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Optica Acta International Journal of Optics

Conditions for Sub-poissonian Photon Statistics and Squeezed States in Resonance Fluorescence

Henk F. Arnoldus, Gerard Nienhuis

Published Nov 1, 1983• 50 citations
Publisher

Abstract

We study the conditions for sub-poissonian photon statistics and squeezed states in the field of resonance fluorescence of a two-state atom. These conditions as a function of the detuning from resonance, the linewidth and the Rabi frequency have some overlap, but they are largely complementary. Super-poissonian statistics arise for small linewidths and large detunings, irrespective of the Rabi frequency. Squeezed states require small linewidths and either low or moderate Rabi frequencies, or large detunings from resonance.

DOI
10.1080/713821098

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We study the conditions for sub-poissonian photon statistics and squeezed states in the field of resonance fluorescence of a two-state atom. These conditions as a function of the detuning from resonance, the linewidth and the Rabi frequency have some overlap, but they are largely complementary. Super-poissonian statistics arise for small linewidths and large detunings, irrespective of the Rabi frequency. Squeezed states require small linewidths and either low or moderate Rabi frequencies, or large detunings from resonance.
We have studied the statistics of fluorescent photons emitted by a two-state atom in a laser beam in the limit where either the detuning or the Rabi frequency is large. For this case, the spectrum of resonance fluorescence has three separated lines. We have obtained closed form expressions for the conditional probability density for the emission of the nth photon and for the probability for emission of n photons in a time interval [0,T]. Our solutions are complementary to the known solutions for the case of perfect resonance.
The statistical fluctuations of light can, under certain circumstances, exhibit a number of interesting nonclassical features. These include photon antibunching, sub-Poissonian statistics, and squeezing, all of which exist only in a quantum field. The three effects are distinct, and do not necessarily go together, although the first two are sometimes mistakenly treated as interchangeable. Both photon antibunching and sub-Poissonian statistics have been observed in experiments on resonance fluorescence from single atoms, which is described. Squeezing has not yet been seen experimentally, although many nonlinear processes are expected to give rise to it. The squeezed state can be recognized in heterodyne or homodyne experiments, where the squeezing becomes manifest as sub-Poissonian photon fluctuations.
It is pointed out that, although squeezing and sub-Poissonian photon statistics need not go together, in the sense that an electromagnetic field may exhibit one but not the other, the method that is normally used to detect a squeezed state automatically generates sub-Poissonian photon statistics. However, when these considerations are applied to the fluorescence from a coherently driven atom, which exhibits both squeezing and sub-Poisson fluctuations, one finds that the statistics of the emitted photons show even larger departures from classical field theory than the squeezing.
The authors present analytical and numerical results for resonance fluorescence produced by a two-level atom damped by a broad-band squeezed vacuum. Previous theoretical analyses of this model have assumed that the laser frequency and the carrier frequency of the squeezed vacuum are equal. The authors introduce a non-zero detuning between the laser frequency and the carrier frequency while maintaining resonance between the laser frequency and atomic resonance. In the absence of the driving field there is a squeezing threshold: above threshold the decay rate of the atomic polarization can be reduced, and below threshold a squeezing-induced two peak spectrum and frequency shift, which is analogous to the Bloch-Siegert shift, are predicted. In the presence of the driving field, the spectrum is asymmetric for Rabi frequencies smaller or comparable to the detuning of the squeezed vacuum. A symmetric spectrum is obtained for large Rabi frequencies. An interpretation is predicted by means of a dressed-state analysis. The authors find that for not too large Rabi frequencies a remarkably large population inversion can be induced in the dressed states, even at exact resonance of the driving field, provided that the laser frequency and carrier frequency are detuned. Moreover, for detection times larger than the inverse detuning, the spectrum is insensitive to the phase between the driving field and the squeezed vacuum, in marked contrast to the case of no detuning.