence measurements which are used to characterize the sample. The incoherent relaxation dynamics of the population of photoexcited excitons are examined, allowing for a determination of both the lifetime of the excitons and the time scale for relaxation between the two polarization eigenstates of the system. The three-dimensional quantum confinement results in the suppression of these relaxation processes, as predicted. The use of coherent spectroscopic techniques allows for the first unambiguous demonstration of an optically-induced nonradiative Raman coherence in these quantum dots. Simultaneous excitation of both polarization states of the exciton results in a coherent superposition state, whose temporal evolution is observed through the homodyne-detection scheme. In these transient experiments, this is manifested as a beating in the nonlinear response, which allows us to directly measure the fine-structure splitting between the polarization states. Utilizing optical pulse shaping techniques, transient spectral hole burning is performed, which allows for the nonlinear response to be spectrally resolved. As expected for the strongly confined quantum dot excitons, the results show that diffusion among the localized states is not a significant effect. Temperature dependent measurements show that at elevated temperatures, extra dephasing processes, potentially related to acoustic phonon scattering, become important. Finally, this technique allows for the first direct observation of the induced absorption from the exciton to biexciton transition in these InAs quantum dots, and a measurement of the associated binding energy. These results lay the foundation for future studies in this material system, and for the possible development of quantum logic devices utilizing quantum dots.

•Jan 1, 2002•0 citations
A coherent absorption dip in pump-probe experiment performed on a ten layer optically thin InGaAs∕GaAs quantum dot (QD) structure has been observed. Measurements performed for different wavelengths, polarizations, pulse widths, and temperatures allow assigning the dip to electromagnetically induced transparency (EIT). The EIT scheme is based on coupling of excitons with different spins in asymmetric QDs. Using spectrally narrow pulses, detrimental effect of the inhomogeneous broadening is reduced since only the QDs with transitions resonant with the pulse wavelength are addressed and participate in the EIT. The effect has been observed at temperatures up to 140K.
This chapter discusses advantage of the many-body Coulomb interactions to generate and manipulate nonradiative quantum coherences. It describes theoretically, the manifestation and behavior of electromagnetically induced transparency (EIT) processes in transient regimes. The chapter also discusses experimental demonstrations of EIT using excitons in gallium arsenide quantum-well structures. It shows that many-body Coulomb interactions between excitons can be exploited for the generation and manipulation of exciton spin coherence and biexciton coherence. The chapter provides the similarities and especially the essential differences in EIT processes between atomic and excitonic systems. It focuses on the changes in the absorption spectrum induced by EIT; these changes are also accompanied by corresponding changes in the refractive index. The absorption spectrum features a distinct EIT dip similar to that observed for cw excitations. The experimental setup for transient EIT studies was based on a standard transient pump-probe configuration, but with different pump and probe pulse durations.
We report experimental studies of electromagnetically induced transparency (EIT) arising from exciton spin coherence in the transient optical response of GaAs quantum wells. The exciton spin coherence, which is a direct result of Coulomb correlations between excitons with opposite spins, is induced via bound or unbound two-exciton states. Theoretical analyses based on a three-level model illustrate the manifestation of EIT in a transient regime and provide qualitative guidance for understanding the transient behaviors observed in the EIT experiments. Additional studies of the effects of exciton energy renormalization on optical Stark splitting also provide insights on how exciton many-body interactions can lead to unusual time-dependent asymmetric EIT line shapes.
.A numerical investigation of pulse propagation in a quantum dot structure in the regime of electromagnetically induced transparency is reported. The quantum dot is described as a cone on top of a wetting layer and the calculated energy levels and dipole moments are used in an effective three-level model. Pulse propagation characteristics such as degree of slowdown, absorption, and pulse distortion are investigated with respect to their dependence on the dephasing rates and pulse width. It is seen how Rabi oscillations can seriously distort the pulse when the spectral width of the pulse becomes too large compared to the width of the EIT window.
We investigate the dephasing mechanism of optically-induced exciton coherence in an ensemble of InAs self-assembled quantum dots (QDs) using a two-pulse photon-echo (PE) technique. The sample was fabricated on an InP (311)B substrate using strain compensation to control the emission wavelength. This technique also enabled us to fabricate a 150-layer stacked QD structure for enhancing the PE signal intensity. We show the measured decay time of PE signal intensity for resonant excitation of ground-state transition is extremely long, which corresponds to ultralong coherence times of excitons in our QDs. We confirmed that non-radiative population relaxation and pure dephasing are considerably smaller than the radiative relaxation at low temperature. Furthermore, we demonstrate the ultrafast coherent control of QD exciton polarization by changing the pulse areas (Rabi oscillations) in the PE experiment. We also propose a new scheme for implementing QD quantum memory by using the PE technique.
The three-dimensional confinement created by the ultrasmall semiconductor structures known as quantum dots greatly modifies the optical properties of the spatially localized carriers. These systems are presently of great interest to the research community, both for the improved understanding of the physics of confined structures, and for the potential applications of these systems to areas such as optoelectronics and quantum computing. Here, the techniques of transient coherent nonlinear optical spectroscopy are applied to the investigation of excitons confined within InAs/GaAs self-assembled quantum dots. These methods provide a powerful tool for the study of dynamic processes in these novel materials. The nonlinear measurements are based on the differential transmission experimental geometry, and utilize ultrafast pulsed lasers in order to temporally resolve the carrier dynamics after excitation. The experiments performed here are resonant with the ground state absorption of the quantum dots, as evidenced by comparison with the photoluminescence measurements which are used to characterize the sample. The incoherent relaxation dynamics of the population of photoexcited excitons are examined, allowing for a determination of both the lifetime of the excitons and the time scale for relaxation between the two polarization eigenstates of the system. The three-dimensional quantum confinement results in the suppression of these relaxation processes, as predicted. The use of coherent spectroscopic techniques allows for the first unambiguous demonstration of an optically-induced nonradiative Raman coherence in these quantum dots. Simultaneous excitation of both polarization states of the exciton results in a coherent superposition state, whose temporal evolution is observed through the homodyne-detection scheme. In these transient experiments, this is manifested as a beating in the nonlinear response, which allows us to directly measure the fine-structure splitting between the polarization states. Utilizing optical pulse shaping techniques, transient spectral hole burning is performed, which allows for the nonlinear response to be spectrally resolved. As expected for the strongly confined quantum dot excitons, the results show that diffusion among the localized states is not a significant effect. Temperature dependent measurements show that at elevated temperatures, extra dephasing processes, potentially related to acoustic phonon scattering, become important. Finally, this technique allows for the first direct observation of the induced absorption from the exciton to biexciton transition in these InAs quantum dots, and a measurement of the associated binding energy. These results lay the foundation for future studies in this material system, and for the possible development of quantum logic devices utilizing quantum dots.