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Nonlinear Guided Waves and Their Applications

Negative group velocities in quasi-phase-matched second-order nonlinear optical interactions

Stefano Longhi, P. Laporta, Marcello Marano

Published Jan 1, 2002• 0 citations
Publisher

Abstract

The existence of anomalous, i.e. superluminal or negative, group velocities [1] provides one of the most amazing phenomenon of wave propagation which is compatible with, and even a consequence of, causality [2]. Anomalous wave propagation generally relies on the resonant interaction of light with an atomic medium, i.e. it exploits the dispersive properties of absorptive [3] or inverted [4,5] atomic media near resonances. Evanescent wave propagation across photonic barriers [1] provides the other wide framework where anomalous group velocities have been observed, however in such cases the achievement of a negative group velocity seems unlikely. By exploiting the dispersive properties of a gain doublet, a narrow spectral region of transparent anomalous dispersion around the dip center of two Lorentzian gain lines, leading to negative transit times and no pulse attenuation, can be created [4]. A recent demonstration thereof has been indeed reported in an experiment by Wang and coworkers using Cs vapor [5].

DOI
10.1364/nlgw.2002.nlmd4

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Scientific Reports•Apr 9, 2013•22 citations
The existence of anomalous, i.e. superluminal or negative, group velocities [1] provides one of the most amazing phenomenon of wave propagation which is compatible with, and even a consequence of, causality [2]. Anomalous wave propagation generally relies on the resonant interaction of light with an atomic medium, i.e. it exploits the dispersive properties of absorptive [3] or inverted [4,5] atomic media near resonances. Evanescent wave propagation across photonic barriers [1] provides the other wide framework where anomalous group velocities have been observed, however in such cases the achievement of a negative group velocity seems unlikely. By exploiting the dispersive properties of a gain doublet, a narrow spectral region of transparent anomalous dispersion around the dip center of two Lorentzian gain lines, leading to negative transit times and no pulse attenuation, can be created [4]. A recent demonstration thereof has been indeed reported in an experiment by Wang and coworkers using Cs vapor [5].
Anomalous dispersion cannot occur in a transparent passive medium where electromagnetic radiation is being absorbed at all frequencies, as pointed out by Landau and Lifshitz. Here we show, both theoretically and experimentally, that transparent linear anomalous dispersion can occur when a gain doublet is present. Therefore, a superluminal light-pulse propagation can be observed even at a negative 7group velocity through a transparent medium with almost no pulse distortion. Consequently, a negative transit time is experimentally observed resulting in the peak of the incident light pulse to exit the medium even before entering it. This counterintuitive effect is a direct result of the rephasing process owing to the wave nature of light and is not at odds with either causality or Einstein's theory of special relativity.
Optical pulse propagation in photonic grating structures can show anomalous (i.e., superluminal or negative) group velocities under certain circumstances owing to the anomalous dispersive properties induced by the periodic grating structure. Such phenomena can be observed for either linear pulse propagation in passive dielectric grating structures, such as in fiber Bragg gratings (FBGs), as well as in frequency-conversion processes exploiting second-order cascading effects in quasi-phase-matched (QPM) nonlinear crystals. Engineering of the grating structure can be exploited to observe a wide variety of anomalous pulse transmission and reflection behaviors. In this article, we review the main recent experimental and theoretical achievements obtained by our group in this field. In particular, we report on superluminal propagation of picosecond optical pulses at the 1.5-μm wavelength of optical communications in FBGs, both in transmission and reflection configurations, with the observation of group velocities as large as ∼5c/sub 0/. We also show that the phenomenon of transparent pulse propagation at a negative group velocity in a gain doublet atomic amplifier, recently observed in cesium vapor by Wang and co-workers (L. J. Wang, A. Kuzmich, and A. Dogariu, Nature vol.406, p.277-9, 2000), can be achieved as well in a photonic parametric amplifier by exploiting the anomalous dispersive properties of the amplifier induced by a suitably designed QPM grating profile.
The mechanisms leading to a seemingly superluminal propagation of light in dispersive media are examined. The anomalous dispersion near an absorption line, involved in the first experiments displaying negative group velocity propagation, is shown to be not only simpler but also more efficient than the so-called transparent dispersion used in the later experiments of Wang et al. (Nature (London) 406, 277 (2000)) and of Dogariu et al. (Phys.Rev.A 63, 053806 (2001)). The modest pulse advances observed by these authors can in particular be reproduced with a better overall transmittance of the medium and the significant advances attained with a single-line arrangement would probably be unattainable with their gain-doublet arrangement.
In the region between two lines of a doublet of an inverted medium, there exists a point of zero group-velocity dispersion, where highly superluminal effects may be observable without significant gain, loss, distortion, or broadening. The results of this group-velocity analysis hold for sufficiently narrow-band, analytic pulses, and do not constitute a violation of causality, although the group, ``signal,'' and energy velocities as defined by Sommerfeld and Brillouin may all exceed c or even become negative. No sharp disturbance in the pulse (a real signal) could propagate faster than light, but the scheme offers an unusual noiseless amplification scheme for the leading edge of a pulse, both at the classical and at the single-photon level.
Summary form only given. We use gain-assisted linear anomalous dispersion to demonstrate superluminal light pulse propagation with a negative group velocity through a transparent atomic medium. We place two Raman gain peaks closely to obtain an essentially lossless anomalous dispersion region that results in a superluminal group velocity. The group velocity of a pulse in this region exceeds c and can even become negative,while the shape of the pulse is preserved. We measured a negative group velocity index of n/sub g/=-315(/spl plusmn/5). Experimentally, a light pulse propagating through the spin-polarized atomic vapor cell exits from it earlier than propagating through the same distance in vacuum by a time difference that is 315 times of the vacuum light propagation time L/c=0.2 ns.
Scientific community has well recognized that a Lorentzian medium exhibits anomalous dispersion behavior in its resonance absorption region. To satisfy the Krammers-Kronig relation, such an anomalous region has to be accompanied with significant loss, and thus, experimental observations of negative group velocity in this region generally require a gain-assisted approach. In this letter, we demonstrate that the negative group velocity can also be observed in the absence of absorption resonance. We show that the k-surface of a passive uniaxial Lorentzian medium undergoes a distortion near the plasma frequency. This process yields an anomalous dispersion bandwidth that is far away from the absorption resonance region, and enables the observation of negative group velocity at the plasma frequency band. Introducing anomalous dispersion in a well-controlled manner would greatly benefit the research of ultrafast photonics and find potential applications in optical delay lines, optical data storage and devices for quantum information processing.