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International Conference on Atomic Physics (ICAP)

High-resolution, high-accuracy spectroscopy of trapped ions

Dana J. Berkeland, J.D. Miller, Flávio C. Cruz, Brent C. Young, Robert J. Rafac, Xinyi Huang, Wayne M. Itano, Jonas Bergquist, D. J. Wineland

Published Jan 1, 1999• 1 citation
Publisher

Abstract

Microwave spectroscopy using trapped and cooled ions can achieve precision and accuracy comparable to the best cesium frequency standards. We discuss standards based on 199Hg+ ions trapped in linear Paul traps: the Jet Propulsion Laboratory (JPL) standard, which uses up to 107 atoms confined near the trap axis, and the recently evaluated NIST standard, which uses approximately ten ions laser cooled and crystalized on the trap axis. We consider future directions in trapped ion frequency standard work, including the use of entangled states for achieving higher precision, and progress on trapped ion optical frequency standards. Finally, we discuss scientific and technical applications of extremely stable frequency standards.

DOI
10.1063/1.59372

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Microwave spectroscopy using trapped and cooled ions can achieve precision and accuracy comparable to the best cesium frequency standards. We discuss standards based on 199Hg+ ions trapped in linear Paul traps: the Jet Propulsion Laboratory (JPL) standard, which uses up to 107 atoms confined near the trap axis, and the recently evaluated NIST standard, which uses approximately ten ions laser cooled and crystalized on the trap axis. We consider future directions in trapped ion frequency standard work, including the use of entangled states for achieving higher precision, and progress on trapped ion optical frequency standards. Finally, we discuss scientific and technical applications of extremely stable frequency standards.
Microwave spectroscopy using trapped and cooled ions can achieve precision and accuracy comparable to the best cesium frequency standards. We discuss standards based on 199Hg+ ions trapped in linear Paul traps: the Jet Propulsion Laboratory (JPL) standard, which uses up to 107 atoms confined near the trap axis, and the recently evaluated NIST standard, which uses approximately ten ions laser cooled and crystalized on the trap axis. We consider future directions in trapped ion frequency standard work, including the use of entangled states for achieving higher precision, and progress on trapped ion optical frequency standards. Finally, we discuss scientific and technical applications of extremely stable frequency standards.
Experimental research toward the realization of an optical frequency standard of high accuracy is briefly reviewed. The studies concentrated on single, laser-cooled ions since they offer several attractive features for the achievement of high accuracy. These features include long storage time which eliminates transit-time broadening, confinement that is nearly nonperturbative to the internal level structure of the ion, laser-cooling that reduces motional shifts to small values, and electron-shelving whereby transitions to long-lived states can be detected with unit probability. The authors studied spectroscopically the electric-quadrupole allowed transition at 282 nm in a single, laser-cooled /sup 199/Hg/sup +/ ion stored in an RF Paul trap with extremely high resolution. The measured linewidth is limited by the spectral purity of the laser to about 80 Hz. Possible improvements and future directions are discussed.>
We discuss frequency standards based on laser-cooled 199Hg+ ions confined in cryogenic rf traps. In one experiment, the frequency of a microwave source is served to the ions' ground-state hyperfine transition at 40.5 GHz. For seven ions and a Ramsey free precession time of 100 s, the fractional frequency stability is 3.3 (2) X 10-13 (tau) -1/2 for measurement times (tau) < 2 h. The ground-state hyperfine interval is measured to be 40 507 347 996.841 59 (14) (41) Hz, where the first number in parentheses is the uncertainty due to statistics and systematic errors, and the second is the uncertainty in the frequency of the time scale to which the standard is compared. In a second experiment under development, a strong-binding cryogenic trap will confine a single ion used for an optical frequency standard based on a narrow electric quadrupole transition at 282 nm. The bandwidth of the laser used to drive this transition is less than 10 Hz at 563 nm.
Transitions between discrete energy levels in well-isolated atomic systems are highly reproducible and therefore make ideal references for highly accurate frequency standards or clocks. In particular, a single laser-cooled ion confined in a radiofrequency ion trap closely approximates the spectroscopic ideal of a particle at rest in a perturbation-free environment. Narrow optical transitions in such systems are therefore very promising for the realization of optical clocks with accuracy around 2 orders of magnitude higher than current microwave primary standards. In this paper the fundamental aspects, current performance and applications of trapped ion optical clocks are reviewed and the potential for future improvements is considered.