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Physica C Superconductivity

Charge excitations and resonant inelastic X-ray scattering in ladder cuprates

Kenji Tsutsui, Takami Tohyama, Sadamichi Maekawa

Published Mar 29, 2007• 1 citation
Publisher
DOI
10.1016/j.physc.2007.03.188

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arXiv:cond-mat/0303242•Physical Review Letters•Sep 11, 2003•59 citations
Resonant inelastic x-ray scattering (RIXS) has become an important tool for studying elementary excitations in correlated materials. Here, we present a systematic theoretical investigation of the Cu LLL-edge RIXS spectra of undoped and doped cuprate two-leg spin-ladders in both the non-spin-conserving (NSC) and spin-conserving (SC) channels. The spectra are rich and host many exotic excitations. In the NSC channel of the undoped case, we identify one-triplon and bound triplet two-triplon excitations in the strong rung coupling limit, as well as confined spinons in the weak rung coupling limit. In the doped case, we observe a quasiparticle excitation formed from a bound charge and spin-1/21/21/2 in the strong rung coupling limit. In the SC channel, we also identify several new features, including bound singlet two-triplon excitations and confined spinons in the undoped ladders in the strong and weak rung coupling limits, respectively. Conversely, in the doped case, the SC channel primarily probes both gapless and gapped charge excitations. Finally, we revisit the available data for the ladder compound Sr14Cu24O41{\mathrm{Sr}}_{14}{\mathrm{Cu}}_{24}{\mathrm{O}}_{41}Sr14​Cu24​O41​ in the context of our results.
Predictions are made for the momentum- and carrier-dependent degradation of the Mott gap upon doping in high-T(c) cuprates as would be observed in Cu K-edge resonant inelastic x-ray scattering (RIXS). The two-dimensional Hubbard model with second- and third-nearest-neighbor hopping terms has been studied by numerical exact diagonalization. Special emphasis is placed on the particle-hole asymmetry of the Mott gap excitations. We argue that the Mott gap excitations observed by RIXS are significantly influenced by the interaction between charge carriers and antiferromagnetic correlations.