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Physical Review Letters

Microwave Excitation of Rydberg Atoms in the Presence of Noise

R. Blümel, R. Graham, Leszek Sirko, Uzy Smilansky, HERBERT WALTHER, Koichi Yamada

Published Jan 23, 1989• 84 citations
Publisher

Abstract

We study theoretically and experimentally the effect of noise on Rydberg atoms passing through a strong coherent microwave field. We derive a master equation containing the coherent field exactly. Its solution reveals the presence of four universal dynamical regimes: (i) an initial classical regime, (ii) a subsequent coherent localized regime, (iii) a transition, induced by the noise, in which coherence and localization are destroyed, and (iv) the final regime, where equidistribution over the quasienergy states is reached.

DOI
10.1103/physrevlett.62.341

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We study theoretically and experimentally the effect of noise on Rydberg atoms passing through a strong coherent microwave field. We derive a master equation containing the coherent field exactly. Its solution reveals the presence of four universal dynamical regimes: (i) an initial classical regime, (ii) a subsequent coherent localized regime, (iii) a transition, induced by the noise, in which coherence and localization are destroyed, and (iv) the final regime, where equidistribution over the quasienergy states is reached.
We present experimental and theoretical results on highly excited Rydberg atoms passing through a waveguide. The waveguide is excited in a coherent mode with a superimposed component of technically generated noise. In the theoretical part of the paper we derive and solve a master equation for a Rydberg atom driven by a monochromatic coherent microwave field in the presence of noise. We show that a Rydberg atom subjected to a mixture of coherent modes and noise fields exhibits four dynamical regimes: (i) diffusive broadening, (ii) localization, (iii) destruction of coherence and localization, and (iv) relaxation to equilibrium. The four regimes are passed one after the other as a function of irradiation time. They occur on different time scales and are thus temporally well separated from each other. The theory is checked by an experiment on the time dependence of the population distribution of highly excited rubidium Rydberg atoms initially prepared in a unique and well-defined Rydberg state and irradiated by a strong microwave field. The localization regime, characterized by a ``freezing'' of the width of the wave packet with respect to the Rydberg levels, has been observed. The addition of a small noise component was shown to lead to delocalization after times inversely proportional to the noise power, as predicted by our theory.
The work presented in this dissertation concerns dynamics of Rydberg atom lattices in the presence of noise and dissipation. Rydberg atoms possess a number of exaggerated properties, such as a strong van der Waals interaction. The interplay of that interaction, coherent driving and decoherence leads to intriguing non-equilibrium phenomena. Here, we study the non-equilibrium physics of driven atom lattices in the presence of decoherence caused by either laser phase noise or strong decay. In the first case, we compare between global and local noise and explore their effect on the number of excitations and the full counting statistics. We find that both types of noise give rise to a characteristic distribution of the Rydberg excitation number. The main method employed is the Langevin equation but for the sake of efficiency in certain regimes, we use a Markovian master equation and Monte Carlo rate equations, respectively. In the second case, we consider dissipative systems with more general power-law interactions. We determine the phase diagram in the steady state and analyse its generation dynamics using Monte Carlo rate equations. In contrast to nearest-neighbour models, there is no transition to long-range-ordered phases for realistic interactions and resonant driving. Yet, for finite laser detunings, we show that Rydberg atom lattices can undergo a dissipative phase transition to a long-range-ordered antiferromagnetic phase. We identify the advantages of Monte Carlo rate equations over mean field predictions. Having studied the dynamics of Rydberg atom lattices, we study an application of the strong interactions in such systems for quantum information processing. We investigate the coherent exchange of a single photon between a superconducting microwave cavity and a lattice of strongly interacting Rydberg atoms in the presence of local electric field fluctuations plaguing the cavity surface. We show that despite the increased sensitivity of Rydberg states to electric fields, as compared to ground state atoms, the Rydberg dipole-dipole interaction can be used to protect the system against the dephasing induced by the local noise. Using 1/f1/f1/f and laser phase noise models, we show that compared to the case with non-interacting atoms, our system exhibits longer coherence lifetimes and larger retrieval efficiency of the photon after storing into the atoms.
In this chapter experiments on rubidium Rydberg atoms in external fields are reviewed [1 – 8]. In the first part results on the interaction of microwave radiation with rubidium Rydberg atoms are described. The Rydberg atoms interact with a microwave pulse of a well-defined duration. When applying coherent microwave radiation with a frequency exceeding a certain value, the experimentally observed microwave field strength at which 10% of the atoms are ionized has to be much larger than the value found by classical trajectory calculations. The atoms are stabilized by the dynamical localization. An extremely weak microwave broadband noise which is added to the coherent wave at least partially destroys the localization. This phenomenon depends on the bandwidth of the added noise. In further experiments the dependence of the 10% ionization microwave field strength on the duration τ of the microwave pulse has been investigated. For increasing noise level the 10% ionization field strength ∈ 0.1 develops from a behavior ∈ 0.1 ∼ τ −1/4 to a ∈ 0.1 ∼ τ −1/2 dependence, which is characteristic for a classical diffusion process. The second part of the chapter deals with experiments in strong static crossed electric and magnetic fields. Below as well as above the ionization energy the observed quasi-Landau(QL)-resonances are explained using classical trajectories. The ionization behavior of the QL-resonances is clearly influenced by the spatial structure of the associated classical orbits. In further experiments the dependence of the observed ionization energy on the magnetic field was investigated in the presence of a fixed static electric field.
We examine the theory of potential scattering of Rydberg atoms in a microwave field. The model of a three-level atom is employed to calculate the radiative force emerging in the resonant coherent interaction with the microwave field for the case of a two-photon resonance and high intensities, using the method of quasienergies of the system consisting of the atom and the field. We determine the probabilities of Landau-Zener transitions in the spatial regions where under two-photon resonance conditions the quasienergies of the atoms approach one another by a small quantity. We also study the dynamics of the variation of the spatial profile of a beam of Rydberg atoms caused by resonant scattering. Finally, we give the results of the first experimental observation of the variation of the transverse beam profile when Rydberg atoms pass through a nonuniform microwave field formed in a rectangular waveguide and in resonance with the two-photon 36 P –37 P transition.
We examine theoretically the recent experiments of Lange and Walther on the dynamical interaction of Rydberg atoms in a microwave cavity in the presence of a strong driving field. In particular, we study how the intense field renormalizes the cavity-induced spontaneous emission. For this purpose we derive the master equation for the atomic dynamics by adiabatically eliminating the cavity-field variables, while treating the intense driving field nonperturbatively. We present analytical and numerical solutions of the master equation, taking into account the turn on and turn off of the atom-field coupling in the rest frame of the atoms, as well as the velocity distribution of the atomic beam. We obtain good agreement between theoretical results and experiments.