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Journal of Physics B Atomic Molecular and Optical Physics

Trapping and cooling of Sr+ions: strings and large clouds

S. Removille, Romain Dubessy, B. Dubost, Quentin C. Glorieux, T. Coudreau, S. Guibal, J.-P. Likforman, Luca Guidoni

Published Jul 15, 2009• 19 citations
Publisher

Abstract

This paper reports on trapping and laser cooling of singly ionized strontium ions in a linear Paul trap. We describe the loading technique based on two-photon absorption of femtosecond pulses at a wavelength of 431 nm and we compare this technique to electron-bombardment ionization. We perform Doppler cooling of the ions in the few-ions regime as well as in the case of large clouds. The analysis of the fluorescence spectra and direct imaging of the cloud allows us to identify the Coulomb-crystal regime. These experiments open the way to the use of a large cold trapped-ion cloud as a medium for quantum optics and quantum information experiments.

DOI
10.1088/0953-4075/42/15/154014

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This paper reports on trapping and laser cooling of singly ionized strontium ions in a linear Paul trap. We describe the loading technique based on two-photon absorption of femtosecond pulses at a wavelength of 431 nm and we compare this technique to electron-bombardment ionization. We perform Doppler cooling of the ions in the few-ions regime as well as in the case of large clouds. The analysis of the fluorescence spectra and direct imaging of the cloud allows us to identify the Coulomb-crystal regime. These experiments open the way to the use of a large cold trapped-ion cloud as a medium for quantum optics and quantum information experiments.
This paper reports on trapping and laser-cooling of singly-ionized strontium ions in a linear Paul trap. We demonstrate loading of large ion clouds containing as much as 106 ions and laser cooling down to the Coulomb crystal transition. We observe the spatial segregation of the different Sr+ isotopes due to the mass-dependent Paul trap stiffness. Sympathetic cooling of the different isotopes is demonstrated, either by laser-cooling of 88Sr+ (83% abundance) or of 86Sr+ (10% abundance). These demonstrations open the way to the use of a large ion Coulomb crystal for quantum optics and quantum information experiments, where the strong confinement, the long lifetime, and the absence of perturbation by cooling lasers are crucial.
We report a demonstration of simple and effective loading of strontium ions into a linear radio frequency Paul trap using photoionization. The ionization pathway is 5s2 1S0 -- 5s5p 1P1 -- 5p2 1D2, and the 5p2 1D2 final state is auto-ionizing. Both transitions are driven using diode lasers: a grating-stabilized 922 nm diode doubled in a single pass through potassium niobate to 461 nm and a bare diode at 405 nm. Using this technique, we have reduced the background pressure during the ion loading process by a factor of 2 compared to the conventional technique of electron bombardment. Initial ion temperatures are low enough that the ions immediately form crystals. It is also possible to observe the trapping region with a CCD camera during ion creation, allowing specific ion number loading with high probability.
The use of cold trapped ions for quantum information processing requires the preparation of linear strings of ions at low temperatures and the coherent manipulation by laser light of the quantum state of individual ions in the string. In our experiment, 40Ca+ ions are trapped in a linear Paul trap, forming crystallized linear strings when laser cooled. These strings are observed by fluorescence detection on the S1/2-P1/2 dipole transition at 397 nm using a photomultiplier and a CCD camera. The narrow S1/2-D5/2 quadrupole transition at 729 nm is used to investigate and manipulate the vibrational motion of the ion in the trap. The spectral resolution obtained up to now on this transition is 2 · 10—12, proving long coherence time of the two-level system. Addressing of individual ions in the string is achieved, using a tightly focused laser beam at 729 nm, and detected by the observation of quantum jumps from the S1/2 to the D5/2 level. These experimental techniques make ions in a superposition of their S1/2 and D5/2 states suitable as qubits for quantum information processing. The realization of a two-ion quantum gate furthermore requires ground-state cooling of the string. The status of current experiments is reviewed and techniques to achieve ground-state cooling of ion strings are discussed.
We have developed an apparatus integrating resonance-ionization, ion-trap, and laser-cooling techniques for an ultratrace radioactive isotope 90Sr^{90}\mathrm{Sr}90Sr analysis. Trapped 90Sr+^{90}\mathrm{Sr}^{+}90Sr+ isotope ions were laser cooled, and their $4d\phantom{\rule{0.16em}{0ex}}^{2}D_{3/2}\ensuremath{\rightarrow}5p\phantom{\rule{0.16em}{0ex}}^{2}P_{1/2}$ transition isotope shift was experimentally measured to be $\ensuremath{-}281(17)$ MHz by comparing individual spectra of 88Sr+^{88}\mathrm{Sr}^{+}88Sr+ and 90Sr+^{90}\mathrm{Sr}^{+}90Sr+ ions. Crystallization of 90Sr+^{90}\mathrm{Sr}^{+}90Sr+ was carried out using the resonance frequency value confirmed in our experiment, and then 90Sr+^{90}\mathrm{Sr}^{+}90Sr+ individual ions were successfully observed.
We describe a efficient way to photoionize strontium atoms in a linear radio-frequency trap. We use a 2-photon second order process to excite the autoionization resonance (4d2 + 5p2) 1D2. A doubled pulsed Ti:Saphire laser system is used at 431nm to provide 100fsec pulses at 82Mhz. The fabrication of the laser systems for addressing the Sr+ transitions necessary for laser cooling and excitation of quantum jumps, vacuum system and ion trap structure are also described in detail. With the current setup a easy and repeatable trapping of linear ion chains is achieved at UHV pressures.