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Physical Review A

On-demand all-optical generation of controlled Rb-vapor densities in photonic-band-gap fibers

Amar R. Bhagwat, Aaron D. Slepkov, Vivek Venkataraman, Pablo Londero, Alexander L. Gaeta

Published Jun 5, 2009• 29 citations
Publisher

Abstract

We investigate the time dynamics of light-induced desorption of Rb atoms in hollow-core photonic-band-gap fibers and demonstrate all-optical generation of precisely controlled Rb-vapor densities. We also compare the performance of the desorption process in an unmodified fiber with one with an organosilane-coated core, and based on the vapor depletion and recovery behavior, we propose a mechanism to describe the desorption processes. We further demonstrate that high densities of Rb vapor can be generated after the desorption beam is switched off and use it to realize $\ensuremath{\Lambda}$-scheme electromagnetically induced transparency at control powers as low as 80 nW.

DOI
10.1103/physreva.79.063809

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•Apr 9, 2010•0 citations
We investigate the time dynamics of light-induced desorption of Rb atoms in hollow-core photonic-band-gap fibers and demonstrate all-optical generation of precisely controlled Rb-vapor densities. We also compare the performance of the desorption process in an unmodified fiber with one with an organosilane-coated core, and based on the vapor depletion and recovery behavior, we propose a mechanism to describe the desorption processes. We further demonstrate that high densities of Rb vapor can be generated after the desorption beam is switched off and use it to realize \ensuremathΛ\ensuremath{\Lambda}\ensuremathΛ-scheme electromagnetically induced transparency at control powers as low as 80 nW.
We show that a Rubidium vapor can be produced within the core of a photonic band-gap fiber yielding an optical depth in excess of 2000. Our technique for producing the vapor is based on coating the inner walls of the fiber core with an organosilane and using light-induced atomic desorption to release Rb atoms into the core. We develop a model to describe the dynamics of the atomic density, and as an initial demonstration of the potential of this system for supporting ultra-low-level nonlinear optical interactions, we perform electromagnetically-induced transparency with control-field powers in the nanowatt regime, which represents more than a 1000-fold reduction from the power required for bulk, focused geometries.
We demonstrate the ability to generate extremely large rubidium densities in uncoated hollow-core photonic band-gap fibers using light-induced atomic desorption. Once the fiber is exposed to Rb vapor for 1-2 weeks, and this atomic source is removed, the fiber yields large desorbable densities for an extended period of time. We show that optical depths greater than e(-1200) can be created within seconds. Our observed Rb densities are several orders of magnitude larger than any previously reported to be generated optically, and allow for the demonstration of a relatively easy-to-use fiber-based vapor cell capable of producing large optical depths without the need for thermal tuning.
We show that rubidium vapor can be produced within the core of a photonic band-gap fiber yielding an optical depth in excess of 2,000. Our technique for producing the vapor is based on coating the inner walls of the fiber core with organosilane and using light-induced atomic desorption to release Rb atoms into the core. As an initial demonstration of the potential of this system for supporting ultralow-level nonlinear optical interactions, we perform electromagnetically induced transparency with control-field powers in the nanowatt regime, which represents more than a 1,000-fold reduction from the power required for bulk, focused geometries.
Low-light-level optical nonlinearities are of significant interest for performing operations such as single-photon switching and quantum non-demolition measurements on single-photons. To evoke strong nonlinearities from singlephotons, one can enhance the matter-photon interaction using strongly nonlinear materials such as alkali vapors in combination with an appropriate geometry such as a waveguide, which provides a long interaction length while maintaining a small light mode area. We demonstrate for the first time that such a system can be experimentally realized by loading rubidium vapor inside a hollow-core photonic band-gap fiber. Using the technique of light-induced atomic desorption in this geometry, we have generated optical depths greater than 1000. As a proof of principle, we demonstrate electromagnetically induced transparency (EIT) with control powers 1000 times lower than those used for hot vapor cells in a focused beam geometry. Working with such a high aspect ratio geometry requires us to identify and measure the various sources of decoherence via spectroscopy of desorbed atoms in the fiber. Using such techniques, we also estimate the temperature of the desorbing atoms inside the fiber. The desorption mechanism is studied, and we show that pulsed desorption beams of the right amplitude and duration can be used for generating precisely controlled optical depths. Finally, we investigate the use of various buffer gas techniques for increasing the effective transverse path of the atoms as they move across the fiber in order to reduce their ground state decoherence and map this effect as a function of buffer gas pressure.