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Chemical Physics

Optical Bloch equations and enhanced decay of Rabi oscillations in strong driving fields

Taras Plakhotnik

Published Nov 7, 2005• 4 citations
Publisher
DOI
10.1016/j.chemphys.2005.08.027

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We extend the exciton population equations of a two-level quantum dot system with weak excitation to the ones with strong excitations, in which, the phonon-induced intensity-dependent dephasing time and decay rate are involved. The straightforward calculated populations from the modified population equations demonstrate the damping behavior of Rabi oscillation as the external field increasing. The effect of the intensity-dependent dephasing time and the intensity-dependent decay rate are also discussed.
A superfluorescence effect in a V-type medium with initial Raman inversion, driven by a strong coherent field on one of the transitions, is studied analytically and numerically. It is shown that the collective spontaneous emission evolves in the presence of a minor population of an upper state of a superfluorescent transition. In the limit of the Rabi frequency of a driving field large compared to that of a superfluorescent pulse, the system of two equations for the fields and density-matrix equations for three states of the medium is reduced to Maxwell-Bloch equations for an effective two-level system. The shape of a superfluorescent pulse is perfectly described in terms of a slowly varying envelope function (which is a solution of the Maxwell-Bloch equations), filled with fast oscillations associated with Rabi floppings on the driving transition. In the average, i.e., after integrating over a period of Rabi oscillations, the upper superfluorescent state is populated less than other states, such that the phenomenon may be called ``superfluorescence without inversion'' by analogy with lasing without inversion.
A qubit--harmonic-oscillator open system coupled to thermal baths was considered and the master equation describing the evolution of the open system was deduced when the qubit transition frequency is $\ensuremath{\lesssim}0.1$ the oscillator frequency. The master equation is valid in all the qubit-oscillator state space and holds for all values of the qubit-oscillator coupling including the ultrastrong and deep strong coupling regimes. It only requires an oscillator frequency much larger than the relaxation rates. The qubit-oscillator coupling can enhance or decrease both the relaxation rates and the frequency shifts induced by the thermal baths. It was found that weak, sinusoidal qubit driving forces the qubit-oscillator open system to behave like a driven qubit whose evolution is governed by equations similar to those of the Bloch vector in the optical Bloch equations and whose transition frequency decreases with increasing qubit-oscillator coupling strength. Finally, it was shown how one can reach the adiabatic regime by using sinusoidal qubit driving with large driving frequency and the concepts of $\ensuremath{\pi}$ and $\ensuremath{\pi}/2$ pulses were generalized to manipulate transitions between dressed states.